Wednesday, December 31, 2008

ISI Web of Knowledge Alert - Ghosh, S

ISI Web of Knowledge Citation Alert (Solaris 2.1)

Cited Article: Ghosh, S. Carbon nanotube flow sensors
Alert Expires: 22 OCT 2009
Number of Citing Articles: 1 new records this week (1 in this e-mail)
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Title:
DEP-Based Fabrication and Characterization of Electronic-Grade CNTs for Nano-Sensing Applications

Authors:
Ouyang, MX; Sin, MLY; Chow, GCT; Li, WJ; Han, XL; Janzen, DC

Author Full Names:
Ouyang, Mengxing; Sin, Mandy L. Y.; Chow, Gary C. T.; Li, Wen J.; Han, Xuliang; Janzen, Daniel C.

Source:
2007 7TH IEEE CONFERENCE ON NANOTECHNOLOGY, VOL 1-3 : 1-6 2007

Language:
English

Document Type:
Proceedings Paper

Author Keywords:
Dielectrophoresis; Electronic-grade carbon nanotubes; Micro/nano sensing; Humidity sensor

Keywords Plus:
CARBON; SENSORS; WALL

Abstract:
Sensing devices using electronic-grade carbon nanotubes (EG-CNTs) as resistive sensing element were fabricated by dielectrophoresis (DEP) manipulation. DEP-based fabrication of EG-CNTs is important as it allows some control of the nominal resistance of the fabricated sensors, which is essential to improve the SNR of CNT sensors. The devices were characterized and the potential of EG-CNTs to serve as a novel temperature and humidity sensing element has been demonstrated. Electrical characterization revealed that the EG-CNTs sensors, which exhibit large linear IN range, have both positive and negative TCR at higher operational temperatures. In addition, its resistance-humidity linear dependency proves its humidity sensing capability. Moreover, the EG-CNTs device is capable of operating in nW range. On the foundation of these measurements, we aim to prove EG-CNTs as a promising material for future applications in nano-sensing.

Reprint Address:
Han, XL, Brewer Sci Inc, Rolla, MO USA.

Research Institution addresses:
[Ouyang, Mengxing; Sin, Mandy L. Y.; Chow, Gary C. T.; Li, Wen J.] Chinese Univ Hong Kong, Dept Mech & Automat Engn, Ctr Micro & Nanosyst, Shatin, Hong Kong, Peoples R China

Cited References:
BARONE PW, 2005, NAT MATER, V4, P86, DOI 10.1038/nmat1276.
CHEN Z, 2005, SENS LETT, V3, P274, DOI 10.1166/sl.2005.045.
DRESSELHAUS MS, 1992, NATURE, V358, P195.
FUNG CMKM, 2004, IEEE T NANOTECHNOL, V3, P395, DOI 10.1109/TNANO.2004.834156.
GHOSH S, 2003, SCIENCE, V299, P1042, DOI 10.1126/science.1079080.
HAN X, 2006, FLEXIBLE THIN FILM T.
IIJIMA S, 1991, NATURE, V354, P56.
KONG J, 2000, SCIENCE, V287, P622.
MEYYAPPAN M, 2005, CARBON NANOTUBES SCI, P6.
NA PS, 2005, APPL PHYS LETT, V87, P44.
NAEEMI A, 2007, IEEE ELECTR DEVICE L, V28, P135, DOI 10.1109/LED.2006.889240.
NAEEMI A, 2007, P INT S PHYS DES, P77.
REICH S, 2004, CARBON NANOTUBES BAS, P3.
VARGHESE OK, 2001, SENSOR ACTUAT B-CHEM, V81, P32.
VICTOR TS, 2003, IEEE ICRA, V3, P3648.
WU JA, 2004, PHYS REV B, V69, P53409.
YEOW JT, NANOTECHNOL, V17, P5441.
ZAHAB A, 2000, PHYS REV B, V62, P10000.

Cited Reference Count:
18

Times Cited:
0

Publisher:
IEEE; 345 E 47TH ST, NEW YORK, NY 10017 USA

IDS Number:
BIO98

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ISI Web of Knowledge Alert - Majumder M

ISI Web of Knowledge Citation Alert (Solaris 2.1)

Cited Article: Majumder M. Nanoscale hydrodynamics - Enhanced flow in carbon nanotubes
Alert Expires: 18 OCT 2009
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Title:
The Role of the Substrate Surface Morphology and Water in Growth of Vertically Aligned Single-Walled Carbon Nanotubes

Authors:
Pint, C; Pheasant, S; Nicholas, N; Horton, C; Hauge, R

Author Full Names:
Pint, Cary; Pheasant, Sean; Nicholas, Nolan; Horton, Charles; Hauge, Robert

Source:
JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY 8 (11): 6158-6164 NOV 2008

Language:
English

Document Type:
Proceedings Paper

Author Keywords:
Aligned Single-Walled Carbon Nanotubes; Growth; Morphology

Keywords Plus:
CHEMICAL-VAPOR-DEPOSITION; FILMS; KINETICS; ARRAYS

Abstract:
Growth of high quality, vertically aligned single-walled carbon nanotubes (carpets) is achieved using a rapid insertion hot filament chemical vapor deposition (HF-CVD) technique. The effect of the substrate morphology on growth is explored by comparing carpets grown on epitaxially polished MgO substrates to those grown on "as-cut," macroscopically rough MgO substrates. Depending on the substrate morphology, we observe differences in both the overall carpet morphology as well as the diameter distribution of nanotubes grown in the carpet based on optical measurements. In addition, we explore the role of water in the growth of carpets on MgO and the conventional Al2O3 coated Si substrates. We find that the addition of a small amount of water is beneficial to the growth rates of the SWNT carpets, enhancing the growth rates by up to eight times.

Reprint Address:
Hauge, R, Rice Univ, Dept Chem, Houston, TX 77005 USA.

Research Institution addresses:
[Pheasant, Sean; Horton, Charles; Hauge, Robert] Rice Univ, Dept Chem, Houston, TX 77005 USA; [Pint, Cary; Nicholas, Nolan] Rice Univ, Dept Phys & Astron, Houston, TX 77005 USA; [Pint, Cary; Pheasant, Sean; Nicholas, Nolan; Horton, Charles; Hauge, Robert] Rice Univ, Richard E Smalley Inst Nanoscale Sci & Technol, Houston, TX 77005 USA

Cited References:
AMAMA P, UNPUB.
BACHILO SM, 2002, SCIENCE, V298, P2361, DOI 10.1126/science.1078727.
CHAKRABARTI S, 2006, JPN J APPL PHYS 2, V45, L720, DOI 10.1143/JJAP.45.L720.
CORRY C, 2008, J PHYS CHEM B, V112, P1427.
ERES G, 2005, J PHYS CHEM B, V109, P16684, DOI 10.1021/jp051531i.
ERICSON LM, 2004, SCIENCE, V305, P1447.
GE L, 2007, P NATL ACAD SCI USA, V104, P10792.
HATA K, 2004, SCIENCE, V306, P1362.
JIANG KL, 2002, NATURE, V419, P801.
LI ZR, 2007, APPL PHYS LETT, V90, P3115.
MAJUMDER M, 2005, NATURE, V438, P44, DOI 10.1038/43844a.
MURAKAMI Y, 2004, CHEM PHYS LETT, V385, P298, DOI 10.1016/j.cplett.2003.12.095.
OKITA A, 2006, JPN J APPL PHYS 1, V45, P8323, DOI 10.1143/JJAP.45.83231.
PHEASANT S, UNPUB.
PISANA S, 2007, PHYSICA E, V37, P1, DOI 10.1016/j.physe.2006.06.014.
PURETZKY AA, 2005, APPL PHYS A-MATER, V81, P223, DOI 10.1007/s00339-005-3256-7.
QU L, 2007, ADV MATER, V19, P3844, DOI 10.1002/adma.200700023.
WANG WL, 2006, CHEM PHYS LETT, V419, P81, DOI 10.1016/j.cplett.2005.10.140.
WOOD RF, 2007, PHYS REV B, V75, P5446.
XIONG GY, 2006, CARBON, V44, P969, DOI 10.1016/j.carbon.2005.10.015.
XU YQ, 2006, APPL PHYS LETT, V89, P23116.
YU H, 2006, CARBON, V44, P1706, DOI 10.1016/j.carbon.2006.01.002.
ZHANG GY, 2005, P NATL ACAD SCI USA, V102, P16141, DOI 10.1073/pnas.0507064102.
ZHONG GF, 2005, JPN J APPL PHYS 1, V44, P1558, DOI 10.1143/JJAP.44.1558.
ZHONG GF, 2006, CARBON, V44, P2009, DOI 10.1016/j.carbon.2006.01.027.
ZHONG GF, 2007, J PHYS CHEM B, V111, P1907, DOI 10.1021/jp067776s.

Cited Reference Count:
26

Times Cited:
0

Publisher:
AMER SCIENTIFIC PUBLISHERS; 25650 NORTH LEWIS WAY, STEVENSON RANCH, CA 91381-1439 USA

Subject Category:
Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter

ISSN:
1533-4880

DOI:
10.1166/jnn.2008.SW26

IDS Number:
379IV

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Friday, December 19, 2008

ISI Web of Knowledge Alert - Ghosh, S

ISI Web of Knowledge Citation Alert (Solaris 2.1)

Cited Article: Ghosh, S. Carbon nanotube flow sensors
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Title:
Directed assembly of carbon nanotubes on soft substrates for use as a flexible biosensor array

Authors:
Koh, J; Yi, M; Lee, BY; Kim, TH; Lee, J; Jhon, YM; Hong, S

Author Full Names:
Koh, Juntae; Yi, Mihye; Lee, Byung Yang; Kim, Tae Hyun; Lee, Joohyung; Jhon, Young Min; Hong, Seunghun

Source:
NANOTECHNOLOGY 19 (50): Art. No. 505502 DEC 17 2008

Language:
English

Document Type:
Article

Keywords Plus:
FIELD-EFFECT TRANSISTORS; HIGH-PERFORMANCE; SENSORS; ELECTRONICS; DEVICES; SURFACE; NOISE; WIRES; FILMS; FLOW

Abstract:
We have developed a method to selectively assemble and align carbon nanotubes (CNTs) on soft substrates for use as flexible biosensors. In this strategy, a thin oxide layer was deposited on soft substrates via low temperature plasma enhanced chemical vapor deposition, and a linker-free assembly process was applied on the oxide surface where the assembly of carbon nanotubes was guided by methyl-terminated molecular patterns on the oxide surface. The electrical characterization of the fabricated CNT devices exhibited a typical p-type gating effect and 1/f noise behavior. The bare oxide regions near CNTs were functionalized with glutamate oxidase to fabricate selective biosensors to detect two forms of glutamate substances existing in different situations: L-glutamic acid, a neurotransmitting material, and monosodium glutamate, a food additive.

Reprint Address:
Koh, J, Seoul Natl Univ, Dept Phys & Astron, Seoul 151747, South Korea.

Research Institution addresses:
[Koh, Juntae; Lee, Byung Yang; Kim, Tae Hyun; Lee, Joohyung; Hong, Seunghun] Seoul Natl Univ, Dept Phys & Astron, Seoul 151747, South Korea; [Yi, Mihye] Korea Res Inst Chem Technol, Taejon 305343, South Korea; [Jhon, Young Min] Korea Inst Sci & Technol, Seoul 136791, South Korea

E-mail Address:
shong@phya.snu.ac.kr

Cited References:
AVOURIS P, 2007, NAT NANOTECHNOL, V2, P605, DOI 10.1038/nnano.2007.300.
BESTEMAN K, 2003, NANO LETT, V3, P727, DOI 10.1021/nl034139u.
BRADLEY K, 2003, NANO LETT, V3, P1353, DOI 10.1021/nl0344864.
BRIMAN M, 2006, J APPL PHYS, V100, ARTN 013505.
CHEN ZH, 2006, SCIENCE, V311, P1735, DOI 10.1126/science.1122797.
DUTTA P, 1981, REV MOD PHYS, V53, P497.
GHOSH S, 2003, SCIENCE, V299, P1042, DOI 10.1126/science.1079080.
HILLERED L, 1990, ACTA NEUROCHIR, V102, P91.
HUANG Y, 2001, SCIENCE, V291, P630.
IIJIMA S, 1991, NATURE, V354, P56.
IM J, 2006, J CHEM PHYS, V124, ARTN 224707.
JAVEY A, 2003, NATURE, V424, P654, DOI 10.1038/nature01797.
JAVEY A, 2004, NANO LETT, V4, P447, DOI 10.1021/nl035185x.
KANG J, 2008, NANOTECHNOLOGY, V19, ARTN 135305.
KANG SJ, 2007, NANO LETT, V7, P3343, DOI 10.1021/nl071596s.
KANG SJ, 2007, NAT NANOTECHNOL, V2, P230, DOI 10.1038/nnano.2007.77.
KARPOVICH DS, 1994, LANGMUIR, V10, P3315.
KOEHNE J, 2003, NANOTECHNOLOGY, V14, P1239.
KONG J, 1998, NATURE, V395, P878.
KONG J, 2000, SCIENCE, V287, P622.
KRUPKE R, 2003, SCIENCE, V301, P344, DOI 10.1126/science.1086534.
LEE AC, 2007, NANOTECHNOLOGY, V18, ARTN 455102.
LEE M, 2006, NAT NANOTECHNOL, V1, P66, DOI 10.1038/nnano.2006.46.
MAUNE H, 2006, APPL PHYS LETT, V89, ARTN 173131.
MEITL MA, 2004, NANO LETT, V4, P1643, DOI 10.1021/nl0491935.
MODI A, 2003, NATURE, V424, P171, DOI 10.1038/nature01777.
MYUNG S, 2005, ADV MATER, V17, P2361, DOI 10.1002/adma.200500682.
PARK JU, 2006, ANGEW CHEM INT EDIT, V45, P581, DOI 10.1002/anie.200501799.
RAO SG, 2003, NATURE, V425, P36, DOI 10.1038/425036a.
REZA S, 2006, J APPL PHYS, V99, ARTN 114309.
RUNDLETT KL, 1994, CHIRALITY, V6, P277.
SNOW ES, 2004, APPL PHYS LETT, V85, P4172, DOI 10.1063/1.1812838.
SNOW ES, 2005, SCIENCE, V307, P1942, DOI 10.1126/science.1109128.
SOLIVERES S, 2007, APPL PHYS LETT, V90, ARTN 082107.
SOMEYA T, 2003, NANO LETT, V3, P877, DOI 10.1021/nl034061h.
SUN Y, 2007, APPL PHYS LETT, V90, ARTN 213107.
SUN YG, 2007, ADV MATER, V19, P2818, DOI 10.1002/adma.200602975.
TANS SJ, 1997, NATURE, V386, P474.
VALENTINI L, 2003, APPL PHYS LETT, V82, P961, DOI 10.1063/1.1545166.
WANG YH, 2006, P NATL ACAD SCI USA, V103, P2026, DOI 10.1073/pnas.0511022103.

Cited Reference Count:
40

Times Cited:
0

Publisher:
IOP PUBLISHING LTD; DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND

Subject Category:
Engineering, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied

ISSN:
0957-4484

DOI:
10.1088/0957-4484/19/50/505502

IDS Number:
376TK

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ISI Web of Knowledge Alert - Hummer, G

ISI Web of Knowledge Citation Alert (Solaris 2.1)

Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
Alert Expires: 22 OCT 2009
Number of Citing Articles: 10 new records this week (10 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Water-Induced Programmable Synthesis of Water Pores

Authors:
Perez-Hernandez, N; Roux, MV; Febles, M; Morales, EQ; Perez, C; Fort, D; Martin, JD

Author Full Names:
Perez-Hernandez, Natalia; Roux, M. Victoria; Febles, Martin; Morales, Ezequiel Q.; Perez, Cirilo; Fort, Diego; Martin, Julio D.

Source:
ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS 222 (8-9): 1105-1116 2008

Language:
English

Document Type:
Article

Author Keywords:
Confined Water; Hydrophobic Effect; Hydrophobic Hydration; Water Channels; Chemical Models

Keywords Plus:
HYDROGEN-BOND NETWORK; INFRARED-SPECTROSCOPY; LIQUID H2O; DYNAMICS; CHANNEL; SELECTIVITY; CONDUCTION; MOLECULES

Abstract:
A time-sequential approach to study the hydration thermodynamics of designed organic compacts should prove useful ill other cases where cavities are occupied by multiple water molecules, i.e. natural cell water channels as aquaporins.

Reprint Address:
Perez-Hernandez, N, Free Univ Berlin, Takustr 3, D-14195 Berlin, Germany.

Research Institution addresses:
[Perez-Hernandez, Natalia] Free Univ Berlin, D-14195 Berlin, Germany; [Roux, M. Victoria] CSIC, Inst Quim Fis Rocasolano, E-28006 Madrid, Spain; [Febles, Martin; Perez, Cirilo] Univ La Laguna, Inst Bioorgan, CSIC, E-38206 Tenerife, Spain; [Morales, Ezequiel Q.] CSIC, Inst Prod Nat & Agrobiol, Tenerife 38206, Spain; [Fort, Diego; Martin, Julio D.] CSIC, Inst Invest Quim, Seville 41092, Spain

E-mail Address:
natalia@chemie.fu-berlin.de

Cited References:
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COWAN ML, 2005, NATURE, V434, P199, DOI 10.1038/nature03383.
DUTZLER R, 2002, NATURE, V415, P287.
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FECKO CJ, 2003, SCIENCE, V301, P1698.
FERSHT AR, 1993, PHILOS T ROY SOC A, V345, P141.
FUJIYOSHI Y, 2002, CURR OPIN STRUC BIOL, V12, P509.
GRUBMULLER H, 2003, P NATL ACAD SCI USA, V414, P156.
HILL AM, 2001, RES SCI EDUC, V31, P117.
HUMMER G, 2001, NATURE, V414, P188.
JAHNIG F, 1983, P NATL ACAD SCI-BIOL, V80, P3691.
KLEIN ML, 2001, SCIENCE, V291, P2106.
KOGA K, 2000, NATURE, V408, P564.
LAAGE D, 2006, SCIENCE, V311, P832, DOI 10.1126/science.1122154.
LEVINGER NE, 2002, SCIENCE, V298, P1722.
MORAISCABRAL JH, 2001, NATURE, V414, P37.
OHMINE I, 1999, ACCOUNTS CHEM RES, V32, P741.
PEREZ C, 2000, ORG LETT, V2, P1185.
PEREZHERNANDEZ N, 2004, BIOORGAN MED CHEM, V12, P1305, DOI 10.1016/j.bmc.2003.06.006.
RUAN CY, 2004, SCIENCE, V304, P80.
SUI HX, 2001, NATURE, V414, P872.
TAJKHORSHID E, 2002, SCIENCE, V296, P525.
TANFORD C, 1980, HYDROPHOBIC EFFECT F.
TIELEMAN DP, 2001, Q REV BIOPHYS, V34, P473.
TOKMAKOFF A, 2007, SCIENCE, V317, P54, DOI 10.1126/science.1144515.
WANG J, 2004, PHYS CHEM CHEM PHYS, V100, P7421.
WERNET P, 2004, SCIENCE, V304, P995, DOI 10.1126/science.1096205.

Cited Reference Count:
31

Times Cited:
0

Publisher:
OLDENBOURG VERLAG; LEKTORAT MINT, POSTFACH 80 13 60, D-81613 MUNICH, GERMANY

Subject Category:
Chemistry, Physical

ISSN:
0942-9352

DOI:
10.1524/zpch.2008.5378

IDS Number:
376CU

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Title:
A new physical model for resonance shear measurement of confined liquids between solid surfaces

Authors:
Mizukami, M; Kurihara, K

Author Full Names:
Mizukami, Masashi; Kurihara, Kazue

Source:
REVIEW OF SCIENTIFIC INSTRUMENTS 79 (11): Art. No. 113705 NOV 2008

Language:
English

Document Type:
Article

Author Keywords:
chemical analysis; liquid crystals; liquid structure; liquid theory; mica; organic compounds; rheology; tribology

Keywords Plus:
FORCES; WATER; FILM

Abstract:
This paper describes a new physical model for resonance shear measurement. The resonance shear method developed by us provides a tool for investigating the rheological and tribological properties of liquids confined between two surfaces as a function of the surface distance from micrometer to zero (contact) with nanometer level resolution with high sensitivity and stability. The properties of the confined liquid can be quantitatively studied by analyzing the resonance curve using a physical model. However, the quantitative analysis using the previously developed model was applicable only for the condition of the relatively low liquid viscosity (below similar to 100 Pa s). A new physical model described in this paper enabled us to continuously analyze the properties of confined liquids at all distances, which was not possible by the previous model. It became possible to calculate the movement of a lower surface and the shear rate applied on the confined sample using the param!
eters obtained from the resonance curves.

Reprint Address:
Kurihara, K, Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Aoba Ku, Katahira 2-1-1, Sendai, Miyagi 9808577, Japan.

Research Institution addresses:
[Kurihara, Kazue] Tohoku Univ, Inst Multidisciplinary Res Adv Mat, Aoba Ku, Sendai, Miyagi 9808577, Japan; JST CREST, Tokyo, Japan

E-mail Address:
kurihara@tagen.tohoku.ac.jp

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Cited Reference Count:
20

Times Cited:
0

Publisher:
AMER INST PHYSICS; CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA

Subject Category:
Instruments & Instrumentation; Physics, Applied

ISSN:
0034-6748

DOI:
10.1063/1.3012811

IDS Number:
376WB

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Title:
Interactions between amino acid side chains in cylindrical hydrophobic nanopores with applications to peptide stability

Authors:
Vaitheeswaran, S; Thirumalai, D

Author Full Names:
Vaitheeswaran, S.; Thirumalai, D.

Source:
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA 105 (46): 17636-17641 NOV 18 2008

Language:
English

Document Type:
Article

Author Keywords:
confinement effects on protein stability; hydrophobic interactions; potentials of mean force; water in pores

Keywords Plus:
PROTEIN STABILITY; MOLECULAR CONFINEMENT; WATER; DYNAMICS; SIMULATIONS; HYDRATION; RIBOSOME; NANOTUBE; HELICES; SPACES

Abstract:
Confinement effects on protein stability are relevant in a number of biological applications ranging from encapsulation in the cylindrical cavity of a chaperonin, translocation through pores, and structure formation in the exit tunnel of the ribosome. Consequently, free energies of interaction between amino acid side chains in restricted spaces can provide insights into factors that control protein stability in nanopores. Using all-atom molecular dynamics simulations, we show that 3 pair interactions between side chains-hydrophobic (Ala-Phe), polar (Ser-Asn) and charged (Lys-Glu)-are substantially altered in hydrophobic, water-filled nanopores, relative to bulk water. When the pore holds water at bulk density, the hydrophobic pair is strongly destabilized and is driven to large separations corresponding to the width and the length of the cylindrical pore. As the water density is reduced, the preference of Ala and Phe to be at the boundary decreases, and the contact pair is p!
referred. A model that accounts for the volume accessible to Phe and Ala in the solvent-depleted region near the pore boundary explains the simulation results. In the pore, the hydrogen-bonded interactions between Ser and Asn have an enhanced dependence on their relative orientations, as compared with bulk water. When the side chains of Lys and Glu are restrained to be side by side, parallel to each other, then salt bridgeformation is promoted in the nanopore. Based on these results, we argue and demonstrate that for a generic amphiphilic sequence, cylindrical confinement is likely to enhance thermodynamic stability relative to the bulk.

Reprint Address:
Thirumalai, D, Univ Maryland, Biophys Program, Inst Phys Sci & Technol, College Pk, MD 20742 USA.

Research Institution addresses:
[Vaitheeswaran, S.; Thirumalai, D.] Univ Maryland, Biophys Program, Inst Phys Sci & Technol, College Pk, MD 20742 USA; [Thirumalai, D.] Univ Maryland, Dept Chem & Biochem, College Pk, MD 20742 USA

E-mail Address:
thirum@umd.edu

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Cited Reference Count:
33

Times Cited:
0

Publisher:
NATL ACAD SCIENCES; 2101 CONSTITUTION AVE NW, WASHINGTON, DC 20418 USA

Subject Category:
Multidisciplinary Sciences

ISSN:
0027-8424

DOI:
10.1073/pnas.0803990105

IDS Number:
377BB

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Title:
Kohn-Sham-Like Approach toward a Classical Density-Functional Theory of Inhomogeneous Polar Molecular Liquids: An Application to Liquid Hydrogen Chloride

Authors:
Lischner, J; Arias, TA

Author Full Names:
Lischner, Johannes; Arias, T. A.

Source:
PHYSICAL REVIEW LETTERS 101 (21): Art. No. 216401 NOV 21 2008

Language:
English

Document Type:
Article

Keywords Plus:
NONUNIFORM POLYATOMIC SYSTEMS; WATER; TRANSITION; FLUIDS; FORCE

Abstract:
The Gordian knot of density-functional theories for classical molecular liquids remains finding an accurate free-energy functional in terms of the densities of the atomic sites of the molecules. Following Kohn and Sham, we show how to solve this problem by considering noninteracting molecules in a set of effective potentials. This shift in perspective leads to an accurate and computationally tractable description in terms of simple three-dimensional functions. We also treat both the linear- and saturation- dielectric responses of polar systems, presenting liquid hydrogen chloride as a case study.

Reprint Address:
Lischner, J, Cornell Univ, Atom & Solid State Phys Lab, Ithaca, NY 14853 USA.

Research Institution addresses:
[Lischner, Johannes; Arias, T. A.] Cornell Univ, Atom & Solid State Phys Lab, Ithaca, NY 14853 USA

Cited References:
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Cited Reference Count:
28

Times Cited:
0

Publisher:
AMER PHYSICAL SOC; ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA

Subject Category:
Physics, Multidisciplinary

ISSN:
0031-9007

DOI:
10.1103/PhysRevLett.101.216401

IDS Number:
375VI

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Title:
Movement of hydrogen molecules in pristine, hydrogenated and nitrogen-doped single-walled carbon nanotubes

Authors:
Oh, KS; Kim, DH; Park, S; Lee, JS; Kwon, O; Choi, YK

Author Full Names:
Oh, Kyung Su; Kim, Dong Hyun; Park, Seungho; Lee, Joon Sik; Kwon, Ohmyoung; Choi, Young Ki

Source:
MOLECULAR SIMULATION 34 (10-15): 1245-1252 2008

Language:
English

Document Type:
Article

Author Keywords:
carbon nanotube; self-diffusion coefficient of hydrogen molecules; velocity autocorrelation function; molecular dynamics simulation; density functional theory

Keywords Plus:
ACCELERATED DIFFUSION; JOSEPHSON-JUNCTIONS; ANOMALOUS DIFFUSION; DYNAMICS METHODS; CHAOTIC SYSTEMS; ADSORPTION; TEMPERATURE; FLOW; CONDUCTION

Abstract:
Carbon nanotubes (CNT) are considered promising nano-scale materials because of their unique structural, mechanical and electronic properties. Due to their long seamless cylindrical shaped structures they could be applied as effective nano-channels for mass transfer and relevant storages for hydrogen molecules. We study hydrogen transport mechanisms in CNTs for various chiral indices and different peculiarities, using the molecular dynamics simulation and quantum mechanical approach. Various CNT models such as pristine, hydrogenated and doped by nitrogen atoms of zigzag (10,0), chiral (7,5) and armchair (6,6) types with hydrogen molecules diffusing inside are simulated at 300K. The behaviour of hydrogen molecules inside CNTs is analysed using mean-square displacements and velocity autocorrelation functions. From the quantum mechanical approach, the electronic density distribution of CNT is calculated to verify the smooth characteristics of inner surfaces of nanotubes.

Reprint Address:
Park, S, Hongik Univ, Dept Mech & Syst Design Engn, Seoul, South Korea.

Research Institution addresses:
[Park, Seungho] Hongik Univ, Dept Mech & Syst Design Engn, Seoul, South Korea; [Oh, Kyung Su; Kim, Dong Hyun] Hongik Univ, Dept Mech Engn, Seoul, South Korea; [Lee, Joon Sik] Seoul Natl Univ, Sch Mech & Aerosp Engn, Seoul, South Korea; [Kwon, Ohmyoung] Korea Univ, Dept Mech Engn, Seoul, South Korea; [Choi, Young Ki] Chung Ang Univ, Sch Mech Engn, Seoul 156756, South Korea

E-mail Address:
spark@hongik.ac.kr

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Cited Reference Count:
53

Times Cited:
0

Publisher:
TAYLOR & FRANCIS LTD; 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND

Subject Category:
Chemistry, Physical; Physics, Atomic, Molecular & Chemical

ISSN:
0892-7022

DOI:
10.1080/08927020802129958

IDS Number:
375BR

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Title:
Water infiltration behaviours in carbon nanotubes under quasi-static and dynamic loading conditions

Authors:
Cao, GX; Qiao, Y; Zhou, QL; Chen, X

Author Full Names:
Cao, Guoxin; Qiao, Yu; Zhou, Qulan; Chen, Xi

Source:
MOLECULAR SIMULATION 34 (10-15): 1267-1274 2008

Language:
English

Document Type:
Article

Author Keywords:
carbon nanotube; water; infiltration; pressure; loading rate

Keywords Plus:
TRANSPORT; PRESSURE; PATTERNS

Abstract:
The mechanisms of pressure-driven water infiltration into single walled carbon nanotubes are explored using molecular dynamics simulations. Both quasi-static and dynamic loading conditions are investigated, and the influence of tube size is examined. Under quasi-static loading, the water molecules flow into the tube via surface diffusion at a low pressure and when the external pressure reaches a critical value, the infiltrated water flux can sharply increase to a steady state. Upon dynamic loading, the nominal infiltration length per unit external work is employed to measure the comprehensive effect of the loading rate. It is found that such factor is larger (i.e. infiltration is easier) at a lower loading rate and a larger tube size, which is closely related with the interactions between water molecules and nanotube wall atoms.

Reprint Address:
Chen, X, Columbia Univ, Columbia Nanomech Res Ctr, Dept Civil Engn & Engn Mech, New York, NY 10027 USA.

Research Institution addresses:
[Cao, Guoxin; Zhou, Qulan; Chen, Xi] Columbia Univ, Columbia Nanomech Res Ctr, Dept Civil Engn & Engn Mech, New York, NY 10027 USA; [Qiao, Yu] Univ Calif San Diego, Dept Struct Engn, La Jolla, CA 92093 USA; [Zhou, Qulan] Xian Jiaotong Univ, State Key Lab Power Engn Multiphase Flow, Xian 710049, Peoples R China

E-mail Address:
xichen@civil.columbia.edu

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Cited Reference Count:
27

Times Cited:
0

Publisher:
TAYLOR & FRANCIS LTD; 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND

Subject Category:
Chemistry, Physical; Physics, Atomic, Molecular & Chemical

ISSN:
0892-7022

DOI:
10.1080/08927020802175225

IDS Number:
375BR

========================================================================

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Title:
Removal of aromatic sulfonates from aqueous media by aminated polymeric sorbents: Concentration-dependent selectivity and the application

Authors:
Pan, BC; Zhang, QJ; Pan, BJ; Zhang, WM; Du, W; Ren, HQ

Author Full Names:
Pan, Bingcai; Zhang, Qingjian; Pan, Bingjun; Zhang, Weiming; Du, Wei; Ren, Hongqiang

Source:
MICROPOROUS AND MESOPOROUS MATERIALS 116 (1-3): 63-69 DEC 2008

Language:
English

Document Type:
Article

Author Keywords:
Aromatic sulfonates; Aminated polystyrene sorbent; Removal; Selectivity; Chemical wastewater

Keywords Plus:
ANION-EXCHANGE RESINS; WASTE-WATER TREATMENT; ION-EXCHANGE; INDUSTRIAL EFFLUENTS; MASS SPECTROMETRY; FLUORESCENCE; EQUILIBRIUM; ADSORPTION; PARTICLES; SORPTION

Abstract:
Sorption of aromatic sulfonates onto two aminated polystyrene sorbents with different pore structures (M-101 and D-301) was investigated for optimization of their potential application in chemical wastewater treatment. Sodium benzenesulfonate (BS), sodium 2-naphthalene sulfonate (2-NS) and disodium 2,6-naphthalene disulfonate (2,6-NDS) were selected as reference solutes and sodium sulfate was as a competitive inorganic salt. Sorption selectivity of both sorbents is dependent upon the concentration levels of aromatic sulfonates in solution coexisting with sodium sulfate at a high level. However, both sorbents exhibit different characters. D-301 presents more favorable sorption for the solutes at relatively high levels (e.g., higher than 5 mM for BS, 0.7 mM for 2-NS and 0.05 mM for 2,6-NS), while M-101 removes aromatic sulfonates more completely when the solute concentration kept at relatively low levels. Based on the experimental results, we proposed an integral process of so!
rption onto D-301 followed by secondary-sorption onto M-101 to remove aromatic sulfonates from industrial wastewater completely and economically. Furthermore, the satisfactory performance revealed from large-scale application further demonstrated the feasibility of extending this process to dispose of other associated chemical wastewaters. (C) 2008 Elsevier Inc. All rights reserved.

Reprint Address:
Pan, BC, Nanjing Univ, State Key Lab Pollut Control & Resources Reuse, Nanjing 210093, Peoples R China.

Research Institution addresses:
[Pan, Bingcai] Nanjing Univ, State Key Lab Pollut Control & Resources Reuse, Nanjing 210093, Peoples R China; Nanjing Univ, Sch Environm, Nanjing 210093, Peoples R China

E-mail Address:
bcpan@nju.edu.cn

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37

Times Cited:
0

Publisher:
ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS

Subject Category:
Chemistry, Applied; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary

ISSN:
1387-1811

DOI:
10.1016/j.micromeso.2008.03.016

IDS Number:
375SM

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Title:
Dependence of Single-Walled Carbon Nanotube Adsorption Kinetics on Temperature and Binding Energy

Authors:
Rawat, DS; Krungleviciute, V; Heroux, L; Bulut, A; Calbi, AA; Migone, AD

Author Full Names:
Rawat, D. S.; Krungleviciute, V.; Heroux, L.; Bulut, A.; Calbi, A. A.; Migone, A. D.

Source:
LANGMUIR 24 (23): 13465-13469 DEC 2 2008

Language:
English

Document Type:
Article

Keywords Plus:
GAS-ADSORPTION; DESORPTION-KINETICS; EXTERNAL SURFACES; SELF-DIFFUSION; MASS-TRANSPORT; BUNDLES; MEMBRANES; CF4; PHYSISORPTION; SIMULATIONS

Abstract:
We present results for the isothermal adsorption kinetics of methane, hydrogen, and tetrafluoromethane on closed-ended single-walled carbon nanotubes. In these experiments, we monitor the pressure decrease as a function of time as equilibrium is approached, after a dose of gas is added to the cell containing the nanotubes. The measurements were performed at different fractional coverages limited to the first layer. The results indicate that, for a given coverage and temperature, the equilibration time is an increasing function of E/(k(B)T), where E is the binding energy of the adsorbate and k(B)T is the thermal energy. These findings are consistent with recent theoretical predictions and Computer simulations results that we use to interpret the experimental measurements.

Reprint Address:
Migone, AD, So Illinois Univ, Dept Phys, Carbondale, IL 62901 USA.

Research Institution addresses:
[Rawat, D. S.; Krungleviciute, V.; Heroux, L.; Bulut, A.; Calbi, A. A.; Migone, A. D.] So Illinois Univ, Dept Phys, Carbondale, IL 62901 USA

E-mail Address:
aldo@physics.siu.edu

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Cited Reference Count:
72

Times Cited:
0

Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA

Subject Category:
Chemistry, Physical

ISSN:
0743-7463

DOI:
10.1021/la8022002

IDS Number:
376XO

========================================================================

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Title:
Carbon nanotube mediated microscale membrane extraction

Authors:
Hylton, K; Chen, YH; Mitra, S

Author Full Names:
Hylton, Kamilah; Chen, Yuhong; Mitra, Somenath

Source:
JOURNAL OF CHROMATOGRAPHY A 1211 (1-2): 43-48 NOV 21 2008

Language:
English

Document Type:
Article

Author Keywords:
Carbon nanotube; Membrane; Membrane extraction

Keywords Plus:
MIXED MATRIX MEMBRANES; LIQUID-PHASE MICROEXTRACTION; HOLLOW-FIBER MEMBRANES; GAS SEPARATION; SAMPLE PREPARATION; WATER; CHROMATOGRAPHY; TRANSPORT; FUNCTIONALIZATION; PESTICIDES

Abstract:
We demonstrate that functionalized carbon nanotubes can be readily immobilized into the pore structure of a polymeric membrane, which can dramatically improve its performance in analytical scale membrane extraction. This was accomplished by injecting an aqueous dispersion of the nanotubes through a Polypropylene hollow fiber under pressure. The nanotubes were trapped and held within the pores and served as sorbents facilitating solute exchange from the donor to the acceptor phase. The effectiveness of this carbon nanotube mediated process was studied by direct solvent enrichment of nonpolar organics, and also by selective extraction of organic acids via a supported liquid membrane. In both cases, the enrichment factor measured as the ratio of concentrations in the acceptor to the donor-phases could be increased by more than 200%. (C) 2008 Elsevier B.V. All rights reserved.

Reprint Address:
Mitra, S, Univ Heights, New Jersey Inst Technol, Dept Chem & Environm Sci, Newark, NJ 07104 USA.

Research Institution addresses:
[Chen, Yuhong; Mitra, Somenath] Univ Heights, New Jersey Inst Technol, Dept Chem & Environm Sci, Newark, NJ 07104 USA; [Hylton, Kamilah] Univ Technol, Jamaica, WI USA

E-mail Address:
Mitra@njit.edu

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Cited Reference Count:
47

Times Cited:
0

Publisher:
ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS

Subject Category:
Biochemical Research Methods; Chemistry, Analytical

ISSN:
0021-9673

DOI:
10.1016/j.chroma.2008.09.092

IDS Number:
377RM

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Title:
Influence of Water on the Frequency of Carbon Nanotube Oscillators

Authors:
Qin, Z; Zou, J; Feng, XQ

Author Full Names:
Qin, Zhao; Zou, Jian; Feng, Xi-Qiao

Source:
JOURNAL OF COMPUTATIONAL AND THEORETICAL NANOSCIENCE 5 (7): 1403-1407 JUL 2008

Language:
English

Document Type:
Article

Author Keywords:
Carbon Nanotube; Nano-Oscillator; Frequency; Molecular Dynamics Simulation

Keywords Plus:
MOLECULAR-DYNAMICS SIMULATIONS

Abstract:
Water molecules, which may either be introduced during fabrication of devices or absorbed from servicing environment, affect the performance and reliability of nanodevices and nanosystems. We investigate via theoretical analysis and molecular dynamics simulation the effect of water molecules on the vibration behavior of a double-walled carbon nanotube-based oscillator. It is found that water confined between the two nanotubes may significantly affect the oscillation frequency of the oscillator as a result of the enhancement of van der Waals interaction. An analytical expression is derived for the oscillation frequency in terms of the physical and geometrical parameters of carbon nanotubes and water. The theoretical results have a good agreement with molecular dynamics simulations.

Reprint Address:
Feng, XQ, Tsinghua Univ, Dept Engn Mech, Beijing 100084, Peoples R China.

Research Institution addresses:
[Qin, Zhao; Zou, Jian; Feng, Xi-Qiao] Tsinghua Univ, Dept Engn Mech, Beijing 100084, Peoples R China

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Cited Reference Count:
30

Times Cited:
1

Publisher:
AMER SCIENTIFIC PUBLISHERS; 25650 NORTH LEWIS WAY, STEVENSON RANCH, CA 91381-1439 USA

Subject Category:
Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter

ISSN:
1546-1955

DOI:
10.1166/jctn.2008.027

IDS Number:
376VF

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