Friday, October 29, 2010

ISI Web of Knowledge Alert Expiration Notice

ISI Web of Knowledge Citation Alert Expiration Notice

Cited Article: Saparov, S. Mobility of a one-dimensional confined file of water molecules as a function of file length
Alert Expires: 09 NOV 2010
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b

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ISI Web of Knowledge Alert - Song, X

ISI Web of Knowledge Citation Alert

Cited Article: Song, X. A comparative study on poiseuille flow of simple fluids through cylindrical and slit-like nanochannels
Alert Expires: 09 NOV 2010
Number of Citing Articles: 1 new records this week (1 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
An Investigation for the Usability of K-K Equations for Nano Porous Membranes

Authors:
Lu, JF; Chu, Y; Lu, WQ

Author Full Names:
Lu, Junfeng; Chu, Yang; Lu, Wen-Qiang

Source:
MNHMT2009, VOL 2 : 513-518 2010

Language:
English

Document Type:
Proceedings Paper

Author Keywords:
K-K equations; molecular dynamics (MD); computational fluid dynamics (CFD); ultra-filtration; nano-filtration

KeyWords Plus:
POISEUILLE FLOW; LIQUID; PERMEABILITY; SURFACES; FLUIDS; PORES

Abstract:
As physical model used to interpret the fluid behavior when it passes through a semi-permeable membrane, Kedem-Ketchalsky's (K-K) equations [1, 2] were successfully used in a bunch of filtration processes. However, because they were developed and dedicated to normal ultra- and micro-filtration systems, their limitations were obviously observed in some sort of nano-filtration processes that the pore size of the filtration membrane is only several nanometers. This paper analyzed the feasible utilization scopes of K-K equations. And two methods, Molecular Dynamics (MD) method and Computational Fluid Dynamics (CFD) method, used respectively to analyze nano- and ultra- filtration processes are introduced in this paper.

Reprint Address:
Lu, JF, Chinese Acad Sci, Tech Inst Phys & Chem, Beijing, Peoples R China.

Research Institution addresses:
[Lu, Junfeng] Chinese Acad Sci, Tech Inst Phys & Chem, Beijing, Peoples R China

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Cited Reference Count:
20

Times Cited:
0

Publisher:
AMER SOC MECHANICAL ENGINEERS; THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA

IDS Number:
BRH70

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ISI Web of Knowledge Alert - Ghosh, S

ISI Web of Knowledge Citation Alert

Cited Article: Ghosh, S. Carbon nanotube flow sensors
Alert Expires: 09 NOV 2010
Number of Citing Articles: 2 new records this week (2 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Mobility of a single alkali metal atom on fullerene C-60: First principles molecular dynamical study

Authors:
Ramaniah, LM; Boero, M

Author Full Names:
Ramaniah, Lavanya M.; Boero, Mauro

Source:
JOURNAL OF CHEMICAL PHYSICS 133 (13): Art. No. 134701 OCT 7 2010

Language:
English

Document Type:
Article

KeyWords Plus:
DENSITY-FUNCTIONAL THEORY; REAL-TIME OBSERVATION; COATED FULLERENES; ENDOHEDRAL FULLERENE; SURFACE-DIFFUSION; DOPED FULLERENES; CLUSTERS; MOTION; POTASSIUM; GRAPHITE

Abstract:
The dynamical behavior of a single K or Na alkali metal atom on the surface of a C-60 molecule is investigated via Car-Parrinello molecular dynamics simulations in a temperature range up to 300 K. These provide direct evidence for the heteroatom motion, postulated earlier in pioneering experiments, and show that an alkali metal atom can move both on the surface and radially outward from the surface, resulting in a dynamics ranging from diffusive to free orbital motion, on time-scales of up to a few picoseconds. (C) 2010 American Institute of Physics. [doi: 10.1063/1.3489421]

Reprint Address:
Ramaniah, LM, Bhabha Atom Res Ctr, High Pressure & Synchrotron Radiat Phys Div, Phys Grp, Bombay 400085, Maharashtra, India.

Research Institution addresses:
[Ramaniah, Lavanya M.] Bhabha Atom Res Ctr, High Pressure & Synchrotron Radiat Phys Div, Phys Grp, Bombay 400085, Maharashtra, India; [Boero, Mauro] CNRS, UMR 7504, Inst Phys & Chim Mat Strasbourg, F-67034 Strasbourg 2, France; [Boero, Mauro] Univ Strasbourg, F-67034 Strasbourg 2, France; [Boero, Mauro] JAIST, Res Ctr Integrated Sci, Nomi, Ishikawa 9231292, Japan; [Boero, Mauro] Japan Sci & Technol Agcy, CREST, Tokyo 1020075, Japan

E-mail Address:
lavanya@barc.gov.in

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Cited Reference Count:
67

Times Cited:
0

Publisher:
AMER INST PHYSICS; CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA

Subject Category:
Physics, Atomic, Molecular & Chemical

ISSN:
0021-9606

DOI:
10.1063/1.3489421

IDS Number:
661CE

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Title:
Defence Applications of Polymer Nanocomposites

Authors:
Kurahatti, RV; Surendranathan, AO; Kori, SA; Singh, N; Kumar, AVR; Srivastava, S

Author Full Names:
Kurahatti, R. V.; Surendranathan, A. O.; Kori, S. A.; Singh, Nirbhay; Kumar, A. V. Ramesh; Srivastava, Saurabh

Source:
DEFENCE SCIENCE JOURNAL 60 (5): 551-563 SEP 2010

Language:
English

Document Type:
Review

Author Keywords:
Nanocomposites; nanotechnologies; defence applications; smart materials; polymer-based nanocomposites; medical applications; fuel sources

KeyWords Plus:
POLYPROPYLENE-CLAY HYBRIDS; POLYMER/LAYERED SILICATE NANOCOMPOSITES; WALL CARBON NANOTUBES; MECHANICAL-PROPERTIES; ELECTRICAL-PROPERTIES; EPOXY NANOCOMPOSITES; SURFACE MODIFICATION; LAYERED SILICATES; COMPOSITES; NANOPARTICLES

Abstract:
The potential opportunities promised by nanotechnology for enabling advances in defence technologies are staggering. Although these opportunities are likely to be realised over a few decades, many advantages are currently being explored, particularly for defence applications. This review provides an insight into the capabilities offered by nanocomposites which include smart materials, harder/lighter platforms, new fuel sources and storage as well as novel medical applications. It discusses polymer-based nanocomposite materials, nanoscale fillers and provides examples of the actual and potential uses of nanocomposite materials in defence with practical examples.

Reprint Address:
Kurahatti, RV, Basaveshwar Engn Coll, Bagalkot 587102, Karnataka, India.

Research Institution addresses:
[Kurahatti, R. V.; Kori, S. A.] Basaveshwar Engn Coll, Bagalkot 587102, Karnataka, India; [Surendranathan, A. O.] Natl Inst Technol Karnataka, Surathkal 575025, Karnataka, India; [Singh, Nirbhay; Kumar, A. V. Ramesh; Srivastava, Saurabh] Def Mat & Stores Res & Dev Estab, Kanpur 208013, Uttar Pradesh, India

E-mail Address:
rajukurahatti@gmail.com

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Cited Reference Count:
107

Times Cited:
0

Publisher:
DEFENCE SCIENTIFIC INFORMATION DOCUMENTATION CENTRE; METCALFE HOUSE, DELHI 110054, INDIA

Subject Category:
Multidisciplinary Sciences

ISSN:
0011-748X

IDS Number:
663ZM

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ISI Web of Knowledge Alert Expiration Notice

ISI Web of Knowledge Citation Alert Expiration Notice

Cited Article: Maibaum, L. A coarse-grained model of water confined in a hydrophobic tube
Alert Expires: 09 NOV 2010
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b

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ISI Web of Knowledge Citation Alert Expiration Notice

Cited Article: Zhou, X. Equilibrium and kinetics: Water confined in carbon nanotubes as one-dimensional lattice gas
Alert Expires: 09 NOV 2010
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b

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Cited Article: Song, X. A comparative study on poiseuille flow of simple fluids through cylindrical and slit-like nanochannels
Alert Expires: 09 NOV 2010
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Cited Article: Ghosh, S. Carbon nanotube flow sensors
Alert Expires: 09 NOV 2010
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Cited Article: Zhao, Y. Individual water-filled single-walled carbon nanotubes as hydroelectric power converters
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ISI Web of Knowledge Alert - Hummer, G

ISI Web of Knowledge Citation Alert

Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
Alert Expires: 22 AUG 2011
Number of Citing Articles: 2 new records this week (2 in this e-mail)
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Title:
Molecular Origin of Fast Water Transport in Carbon Nanotube Membranes: Superlubricity versus Curvature Dependent Friction

Authors:
Falk, K; Sedlmeier, F; Joly, L; Netz, RR; Bocquet, L

Author Full Names:
Falk, Kerstin; Sedlmeier, Felix; Joly, Laurent; Netz, Roland R.; Bocquet, Lyderic

Source:
NANO LETTERS 10 (10): 4067-4073 OCT 2010

Language:
English

Document Type:
Article

Author Keywords:
Carbon nanotubes; graphene; confined water; water transport; permeability; membranes; nanofluidics

KeyWords Plus:
HYDRODYNAMIC BOUNDARY-CONDITIONS; FLUID-FLOW; SIMULATION; DYNAMICS; CHANNEL

Abstract:
In this paper, we study the interfacial friction of water at graphitic interfaces with various topologies, water between planar graphene sheets, inside and outside carbon nanotubes, with the goal to disentangle confinement and curvature effects on friction We show that the friction coefficient exhibits a strong curvature dependence, while friction is independent of confinement for the graphene slab, it decreases with carbon nanotube radius for water inside, but increases for water outside As a paradigm the friction coefficient is found to vanish below a threshold diameter for armchair nanotubes Using a statistical description of the interfacial friction, we highlight here a structural origin of this curvature dependence, mainly associated with a curvature-induced incommensurability between the water and carbon structures These results support the recent experiments reporting fast transport of water in nanometric carbon nanotube membranes

Reprint Address:
Bocquet, L, Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France.

Research Institution addresses:
[Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France; [Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] CNRS, UMR 5586, F-69622 Villeurbanne, France; [Sedlmeier, Felix; Netz, Roland R.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany

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Cited Reference Count:
27

Times Cited:
0

Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA

Subject Category:
Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary

ISSN:
1530-6984

DOI:
10.1021/nl1021046

IDS Number:
661KQ

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Title:
Quantum mechanics based force field for carbon (QMFF-Cx) validated to reproduce the mechanical and thermodynamics properties of graphite

Authors:
Pascal, TA; Karasawa, N; Goddard, WA

Author Full Names:
Pascal, Tod A.; Karasawa, Naoki; Goddard, William A., III

Source:
JOURNAL OF CHEMICAL PHYSICS 133 (13): Art. No. 134114 OCT 7 2010

Language:
English

Document Type:
Article

KeyWords Plus:
ANNEALED PYROLYTIC-GRAPHITE; SURFACE PHONON-DISPERSION; DENSITY-FUNCTIONAL THEORY; MOLECULAR-ORBITAL METHODS; GAUSSIAN-TYPE BASIS; MIDI BASIS-SET; AB-INITIO; ORGANIC-MOLECULES; THERMAL-EXPANSION; LATTICE-DYNAMICS

Abstract:
As assemblies of graphene sheets, carbon nanotubes, and fullerenes become components of new nanotechnologies, it is important to be able to predict the structures and properties of these systems. A problem has been that the level of quantum mechanics practical for such systems (density functional theory at the PBE level) cannot describe the London dispersion forces responsible for interaction of the graphene planes (thus graphite falls apart into graphene sheets). To provide a basis for describing these London interactions, we derive the quantum mechanics based force field for carbon (QMFF-Cx) by fitting to results from density functional theory calculations at the M06-2X level, which demonstrates accuracies for a broad class of molecules at short and medium range intermolecular distances. We carried out calculations on the dehydrogenated coronene (C24) dimer, emphasizing two geometries: parallel-displaced X (close to the observed structure in graphite crystal) and PD-Y (the
lowest energy transition state for sliding graphene sheets with respect to each other). A third, eclipsed geometry is calculated to be much higher in energy. The QMFF-Cx force field leads to accurate predictions of available experimental mechanical and thermodynamics data of graphite (lattice vibrations, elastic constants, Poisson ratios, lattice modes, phonon dispersion curves, specific heat, and thermal expansion). This validates the use of M06-2X as a practical method for development of new first principles based generations of QMFF force fields. (C) 2010 American Institute of Physics. [doi:10.1063/1.3456543]

Reprint Address:
Goddard, WA, CALTECH, Mat & Proc Simulat Ctr, Pasadena, CA 91125 USA.

Research Institution addresses:
[Pascal, Tod A.; Goddard, William A., III] CALTECH, Mat & Proc Simulat Ctr, Pasadena, CA 91125 USA; [Pascal, Tod A.; Goddard, William A., III] Korea Adv Inst Sci & Technol, Grad Sch EEWS, Taejon 305701, South Korea; [Karasawa, Naoki] Chitose Inst Sci & Technol, Dept Photon Sci, Sapporo, Hokkaido 0668655, Japan

E-mail Address:
wag@wag.caltech.edu

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Cited Reference Count:
98

Times Cited:
0

Publisher:
AMER INST PHYSICS; CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA

Subject Category:
Physics, Atomic, Molecular & Chemical

ISSN:
0021-9606

DOI:
10.1063/1.3456543

IDS Number:
661CE

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ISI Web of Knowledge Alert - Thompson, P

ISI Web of Knowledge Citation Alert

Cited Article: Thompson, P. A general boundary condition for liquid flow at solid surfaces
Alert Expires: 09 NOV 2010
Number of Citing Articles: 2 new records this week (2 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Scale Effects and Slip Microflow Characteristics of Evaporating Thin Films in a Microchannel

Authors:
Zhao, JJ; Peng, XF; Duan, YY

Author Full Names:
Zhao, J. J.; Peng, X. F.; Duan, Y. Y.

Source:
MNHMT2009, VOL 2 : 61-70 2010

Language:
English

Document Type:
Proceedings Paper

Author Keywords:
Evaporation Thin Film; Scale Effect; Near-wall Miroflow and Microlayer; Wall Slip; Wall Temperature Jump; Microchannel

KeyWords Plus:
HEAT-TRANSFER; FLUID-FLOW; MENISCUS; REGION

Abstract:
Micro flow, phase change and heat transfer characteristics of an evaporating thin film in a microchannel was investigated using an augmented Young-Laplace model and the kinetic theory for transverse flow in a solid-liquid-vapor triple contact line region. A model considering both wall slip and wall temperature jump was developed to explore scale effects of channel width. The results show that the average heat transfer coefficient and Reynolds number in thin film regions decrease with decreasing channel width, indicating worse flow and heat transfer characteristics. The scale effects are caused by increased far-field liquid film curvature and film thickness and consequently lower liquid superheat and lower evaporation pumping capability.
Original models describing wall-affected ordered adsorbed flowing liquid microlayer and variable slip coefficient were established to give the solid-liquid interfacial resistance and wall temperature jump. Microflow and microlayer near a wall increase wall thermal resistance and thus leads to worse film spreading and heat transfer characteristics, which are significant in thin film regions. The microflow model with variable slip coefficient is logical, more reasonable in results and better than the microflow model with constant slip coefficient.

Reprint Address:
Zhao, JJ, Tsinghua Univ, Lab Phase Change & Interfacial Transport Phenomen, Dept Thermal Engn, Beijing 100084, Peoples R China.

Research Institution addresses:
[Zhao, J. J.; Peng, X. F.; Duan, Y. Y.] Tsinghua Univ, Lab Phase Change & Interfacial Transport Phenomen, Dept Thermal Engn, Beijing 100084, Peoples R China

E-mail Address:
pxf-dte@mail.tsinghua.edu.cn

Cited References:
CAREY VP, 1992, LIQUID VAPOR PHASE C, P91.
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WEE SK, 2005, INT J HEAT MASS TRAN, V48, P265, DOI 10.1016/j.ijheatmasstransfer.2004.08.021.

Cited Reference Count:
12

Times Cited:
0

Publisher:
AMER SOC MECHANICAL ENGINEERS; THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA

IDS Number:
BRH70

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Title:
An Investigation for the Usability of K-K Equations for Nano Porous Membranes

Authors:
Lu, JF; Chu, Y; Lu, WQ

Author Full Names:
Lu, Junfeng; Chu, Yang; Lu, Wen-Qiang

Source:
MNHMT2009, VOL 2 : 513-518 2010

Language:
English

Document Type:
Proceedings Paper

Author Keywords:
K-K equations; molecular dynamics (MD); computational fluid dynamics (CFD); ultra-filtration; nano-filtration

KeyWords Plus:
POISEUILLE FLOW; LIQUID; PERMEABILITY; SURFACES; FLUIDS; PORES

Abstract:
As physical model used to interpret the fluid behavior when it passes through a semi-permeable membrane, Kedem-Ketchalsky's (K-K) equations [1, 2] were successfully used in a bunch of filtration processes. However, because they were developed and dedicated to normal ultra- and micro-filtration systems, their limitations were obviously observed in some sort of nano-filtration processes that the pore size of the filtration membrane is only several nanometers. This paper analyzed the feasible utilization scopes of K-K equations. And two methods, Molecular Dynamics (MD) method and Computational Fluid Dynamics (CFD) method, used respectively to analyze nano- and ultra- filtration processes are introduced in this paper.

Reprint Address:
Lu, JF, Chinese Acad Sci, Tech Inst Phys & Chem, Beijing, Peoples R China.

Research Institution addresses:
[Lu, Junfeng] Chinese Acad Sci, Tech Inst Phys & Chem, Beijing, Peoples R China

Cited References:
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Cited Reference Count:
20

Times Cited:
0

Publisher:
AMER SOC MECHANICAL ENGINEERS; THREE PARK AVENUE, NEW YORK, NY 10016-5990 USA

IDS Number:
BRH70

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Cited Article: Thompson, P. A general boundary condition for liquid flow at solid surfaces
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Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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*Order Full Text [ ]
AU Fang, DZ
Striemer, CC
Gaborski, TR
McGrath, JL
Fauchet, PM
AF Fang, David Z.
Striemer, Christopher C.
Gaborski, Thomas R.
McGrath, James L.
Fauchet, Philippe M.
TI Pore Size Control of Ultrathin Silicon Membranes by Rapid Thermal
Carbonization
SO NANO LETTERS
LA English
DT Article
DE Porous nanocrystalline silicon membrane; rapid thermal carbonization;
nanopores; surface functionalization
ID ACETYLENE ADSORPTION; SURFACE; NANOPORES; GROWTH
AB Rapid thermal carbonization in a dilute acetylene (C-2-H-2) atmosphere
has been used to chemically modify and precisely tune the pore size of
ultrachin porous nanocrystalline silicon (pnc-Si) The magnitude of size
reduction was controlled by varying the process temperature and time
Under certain conditions, the carbon coating displayed atomic ordering
indicative of graphene layer formation conformal to the pore walls
Initial experiments show that carbonized membranes follow theoretical
predictions for hydraulic permeability and retain the precise
separation capabilities of untreated membranes
C1 [Fang, David Z.; Striemer, Christopher C.; Fauchet, Philippe M.] Univ Rochester, Dept Elect & Comp Engn, Rochester, NY 14627 USA.
[Striemer, Christopher C.; Gaborski, Thomas R.] SiMPore Inc, W Henrietta, NY 14586 USA.
[McGrath, James L.] Univ Rochester, Dept Biomed Engn, Rochester, NY 14627 USA.
RP Fauchet, PM, Univ Rochester, Dept Elect & Comp Engn, Box 270231,
Rochester, NY 14627 USA.
CR AGRAWAL AA, 2010, BIOMATERIALS, V31, P5408, DOI
10.1016/j.biomaterials.2010.03.041
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GABORSKI TR, 2010, ACS NANO UNPUB
HOLT JK, 2006, SCIENCE, V312, P1034, DOI 10.1126/science.1126298
ISHIMATSU R, ANAL CHEM IN PRESS
KIM E, 2008, J AM CHEM SOC, V130, P4230, DOI 10.1021/ja711258w
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MIKKO R, 1999, NANOTECHNOLOGY, V10, P19
PULCI O, 2003, PHYS STATUS SOLIDI C, P2997
SALONEN J, 2000, STABILITY STUDIES TH
SALONEN J, 2002, J APPL PHYS, V91, P456
SALONEN J, 2004, APPL SURF SCI, V225, P389, DOI
10.1016/j.apsusc.2003.10.028
SAVARIAR EN, 2008, NAT NANOTECHNOL, V3, P112, DOI 10.1038/nnano.2008.6
SNYDER JL, J MEMBR SCI UNPUB
STORM AJ, 2003, NAT MATER, V2, P537, DOI 10.1038/nmat941
STRIEMER CC, 2007, NATURE, V445, P749, DOI 10.1038/nature05532
TONG HD, 2004, NANO LETT, V4, P283, DOI 10.1021/nl0350175
VONBEHREN J, 1995, APPL PHYS LETT, V66, P1662
WHITBY M, 2008, NANO LETT, V8, P2632, DOI 10.1021/nl080705f
YU M, 2009, NANO LETT, V9, P225, DOI 10.1021/nl802816h
NR 28
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
DI 10.1021/nl101602z
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SC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
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PT J
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AU Falk, K
Sedlmeier, F
Joly, L
Netz, RR
Bocquet, L
AF Falk, Kerstin
Sedlmeier, Felix
Joly, Laurent
Netz, Roland R.
Bocquet, Lyderic
TI Molecular Origin of Fast Water Transport in Carbon Nanotube Membranes:
Superlubricity versus Curvature Dependent Friction
SO NANO LETTERS
LA English
DT Article
DE Carbon nanotubes; graphene; confined water; water transport;
permeability; membranes; nanofluidics
ID HYDRODYNAMIC BOUNDARY-CONDITIONS; FLUID-FLOW; SIMULATION; DYNAMICS;
CHANNEL
AB In this paper, we study the interfacial friction of water at graphitic
interfaces with various topologies, water between planar graphene
sheets, inside and outside carbon nanotubes, with the goal to
disentangle confinement and curvature effects on friction We show that
the friction coefficient exhibits a strong curvature dependence, while
friction is independent of confinement for the graphene slab, it
decreases with carbon nanotube radius for water inside, but increases
for water outside As a paradigm the friction coefficient is found to
vanish below a threshold diameter for armchair nanotubes Using a
statistical description of the interfacial friction, we highlight here
a structural origin of this curvature dependence, mainly associated
with a curvature-induced incommensurability between the water and
carbon structures These results support the recent experiments
reporting fast transport of water in nanometric carbon nanotube
membranes
C1 [Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France.
[Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] CNRS, UMR 5586, F-69622 Villeurbanne, France.
[Sedlmeier, Felix; Netz, Roland R.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany.
RP Bocquet, L, Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France.
CR ALEXIADIS A, 2008, CHEM REV, V108, P5014, DOI 10.1021/cr078140f
BARRAT JL, 1999, FARADAY DISCUSS, V112, P119
BEREZHKOVSKII A, 2002, PHYS REV LETT, V89
BOCQUET L, 1994, PHYS REV E A, V49, P3079
BOCQUET L, 2007, SOFT MATTER, V3, P685, DOI 10.1039/b616490k
BOCQUET L, 2010, CHEM SOC REV, V39, P1073, DOI 10.1039/b909366b
CORNELL WD, 1995, J AM CHEM SOC, V117, P5179
DIENWIEBEL M, 2004, PHYS REV LETT, V92, ARTN 126101
ESPANOL P, 1993, J CHEM PHYS, V98, P574
GONG XJ, 2008, PHYS REV LETT, V101, ARTN 257801
HANASAKI I, 2006, J CHEM PHYS, V124, ARTN 144708
HANSEN JP, 1969, PHYS REV, V184, P151
HOLT JK, 2006, SCIENCE, V312, P1034, DOI 10.1126/science.1126298
HUANG DM, 2008, PHYS REV LETT, V101, ARTN 226101
HUMMER G, 2001, NATURE, V414, P188
JOSEPH S, 2008, NANO LETT, V8, P452, DOI 10.1021/nl072385q
KOLESNIKOV AI, 2004, PHYS REV LETT, V93
MAJUMDER M, 2005, NATURE, V438, P44, DOI 10.1038/43844a
PLIMPTON S, 1995, J COMPUT PHYS, V117, P1
SOKHAN VP, 2002, J CHEM PHYS, V117, P8531, DOI 10.1063/1.1512643
SPARREBOOM W, 2009, NAT NANOTECHNOL, V4, P713, DOI
10.1038/NNANO.2009.332
SUI HX, 2001, NATURE, V414, P872
THOMAS JA, 2008, NANO LETT, V8, P2788, DOI 10.1021/nl8013617
THOMAS JA, 2009, PHYS REV LETT, V102, ARTN 184502
VANDERSPOEL D, 2005, J COMPUT CHEM, V26, P1701, DOI 10.1002/jcc.20291
WERDER T, 2003, J PHYS CHEM B, V107, P1345, DOI 10.1021/jp0268112
WHITBY M, 2008, NANO LETT, V8, P2632, DOI 10.1021/nl080705f
NR 27
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
DI 10.1021/nl1021046
PD OCT
VL 10
IS 10
BP 4067
EP 4073
SC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary
GA 661KQ
UT ISI:000282727600045
ER

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ISI Web of Knowledge Alert - Sokhan VP

ISI Web of Knowledge Citation Alert

Cited Article: Sokhan VP. Fluid flow in nanopores: Accurate boundary conditions for carbon nanotubes
Alert Expires: 09 NOV 2010
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Title:
Molecular Origin of Fast Water Transport in Carbon Nanotube Membranes: Superlubricity versus Curvature Dependent Friction

Authors:
Falk, K; Sedlmeier, F; Joly, L; Netz, RR; Bocquet, L

Author Full Names:
Falk, Kerstin; Sedlmeier, Felix; Joly, Laurent; Netz, Roland R.; Bocquet, Lyderic

Source:
NANO LETTERS 10 (10): 4067-4073 OCT 2010

Language:
English

Document Type:
Article

Author Keywords:
Carbon nanotubes; graphene; confined water; water transport; permeability; membranes; nanofluidics

KeyWords Plus:
HYDRODYNAMIC BOUNDARY-CONDITIONS; FLUID-FLOW; SIMULATION; DYNAMICS; CHANNEL

Abstract:
In this paper, we study the interfacial friction of water at graphitic interfaces with various topologies, water between planar graphene sheets, inside and outside carbon nanotubes, with the goal to disentangle confinement and curvature effects on friction We show that the friction coefficient exhibits a strong curvature dependence, while friction is independent of confinement for the graphene slab, it decreases with carbon nanotube radius for water inside, but increases for water outside As a paradigm the friction coefficient is found to vanish below a threshold diameter for armchair nanotubes Using a statistical description of the interfacial friction, we highlight here a structural origin of this curvature dependence, mainly associated with a curvature-induced incommensurability between the water and carbon structures These results support the recent experiments reporting fast transport of water in nanometric carbon nanotube membranes

Reprint Address:
Bocquet, L, Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France.

Research Institution addresses:
[Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France; [Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] CNRS, UMR 5586, F-69622 Villeurbanne, France; [Sedlmeier, Felix; Netz, Roland R.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany

Cited References:
ALEXIADIS A, 2008, CHEM REV, V108, P5014, DOI 10.1021/cr078140f.
BARRAT JL, 1999, FARADAY DISCUSS, V112, P119.
BEREZHKOVSKII A, 2002, PHYS REV LETT, V89.
BOCQUET L, 1994, PHYS REV E A, V49, P3079.
BOCQUET L, 2007, SOFT MATTER, V3, P685, DOI 10.1039/b616490k.
BOCQUET L, 2010, CHEM SOC REV, V39, P1073, DOI 10.1039/b909366b.
CORNELL WD, 1995, J AM CHEM SOC, V117, P5179.
DIENWIEBEL M, 2004, PHYS REV LETT, V92, ARTN 126101.
ESPANOL P, 1993, J CHEM PHYS, V98, P574.
GONG XJ, 2008, PHYS REV LETT, V101, ARTN 257801.
HANASAKI I, 2006, J CHEM PHYS, V124, ARTN 144708.
HANSEN JP, 1969, PHYS REV, V184, P151.
HOLT JK, 2006, SCIENCE, V312, P1034, DOI 10.1126/science.1126298.
HUANG DM, 2008, PHYS REV LETT, V101, ARTN 226101.
HUMMER G, 2001, NATURE, V414, P188.
JOSEPH S, 2008, NANO LETT, V8, P452, DOI 10.1021/nl072385q.
KOLESNIKOV AI, 2004, PHYS REV LETT, V93.
MAJUMDER M, 2005, NATURE, V438, P44, DOI 10.1038/43844a.
PLIMPTON S, 1995, J COMPUT PHYS, V117, P1.
SOKHAN VP, 2002, J CHEM PHYS, V117, P8531, DOI 10.1063/1.1512643.
SPARREBOOM W, 2009, NAT NANOTECHNOL, V4, P713, DOI 10.1038/NNANO.2009.332.
SUI HX, 2001, NATURE, V414, P872.
THOMAS JA, 2008, NANO LETT, V8, P2788, DOI 10.1021/nl8013617.
THOMAS JA, 2009, PHYS REV LETT, V102, ARTN 184502.
VANDERSPOEL D, 2005, J COMPUT CHEM, V26, P1701, DOI 10.1002/jcc.20291.
WERDER T, 2003, J PHYS CHEM B, V107, P1345, DOI 10.1021/jp0268112.
WHITBY M, 2008, NANO LETT, V8, P2632, DOI 10.1021/nl080705f.

Cited Reference Count:
27

Times Cited:
0

Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA

Subject Category:
Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary

ISSN:
1530-6984

DOI:
10.1021/nl1021046

IDS Number:
661KQ

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ISI Web of Knowledge Alert - Majumder M

ISI Web of Knowledge Citation Alert

Cited Article: Majumder M. Nanoscale hydrodynamics - Enhanced flow in carbon nanotubes
Alert Expires: 09 NOV 2010
Number of Citing Articles: 1 new records this week (1 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Molecular Origin of Fast Water Transport in Carbon Nanotube Membranes: Superlubricity versus Curvature Dependent Friction

Authors:
Falk, K; Sedlmeier, F; Joly, L; Netz, RR; Bocquet, L

Author Full Names:
Falk, Kerstin; Sedlmeier, Felix; Joly, Laurent; Netz, Roland R.; Bocquet, Lyderic

Source:
NANO LETTERS 10 (10): 4067-4073 OCT 2010

Language:
English

Document Type:
Article

Author Keywords:
Carbon nanotubes; graphene; confined water; water transport; permeability; membranes; nanofluidics

KeyWords Plus:
HYDRODYNAMIC BOUNDARY-CONDITIONS; FLUID-FLOW; SIMULATION; DYNAMICS; CHANNEL

Abstract:
In this paper, we study the interfacial friction of water at graphitic interfaces with various topologies, water between planar graphene sheets, inside and outside carbon nanotubes, with the goal to disentangle confinement and curvature effects on friction We show that the friction coefficient exhibits a strong curvature dependence, while friction is independent of confinement for the graphene slab, it decreases with carbon nanotube radius for water inside, but increases for water outside As a paradigm the friction coefficient is found to vanish below a threshold diameter for armchair nanotubes Using a statistical description of the interfacial friction, we highlight here a structural origin of this curvature dependence, mainly associated with a curvature-induced incommensurability between the water and carbon structures These results support the recent experiments reporting fast transport of water in nanometric carbon nanotube membranes

Reprint Address:
Bocquet, L, Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France.

Research Institution addresses:
[Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France; [Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] CNRS, UMR 5586, F-69622 Villeurbanne, France; [Sedlmeier, Felix; Netz, Roland R.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany

Cited References:
ALEXIADIS A, 2008, CHEM REV, V108, P5014, DOI 10.1021/cr078140f.
BARRAT JL, 1999, FARADAY DISCUSS, V112, P119.
BEREZHKOVSKII A, 2002, PHYS REV LETT, V89.
BOCQUET L, 1994, PHYS REV E A, V49, P3079.
BOCQUET L, 2007, SOFT MATTER, V3, P685, DOI 10.1039/b616490k.
BOCQUET L, 2010, CHEM SOC REV, V39, P1073, DOI 10.1039/b909366b.
CORNELL WD, 1995, J AM CHEM SOC, V117, P5179.
DIENWIEBEL M, 2004, PHYS REV LETT, V92, ARTN 126101.
ESPANOL P, 1993, J CHEM PHYS, V98, P574.
GONG XJ, 2008, PHYS REV LETT, V101, ARTN 257801.
HANASAKI I, 2006, J CHEM PHYS, V124, ARTN 144708.
HANSEN JP, 1969, PHYS REV, V184, P151.
HOLT JK, 2006, SCIENCE, V312, P1034, DOI 10.1126/science.1126298.
HUANG DM, 2008, PHYS REV LETT, V101, ARTN 226101.
HUMMER G, 2001, NATURE, V414, P188.
JOSEPH S, 2008, NANO LETT, V8, P452, DOI 10.1021/nl072385q.
KOLESNIKOV AI, 2004, PHYS REV LETT, V93.
MAJUMDER M, 2005, NATURE, V438, P44, DOI 10.1038/43844a.
PLIMPTON S, 1995, J COMPUT PHYS, V117, P1.
SOKHAN VP, 2002, J CHEM PHYS, V117, P8531, DOI 10.1063/1.1512643.
SPARREBOOM W, 2009, NAT NANOTECHNOL, V4, P713, DOI 10.1038/NNANO.2009.332.
SUI HX, 2001, NATURE, V414, P872.
THOMAS JA, 2008, NANO LETT, V8, P2788, DOI 10.1021/nl8013617.
THOMAS JA, 2009, PHYS REV LETT, V102, ARTN 184502.
VANDERSPOEL D, 2005, J COMPUT CHEM, V26, P1701, DOI 10.1002/jcc.20291.
WERDER T, 2003, J PHYS CHEM B, V107, P1345, DOI 10.1021/jp0268112.
WHITBY M, 2008, NANO LETT, V8, P2632, DOI 10.1021/nl080705f.

Cited Reference Count:
27

Times Cited:
0

Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA

Subject Category:
Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary

ISSN:
1530-6984

DOI:
10.1021/nl1021046

IDS Number:
661KQ

========================================================================
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All Customers
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ISI Web of Knowledge Alert Expiration Notice

ISI Web of Knowledge Citation Alert Expiration Notice

Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
Alert Expires: 09 NOV 2010
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b

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ISI Web of Knowledge Alert - Hanasaki I

ISI Web of Knowledge Citation Alert

Cited Article: Hanasaki I. Flow structure of water in carbon nanotubes: Poiseuille type or plug-like?
Alert Expires: 09 NOV 2010
Number of Citing Articles: 1 new records this week (1 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Molecular Origin of Fast Water Transport in Carbon Nanotube Membranes: Superlubricity versus Curvature Dependent Friction

Authors:
Falk, K; Sedlmeier, F; Joly, L; Netz, RR; Bocquet, L

Author Full Names:
Falk, Kerstin; Sedlmeier, Felix; Joly, Laurent; Netz, Roland R.; Bocquet, Lyderic

Source:
NANO LETTERS 10 (10): 4067-4073 OCT 2010

Language:
English

Document Type:
Article

Author Keywords:
Carbon nanotubes; graphene; confined water; water transport; permeability; membranes; nanofluidics

KeyWords Plus:
HYDRODYNAMIC BOUNDARY-CONDITIONS; FLUID-FLOW; SIMULATION; DYNAMICS; CHANNEL

Abstract:
In this paper, we study the interfacial friction of water at graphitic interfaces with various topologies, water between planar graphene sheets, inside and outside carbon nanotubes, with the goal to disentangle confinement and curvature effects on friction We show that the friction coefficient exhibits a strong curvature dependence, while friction is independent of confinement for the graphene slab, it decreases with carbon nanotube radius for water inside, but increases for water outside As a paradigm the friction coefficient is found to vanish below a threshold diameter for armchair nanotubes Using a statistical description of the interfacial friction, we highlight here a structural origin of this curvature dependence, mainly associated with a curvature-induced incommensurability between the water and carbon structures These results support the recent experiments reporting fast transport of water in nanometric carbon nanotube membranes

Reprint Address:
Bocquet, L, Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France.

Research Institution addresses:
[Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] Univ Lyon 1, LPMCN, F-69622 Villeurbanne, France; [Falk, Kerstin; Joly, Laurent; Bocquet, Lyderic] CNRS, UMR 5586, F-69622 Villeurbanne, France; [Sedlmeier, Felix; Netz, Roland R.] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany

Cited References:
ALEXIADIS A, 2008, CHEM REV, V108, P5014, DOI 10.1021/cr078140f.
BARRAT JL, 1999, FARADAY DISCUSS, V112, P119.
BEREZHKOVSKII A, 2002, PHYS REV LETT, V89.
BOCQUET L, 1994, PHYS REV E A, V49, P3079.
BOCQUET L, 2007, SOFT MATTER, V3, P685, DOI 10.1039/b616490k.
BOCQUET L, 2010, CHEM SOC REV, V39, P1073, DOI 10.1039/b909366b.
CORNELL WD, 1995, J AM CHEM SOC, V117, P5179.
DIENWIEBEL M, 2004, PHYS REV LETT, V92, ARTN 126101.
ESPANOL P, 1993, J CHEM PHYS, V98, P574.
GONG XJ, 2008, PHYS REV LETT, V101, ARTN 257801.
HANASAKI I, 2006, J CHEM PHYS, V124, ARTN 144708.
HANSEN JP, 1969, PHYS REV, V184, P151.
HOLT JK, 2006, SCIENCE, V312, P1034, DOI 10.1126/science.1126298.
HUANG DM, 2008, PHYS REV LETT, V101, ARTN 226101.
HUMMER G, 2001, NATURE, V414, P188.
JOSEPH S, 2008, NANO LETT, V8, P452, DOI 10.1021/nl072385q.
KOLESNIKOV AI, 2004, PHYS REV LETT, V93.
MAJUMDER M, 2005, NATURE, V438, P44, DOI 10.1038/43844a.
PLIMPTON S, 1995, J COMPUT PHYS, V117, P1.
SOKHAN VP, 2002, J CHEM PHYS, V117, P8531, DOI 10.1063/1.1512643.
SPARREBOOM W, 2009, NAT NANOTECHNOL, V4, P713, DOI 10.1038/NNANO.2009.332.
SUI HX, 2001, NATURE, V414, P872.
THOMAS JA, 2008, NANO LETT, V8, P2788, DOI 10.1021/nl8013617.
THOMAS JA, 2009, PHYS REV LETT, V102, ARTN 184502.
VANDERSPOEL D, 2005, J COMPUT CHEM, V26, P1701, DOI 10.1002/jcc.20291.
WERDER T, 2003, J PHYS CHEM B, V107, P1345, DOI 10.1021/jp0268112.
WHITBY M, 2008, NANO LETT, V8, P2632, DOI 10.1021/nl080705f.

Cited Reference Count:
27

Times Cited:
0

Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA

Subject Category:
Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary

ISSN:
1530-6984

DOI:
10.1021/nl1021046

IDS Number:
661KQ

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ISI Web of Knowledge Alert Expiration Notice

ISI Web of Knowledge Citation Alert Expiration Notice

Cited Article: Sokhan VP. Fluid flow in nanopores: Accurate boundary conditions for carbon nanotubes
Alert Expires: 09 NOV 2010
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b

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ISI Web of Knowledge Alert Expiration Notice

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Cited Article: Hanasaki I. Flow structure of water in carbon nanotubes: Poiseuille type or plug-like?
Alert Expires: 09 NOV 2010
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b

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ISI Web of Knowledge Alert Expiration Notice

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Cited Article: Majumder M. Nanoscale hydrodynamics - Enhanced flow in carbon nanotubes
Alert Expires: 09 NOV 2010
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b

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ISI Web of Knowledge Alert Expiration Notice

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Cited Article: Lichter S. Mechanisms for liquid slip at solid surfaces
Alert Expires: 09 NOV 2010
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b

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Friday, October 22, 2010

ISI Web of Knowledge Alert - Ghosh, S

ISI Web of Knowledge Citation Alert

Cited Article: Ghosh, S. Carbon nanotube flow sensors
Alert Expires: 09 NOV 2010
Number of Citing Articles: 1 new records this week (1 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Elastic Response of Carbon Nanotube Forests to Aerodynamic Stresses

Authors:
Battiato, I; Bandaru, PR; Tartakovsky, DM

Author Full Names:
Battiato, Ilenia; Bandaru, Prabhakar R.; Tartakovsky, Daniel M.

Source:
PHYSICAL REVIEW LETTERS 105 (14): Art. No. 144504 OCT 1 2010

Language:
English

Document Type:
Article

KeyWords Plus:
FLOW

Abstract:
The ability to determine static and (hydro) dynamic properties of carbon nanotubes (CNTs) is crucial for many applications. While their static properties (e.g., solubility and wettability) are fairly well understood, their mechanical responses (e.g., deflection under shear) to ambient fluid flow are to a large extent unknown. We analyze the elastic response of single-walled CNT forests, attached to the bottom wall of a channel, to the aerodynamic loading exerted by both laminar and turbulent flows. Our analysis yields analytical expressions for velocity distributions, the drag coefficient, and bending profiles of individual CNTs. This enables us to determine flexural rigidity of CNTs in wind-tunnel experiments. The model predictions agree with laboratory experiments for a large range of channel velocities.

Reprint Address:
Battiato, I, Univ Calif San Diego, La Jolla, CA 92093 USA.

Research Institution addresses:
[Battiato, Ilenia; Bandaru, Prabhakar R.; Tartakovsky, Daniel M.] Univ Calif San Diego, La Jolla, CA 92093 USA

E-mail Address:
dmt@ucsd.edu

Cited References:
BAUGHMAN RH, 2002, SCIENCE, V297, P787.
BEER FP, 2006, MECH MAT.
DECK CP, 2009, J APPL PHYS, V106, P74304, ARTN 074304.
FALVO MR, 1997, NATURE, V389, P582.
FORD AN, 2006, IND ENG CHEM RES, V45, P1797, DOI 10.1021/ie050932h.
GHOSH S, 2003, SCIENCE, V299, P1042, DOI 10.1126/science.1079080.
HAPPEL J, 1959, AICHE J, V5, P174.
HUANG JY, 2006, NATURE, V439, P281, DOI 10.1038/439281a.
JOSEPH P, 2006, PHYS REV LETT, V97, ARTN 156104.
KIM P, 1999, SCIENCE, V286, P2148.
PONCHARAL P, 1999, SCIENCE, V283, P1513.
POPE SB, 2000, TURBULENT FLOWS.
TREACY MMJ, 1996, NATURE, V381, P678.
VALDESPARADA FJ, 2007, PHYSICA A, V385, P69, DOI 10.1016/j.physa.2007.06.012.
WALTHER JH, 2004, PHYS REV E 1, V69, ARTN 062201.
WEINBAUM S, 2003, P NATL ACAD SCI USA, V100, P7988, DOI 10.1073/pnas.1332808100.
WILSON M, 2009, PHYS TODAY, V62, P16.

Cited Reference Count:
17

Times Cited:
0

Publisher:
AMER PHYSICAL SOC; ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA

Subject Category:
Physics, Multidisciplinary

ISSN:
0031-9007

DOI:
10.1103/PhysRevLett.105.144504

IDS Number:
656UF

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ISI Web of Knowledge Alert - Hummer, G

ISI Web of Knowledge Citation Alert

Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
Alert Expires: 22 AUG 2011
Number of Citing Articles: 1 new records this week (1 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Nanofiltration of Electrolyte Solutions by Sub-2nm Carbon Nanotube Membranes

Authors:
Fornasiero, F; Park, HG; Holt, JK; Stadermann, M; Kim, S; Bin In, J; Grigoropoulos, CP; Noy, A; Bakajin, O

Author Full Names:
Fornasiero, Francesco; Park, Hyung Gyu; Holt, Jason K.; Stadermann, Michael; Kim, Sangil; Bin In, Jung; Grigoropoulos, Costas P.; Noy, Aleksandr; Bakajin, Olgica

Source:
CLEAN TECHNOLOGY 2008: BIO ENERGY, RENEWABLES, GREEN BUILDING, SMART GRID, STORAGE, AND WATER : 380-383 2008

Language:
English

Document Type:
Proceedings Paper

Author Keywords:
carbon nanotube; membrane; ion exclusion; fast flow

KeyWords Plus:
WATER; TRANSPORT; GROWTH

Abstract:
Both MD simulations and experimental studies have shown that liquid and gas flow through carbon nanotubes with nanometer size diameter is exceptionally fast. For applications in separation technology, selectivity is required together with fast flow. In this work, we use pressure-driven filtration experiments to study ion exclusion in silicon nitride/sub-2-nm CNT composite membranes as a function of solution ionic strength, pH, and ion valence. We show that carbon nanotube membranes exhibit significant ion exclusion at low salt concentration. Our results support a rejection mechanism dominated by electrostatic interactions between fixed membrane charges and mobile ions, while steric and hydrodynamic effects appear to be less important. Comparison with commercial nanofiltration membranes for water softening reveals that our carbon nanotube membranes provides far superior water fluxes for similar ion rejection capabilities.

Reprint Address:
Fornasiero, F, LLNL, Biosci & Biotechnol Div, CMELS, Livermore, CA 94550 USA.

Research Institution addresses:
[Fornasiero, Francesco; Park, Hyung Gyu; Holt, Jason K.; Stadermann, Michael; Noy, Aleksandr; Bakajin, Olgica] LLNL, Biosci & Biotechnol Div, CMELS, Livermore, CA 94550 USA

Cited References:
CHEUNG CL, 2002, J PHYS CHEM B, V106, P2429.
FORNASIERO F, 2008, PNAS IN PRESS.
FRANKLIN NR, 2002, APPL PHYS LETT, V81, P913.
FUTABA DN, 2006, NAT MATER, V5, P987, DOI 10.1038/nmat1782.
HOLT JK, 2006, SCIENCE, V312, P1034, DOI 10.1126/science.1126298.
HUMMER G, 2001, NATURE, V414, P188.
JOSEPH S, 2008, NANO LETT, V8, P452, DOI 10.1021/nl072385q.
KALRA A, 2003, P NATL ACAD SCI USA, V100, P10175.
KOLESNIKOV AI, 2004, PHYS REV LETT, V93, ARTN 035503.
LOISEAU A, 2006, LECT NOTE PHYS, V677, P49.
MAJUMDER M, 2005, NATURE, V438, P44, DOI 10.1038/43844a.
MAMONTOV E, 2006, J CHEM PHYS, V124, ARTN 194703.
MANIWA Y, 2007, NAT MATER, V6, P135, DOI 10.1038/nmat1823.
NAGUIB N, 2004, NANO LETT, V4, P2237, DOI 10.1021/nl0484907.
NOY A, 2007, NANO TODAY, V2, P22.
PURETZKY AA, 2005, APPL PHYS A-MATER, V81, P223, DOI 10.1007/s00339-005-3256-7.
YAMADA T, 2006, NAT NANOTECHNOL, V1, P131, DOI 10.1038/nnano.2006.95.

Cited Reference Count:
17

Times Cited:
0

Publisher:
CRC PRESS-TAYLOR & FRANCIS GROUP; 6000 BROKEN SOUND PARKWAY NW, STE 300, BOCA RATON, FL 33487-2742 USA

IDS Number:
BRC37

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