ISI Web of Knowledge Alert - Holt JK

ISI Web of Knowledge Citation Alert

Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
Alert Expires: 18 OCT 2009
Number of Citing Articles: 2 new records this week (2 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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AU Peng, XS
Jin, J
Nakamura, Y
Ohno, T
Ichinose, I
AF Peng, Xinsheng
Jin, Jian
Nakamura, Yoshimichi
Ohno, Takahisa
Ichinose, Izumi
TI Ultrafast permeation of water through protein-based membranes
SO NATURE NANOTECHNOLOGY
LA English
DT Article
ID COPPER HYDROXIDE NANOSTRANDS; CARBON NANOTUBE MEMBRANES; FAST
MASS-TRANSPORT; ULTRAFILTRATION MEMBRANES; NANOFILTRATION MEMBRANES;
SEPARATION; MODEL
AB Pressure-driven filtration by porous membranes is widely used in the
production of drinking water from ground and surface water(1-3).
Permeation theory predicts that filtration rate is proportional to the
pressure difference across the filtration membrane and inversely
proportional to the thickness of the membrane(4). However, these
membranes need to be able to withstand high water fluxes and pressures,
which means that the active separation layers in commercial filtration
systems typically have a thickness of a few tens to several hundreds of
nanometres(5). Filtration performance might be improved by the use of
ultrathin porous silicon membranes(6) or carbon nanotubes immobilized
in silicon nitride(7) or polymer films(8,9), but these structures are
difficult to fabricate. Here, we report a new type of filtration
membrane made of crosslinked proteins that are mechanically robust and
contain channels with diameters of less than 2.2 nm. We find that a
60-nm-thick membrane can concentrate aqueous dyes from fluxes up to
9,000 l h(-1) m(-2) bar(-1), which is similar to 1,000 times higher
than the fluxes that can be withstood by commercial filtration
membranes with similar rejection properties(1,10,11). Based on these
results and molecular dynamics simulations, we propose that
protein-surrounded channels with effective lengths of less than 5.8 nm
can separate dye molecules while allowing the ultrafast permeation of
water at applied pressures of less than 1 bar.
C1 [Peng, Xinsheng; Jin, Jian; Ichinose, Izumi] Natl Inst Mat Sci, Organ Nanomat Ctr, Tsukuba, Ibaraki 3050044, Japan.
[Nakamura, Yoshimichi; Ohno, Takahisa] Natl Inst Mat Sci, Computat Mat Sci Ctr, Tsukuba, Ibaraki 3050047, Japan.
[Ohno, Takahisa; Ichinose, Izumi] JST, CREST, Chiyoda Ku, Tokyo 1020075, Japan.
RP Ichinose, I, Natl Inst Mat Sci, Organ Nanomat Ctr, 1-1 Namiki, Tsukuba,
Ibaraki 3050044, Japan.
EM ICHINOSE.lzumi@nims.go.jp
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NR 28
TC 1
PU NATURE PUBLISHING GROUP; MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1
9XW, ENGLAND
SN 1748-3387
DI 10.1038/NNANO.2009.90
PD JUN
VL 4
IS 6
BP 353
EP 357
SC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
GA 459TA
UT ISI:000267131500011
ER

PT J
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AU Ji, QM
Acharya, S
Hill, JP
Vinu, A
Yoon, SB
Yu, JS
Sakamoto, K
Ariga, K
AF Ji, Qingmin
Acharya, Somobrata
Hill, Jonathan P.
Vinu, Ajayan
Yoon, Suk Bon
Yu, Jong-Sung
Sakamoto, Kazutami
Ariga, Katsuhiko
TI Hierarchic Nanostructure for Auto-Modulation of Material Release:
Mesoporous Nanocompartment Films
SO ADVANCED FUNCTIONAL MATERIALS
LA English
DT Article
ID CONTROLLED DRUG-RELEASE; POLYELECTROLYTE MULTILAYER FILMS; RESPONSIVE
CONTROLLED-RELEASE; POROUS-GLASS PLATE; SUPRAMOLECULAR NANOVALVE;
CORE/MESOPOROUS SHELL; SILICA NANOPARTICLES; PERMEATION CONTROL;
TRIGGERED RELEASE; GUEST MOLECULES
AB The preparation of mesoporous nanocompartment films composed of both
hollow silica capsules and silica particles by using layer-by-layer
(LbL) adsorption is described. The resultant nanocompartment films
exhibit stepwise release, of encapsulated water molecules without
application of external stimuli. The hollow hierarchic pore structure
of the silica capsules, including their internal void and mesoporous
walls, is a key factor for the regulation and stepwise release of
water, and is probably caused by the non- equilibrated concurrent
evaporation of material from the mesopore and capillary penetration
into the mesopores. The number of release steps and rate of release can
be tuned by variation of several parameters including water content,
ambient temperature, layer multiplicity, and co-adduct particle size.
Application of the mesoporous nanocompartment films for the release of
substances, including therapeutic agents and fragrances, indicates that
the stepwise material release can be applied for a wide range of liquid
substances. The films should lead to a novel-material release system
useful even for biomedical applications capable of controlled and
sustained delivery of drug molecules.
C1 [Ji, Qingmin; Acharya, Somobrata; Hill, Jonathan P.; Vinu, Ajayan; Ariga, Katsuhiko] Natl Inst Mat Sci, World Premier Int Res Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki 3050044, Japan.
[Yoon, Suk Bon; Yu, Jong-Sung] Korea Univ, Dept Adv Mat Chem, Jochiwon 339700, Chungnam, South Korea.
[Sakamoto, Kazutami] Tokyo Univ Sci, Chiba 2788510, Japan.
RP Ji, QM, Natl Inst Mat Sci, World Premier Int Res Ctr Mat
Nanoarchitecton, 1-1 Namiki, Tsukuba, Ibaraki 3050044, Japan.
EM jsyu212@korea.ac.kr
ARIGA.Katsuhiko@nims.go.jp
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NR 89
TC 0
PU WILEY-V C H VERLAG GMBH; PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
SN 1616-301X
DI 10.1002/adfm.200801762
PD JUN 9
VL 19
IS 11
BP 1792
EP 1799
SC Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience &
Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied;
Physics, Condensed Matter
GA 461XA
UT ISI:000267305500015
ER

EF

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ISI Web of Knowledge Alert - Sokhan VP

ISI Web of Knowledge Citation Alert

Cited Article: Sokhan VP. Fluid flow in nanopores: Accurate boundary conditions for carbon nanotubes
Alert Expires: 18 OCT 2009
Number of Citing Articles: 1 new records this week (1 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Observation of fluid layering and reverse motion in double-walled carbon nanotubes

Authors:
Yaghmaei, K; Rafii-Tabar, H

Author Full Names:
Yaghmaei, K.; Rafii-Tabar, H.

Source:
CURRENT APPLIED PHYSICS 9 (6): 1411-1422 NOV 2009

Language:
English

Document Type:
Article

Author Keywords:
Argon fluid flow; Double-walled carbon nanotube; Density profile; Velocity variation; Nano-fluidics; Filtering; MD simulation

KeyWords Plus:
MOLECULAR-DYNAMICS; FLOW; TRANSPORT; LIQUIDS

Abstract:
Most rnodelling-based research in the field of carbon nanotube-related nano-fluidics has been concerned with the fluid flow in single-walled carbon nanotubes (SWCNTs), showing that the dynamics of the channel affect the structure and behaviour of the fluid. We have extended this work by modelling the flow of Ar in a double-walled carbon nanotube, and have modelled the flow in both the inner shell and the outer annular region of such a nanotube. We have found that the flows in these channels are strongly correlated, such that the fluid moves in opposite directions in these two regions. This phenomenon can give rise to a circulatory motion which can be exploited in nano-fluidic devices. Fluid layering phenomenon, that is usually associated with the flow of fluids in nano-scale channels, is also observed. Furthermore, we have also found that the fluid velocity in dynamic channels is smaller than in static channels, in line with the findings reported for single-walled carbon nan!
otubes. (c) 2009 Elsevier B.V. All rights reserved.

Reprint Address:
Rafii-Tabar, H, IPM, Inst Res Fundamental Sci, POB 19395-5531, Tehran, Iran.

Research Institution addresses:
[Rafii-Tabar, H.] IPM, Inst Res Fundamental Sci, Tehran, Iran; [Yaghmaei, K.] Islam Azad Univ, Grad Sch Environm & Energy Sci & Res, Tehran, Iran; [Rafii-Tabar, H.] Shaheed Beheshti Univ Med Sci, Dept Biomed Engn & Med Phys, Tehran, Iran; [Rafii-Tabar, H.] Shaheed Beheshti Univ Med Sci, Res Ctr Med Nanotechnol & Tissue Engn, Tehran, Iran

E-mail Address:
rafii-tabar@nano.ipm.ac.ir

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Cited Reference Count:
29

Times Cited:
0

Publisher:
ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS

Subject Category:
Materials Science, Multidisciplinary; Physics, Applied

ISSN:
1567-1739

DOI:
10.1016/j.cap.2009.03.015

IDS Number:
459YZ

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ISI Web of Knowledge Alert - Hummer, G

ISI Web of Knowledge Citation Alert

Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
Alert Expires: 22 OCT 2009
Number of Citing Articles: 1 new records this week (1 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Water transport behavior of chitosan porous membranes containing multi-walled carbon nanotubes (MWNTs)

Authors:
Tang, CY; Zhang, Q; Wang, K; Fu, Q; Zhang, CL

Author Full Names:
Tang, Changyu; Zhang, Qin; Wang, Ke; Fu, Qiang; Zhang, Chaoliang

Source:
JOURNAL OF MEMBRANE SCIENCE 337 (1-2): 240-247 JUL 15 2009

Language:
English

Document Type:
Article

Author Keywords:
Chitosan; Multi-walled carbon nanotubes; Polyethylene glycol; Porous membrane; Water transport

KeyWords Plus:
MIXED MATRIX MEMBRANES; MECHANICAL-PROPERTIES; BLEND MEMBRANES; POLYMER BLENDS; GAS SEPARATION; POLYSULFONE; FABRICATION; COMPOSITES; MORPHOLOGY; FLUX

Abstract:
In this work., the effects of MWNTs content on water transport behaviors and tensile properties of prepared chitosan porous membranes were investigated. In the case of chitosan membrane using low molecular weight PEG6000 as a porogen, a percolation-like behavior of water transport rate was observed for the first time in composite membranes with a critical MWNTs content (5 wt%). The water flux of composite membrane with 10 wt% MWNTs (128.1 L/m(2) h) is 4.6 times that of neat one (27.6 L/m(2) h). This could be understood as due to the formation of MWNTs network located among the pore network of chitosan membrane at high MWNTs content, where the hollow nanochannel of MWNTs and their interspaces could provide a new transport channel for water. In contrary, when high molecular weight PEG10000 is used as the porogen, a decreased water flux of the prepared composite membrane is found with increase of MWNTs content. In this case, a strong compatibilizing effect of MWNTs on chitosan/!
PEG10000 blends is observed, resulting in a decreased pore size and poor water flux of the membranes. Furthermore, a greatly improved tensile strength of chitosan porous membranes has been achieved by adding MWNTs, no matter which molecular weight PEG is used as porogen. Our work provides a novel way to improve water flux and/or control the pore size of polymer porous membranes by using MWNTs. (C) 2009 Elsevier B.V. All rights reserved.

Reprint Address:
Fu, Q, Sichuan Univ, Dept Polymer Sci & Mat, State Key Lab Polymer Mat Engn, Chengdu 610065, Peoples R China.

Research Institution addresses:
[Tang, Changyu; Zhang, Qin; Wang, Ke; Fu, Qiang] Sichuan Univ, Dept Polymer Sci & Mat, State Key Lab Polymer Mat Engn, Chengdu 610065, Peoples R China; [Zhang, Chaoliang] State Key Lab Oral Dis, Chengdu 610065, Peoples R China

E-mail Address:
qiangfu@scu.edu.cn

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Cited Reference Count:
36

Times Cited:
0

Publisher:
ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS

Subject Category:
Engineering, Chemical; Polymer Science

ISSN:
0376-7388

DOI:
10.1016/j.memsci.2009.03.048

IDS Number:
458LS

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Cited Article:   Thompson, P. A general boundary condition for liquid flow at solid surfaces Alert Expires:   21 OCT 2009 Number of Citing Articles:   1 new records this week (1 in this e-mail) Organization ID:   3b97d1bbc1878baed0ab183d8b03130b

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Title: Wetting and spreading

Authors: Bonn, D; Eggers, J; Indekeu, J; Meunier, J; Rolley, E

Author Full Names: Bonn, Daniel; Eggers, Jens; Indekeu, Joseph; Meunier, Jacques; Rolley, Etienne

Source: REVIEWS OF MODERN PHYSICS 81 (2): 739-805 APR-JUN 2009

Language: English

Document Type: Review

KeyWords Plus: MOVING CONTACT-LINE; LONG-RANGE FORCES; COLLOID-POLYMER MIXTURES; LIQUID-VAPOR INTERFACES; CRITICAL CASIMIR FORCES; HARD-SPHERE MIXTURES; THIN FLUID FILMS; CHEMICALLY STRUCTURED SURFACES; MONTE-CARLO SIMULATIONS; DRIVEN COATING FILMS

Abstract: Wetting phenomena are ubiquitous in nature and technology. A solid substrate exposed to the environment is almost invariably covered by a layer of fluid material. In this review, the surface forces that lead to wetting are considered, and the equilibrium surface coverage of a substrate in contact with a drop of liquid. Depending on the nature of the surface forces involved, different scenarios for wetting phase transitions are possible; recent progress allows us to relate the critical exponents directly to the nature of the surface forces which lead to the different wetting scenarios. Thermal fluctuation effects, which can be greatly enhanced for wetting of geometrically or chemically structured substrates, and are much stronger in colloidal suspensions, modify the adsorption singularities. Macroscopic descriptions and microscopic theories have been developed to understand and predict wetting behavior relevant to microfluidics and nanofluidics applications. Then the dynamics! of wetting is examined. A drop, placed on a substrate which it wets, spreads out to form a film. Conversely, a nonwetted substrate previously covered by a film dewets upon an appropriate change of system parameters. The hydrodynamics of both wetting and dewetting is influenced by the presence of the three-phase contact line separating "wet" regions from those that are either dry or covered by a microscopic film only. Recent theoretical, experimental, and numerical progress in the description of moving contact line dynamics are reviewed, and its relation to the thermodynamics of wetting is explored. In addition, recent progress on rough surfaces is surveyed. The anchoring of contact lines and contact angle hysteresis are explored resulting from surface inhomogeneities. Further, new ways to mold wetting characteristics according to technological constraints are discussed, for example, the use of patterned surfaces, surfactants, or complex fluids.

Reprint Address: Bonn, D, Ecole Normale Super, Lab Phys Stat, 24 Rue Lhomond, F-75005 Paris, France.

Research Institution addresses: [Bonn, Daniel; Meunier, Jacques; Rolley, Etienne] Ecole Normale Super, Lab Phys Stat, F-75005 Paris, France; [Bonn, Daniel] Univ Amsterdam, Waals Zeeman Inst, NL-1018 XE Amsterdam, Netherlands; [Eggers, Jens] Univ Bristol, Sch Math, Bristol BS8 1TW, Avon, England; [Indekeu, Joseph] Katholieke Univ Leuven, Inst Theoret Fys, B-3001 Louvain, Belgium

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Cited Reference Count: 588

Times Cited: 0

Publisher: AMER PHYSICAL SOC; ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA

Subject Category: Physics, Multidisciplinary

ISSN: 0034-6861

DOI: 10.1103/RevModPhys.81.739

IDS Number: 460OR

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Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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AU Srikar, R
Yarin, AL
Megaridis, CM
AF Srikar, R.
Yarin, A. L.
Megaridis, C. M.
TI Fluidic delivery of homogeneous solutions through carbon tube bundles
SO NANOTECHNOLOGY
LA English
DT Article
ID POLYMER NANOFIBERS; RHODAMINE-B; NANOTUBES; TRANSPORT; RELEASE;
MEMBRANES; DEVICES; FLOW
AB A wide array of technological applications requires localized high-rate
delivery of dissolved compounds (in particular, biological ones), which
can be achieved by forcing the solutions or suspensions of such
compounds through nano or microtubes and their bundled assemblies.
Using a water-soluble compound, the fluorescent dye Rhodamine 610
chloride, frequently used as a model drug release compound, it is shown
that deposit buildup on the inner walls of the delivery channels and
its adverse consequences pose a severe challenge to implementing
pressure-driven long-term fluidic delivery through nano and
microcapillaries, even in the case of such homogeneous solutions.
Pressure-driven delivery (3-6 bar) of homogeneous dye solutions through
macroscopically-long (similar to 1 cm) carbon nano and microtubes with
inner diameters in the range 100 nm-1 mu m and their bundled parallel
assemblies is studied experimentally and theoretically. It is shown
that the flow delivery gradually shifts from fast convection-dominated
(unobstructed) to slow jammed convection, and ultimately to
diffusion-limited transport through a porous deposit. The
jamming/clogging phenomena appear to be rather generic: they were
observed in a wide concentration range for two fluorescent dyes in
carbon nano and microtubes, as well as in comparable transparent glass
microcapillaries. The aim of the present work is to study the physics
of jamming, rather than the chemical reasons for the affinity of dye
molecules to the tube walls.
C1 [Srikar, R.; Yarin, A. L.; Megaridis, C. M.] Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA.
[Yarin, A. L.] Tech Univ Darmstadt, Ctr Smart Interfaces, D-64287 Darmstadt, Germany.
RP Yarin, AL, Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA.
EM ayarin@uic.edu
CR BAZILEVSKY AV, 2008, LAP CHIP, V7, P152
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NR 28
TC 0
PU IOP PUBLISHING LTD; DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND
SN 0957-4484
DI 10.1088/0957-4484/20/27/275706
PD JUL 8
VL 20
IS 27
AR 275706
SC Engineering, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary; Physics, Applied
GA 459GN
UT ISI:000267089600028
ER

PT J
*Record 2 of 3.
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AU Liang, CD
Xie, H
Schwartz, V
Howe, J
Dai, S
Overbury, SH
AF Liang, Chengdu
Xie, Hong
Schwartz, Viviane
Howe, Jane
Dai, Sheng
Overbury, Steven H.
TI Open-Cage Fullerene-like Graphitic Carbons as Catalysts for Oxidative
Dehydrogenation of Isobutane
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID ORDERED MESOPOROUS POLYMERS; BLOCK-COPOLYMERS; NANOTUBES; ETHYLBENZENE;
TRANSFORMATION; FRAMEWORKS
AB We report herein a facile synthesis of fullerene-like cages, which can
be opened and closed through simple thermal treatments. A glassy carbon
with enclosed fullerene-like cages of 2-3 nm was synthesized through a
soft-template approach that created open mesopores of 7 nm. The open
mesopores provided access to the fullerene-like cages, which were
opened and closed through heat treatments in air and inert gas at
various temperatures. Catalytic measurements showed that the open cages
displayed strikingly higher activity for the oxidative dehydrogenation
of isobutane in comparison to the closed ones. We anticipate that this
synthesis approach could unravel an avenue for pursuing fundamental
understanding of the unique catalytic properties of graphitic carbon
nanostructures.
C1 [Liang, Chengdu; Xie, Hong; Schwartz, Viviane; Dai, Sheng; Overbury, Steven H.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.
[Howe, Jane] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA.
[Dai, Sheng; Overbury, Steven H.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA.
RP Liang, CD, Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN
37831 USA.
EM liangcn@ornl.gov
schwartzv@ornl.gov
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10.1016/j.apcata.2007.02.008
NR 30
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
DI 10.1021/ja900888p
PD JUN 10
VL 131
IS 22
BP 7735
EP 7741
SC Chemistry, Multidisciplinary
GA 460HD
UT ISI:000267177900063
ER

PT J
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AU Tang, CY
Zhang, Q
Wang, K
Fu, Q
Zhang, CL
AF Tang, Changyu
Zhang, Qin
Wang, Ke
Fu, Qiang
Zhang, Chaoliang
TI Water transport behavior of chitosan porous membranes containing
multi-walled carbon nanotubes (MWNTs)
SO JOURNAL OF MEMBRANE SCIENCE
LA English
DT Article
DE Chitosan; Multi-walled carbon nanotubes; Polyethylene glycol; Porous
membrane; Water transport
ID MIXED MATRIX MEMBRANES; MECHANICAL-PROPERTIES; BLEND MEMBRANES; POLYMER
BLENDS; GAS SEPARATION; POLYSULFONE; FABRICATION; COMPOSITES;
MORPHOLOGY; FLUX
AB In this work., the effects of MWNTs content on water transport
behaviors and tensile properties of prepared chitosan porous membranes
were investigated. In the case of chitosan membrane using low molecular
weight PEG6000 as a porogen, a percolation-like behavior of water
transport rate was observed for the first time in composite membranes
with a critical MWNTs content (5 wt%). The water flux of composite
membrane with 10 wt% MWNTs (128.1 L/m(2) h) is 4.6 times that of neat
one (27.6 L/m(2) h). This could be understood as due to the formation
of MWNTs network located among the pore network of chitosan membrane at
high MWNTs content, where the hollow nanochannel of MWNTs and their
interspaces could provide a new transport channel for water. In
contrary, when high molecular weight PEG10000 is used as the porogen, a
decreased water flux of the prepared composite membrane is found with
increase of MWNTs content. In this case, a strong compatibilizing
effect of MWNTs on chitosan/PEG10000 blends is observed, resulting in a
decreased pore size and poor water flux of the membranes. Furthermore,
a greatly improved tensile strength of chitosan porous membranes has
been achieved by adding MWNTs, no matter which molecular weight PEG is
used as porogen. Our work provides a novel way to improve water flux
and/or control the pore size of polymer porous membranes by using
MWNTs. (C) 2009 Elsevier B.V. All rights reserved.
C1 [Tang, Changyu; Zhang, Qin; Wang, Ke; Fu, Qiang] Sichuan Univ, Dept Polymer Sci & Mat, State Key Lab Polymer Mat Engn, Chengdu 610065, Peoples R China.
[Zhang, Chaoliang] State Key Lab Oral Dis, Chengdu 610065, Peoples R China.
RP Fu, Q, Sichuan Univ, Dept Polymer Sci & Mat, State Key Lab Polymer Mat
Engn, Chengdu 610065, Peoples R China.
EM qiangfu@scu.edu.cn
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NR 36
TC 0
PU ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0376-7388
DI 10.1016/j.memsci.2009.03.048
PD JUL 15
VL 337
IS 1-2
BP 240
EP 247
SC Engineering, Chemical; Polymer Science
GA 458LS
UT ISI:000267025500027
ER

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ISI Web of Knowledge Alert - Majumder M

ISI Web of Knowledge Citation Alert

Cited Article: Majumder M. Nanoscale hydrodynamics - Enhanced flow in carbon nanotubes
Alert Expires: 18 OCT 2009
Number of Citing Articles: 2 new records this week (2 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Fluidic delivery of homogeneous solutions through carbon tube bundles

Authors:
Srikar, R; Yarin, AL; Megaridis, CM

Author Full Names:
Srikar, R.; Yarin, A. L.; Megaridis, C. M.

Source:
NANOTECHNOLOGY 20 (27): Art. No. 275706 JUL 8 2009

Language:
English

Document Type:
Article

KeyWords Plus:
POLYMER NANOFIBERS; RHODAMINE-B; NANOTUBES; TRANSPORT; RELEASE; MEMBRANES; DEVICES; FLOW

Abstract:
A wide array of technological applications requires localized high-rate delivery of dissolved compounds (in particular, biological ones), which can be achieved by forcing the solutions or suspensions of such compounds through nano or microtubes and their bundled assemblies. Using a water-soluble compound, the fluorescent dye Rhodamine 610 chloride, frequently used as a model drug release compound, it is shown that deposit buildup on the inner walls of the delivery channels and its adverse consequences pose a severe challenge to implementing pressure-driven long-term fluidic delivery through nano and microcapillaries, even in the case of such homogeneous solutions. Pressure-driven delivery (3-6 bar) of homogeneous dye solutions through macroscopically-long (similar to 1 cm) carbon nano and microtubes with inner diameters in the range 100 nm-1 mu m and their bundled parallel assemblies is studied experimentally and theoretically. It is shown that the flow delivery gradually sh!
ifts from fast convection-dominated (unobstructed) to slow jammed convection, and ultimately to diffusion-limited transport through a porous deposit. The jamming/clogging phenomena appear to be rather generic: they were observed in a wide concentration range for two fluorescent dyes in carbon nano and microtubes, as well as in comparable transparent glass microcapillaries. The aim of the present work is to study the physics of jamming, rather than the chemical reasons for the affinity of dye molecules to the tube walls.

Reprint Address:
Yarin, AL, Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA.

Research Institution addresses:
[Srikar, R.; Yarin, A. L.; Megaridis, C. M.] Univ Illinois, Dept Mech & Ind Engn, Chicago, IL 60607 USA; [Yarin, A. L.] Tech Univ Darmstadt, Ctr Smart Interfaces, D-64287 Darmstadt, Germany

E-mail Address:
ayarin@uic.edu

Cited References:
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ZUSSMAN E, 2006, ADV MATER, V18, P348, DOI 10.1002/adma.200501153.

Cited Reference Count:
28

Times Cited:
0

Publisher:
IOP PUBLISHING LTD; DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND

Subject Category:
Engineering, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied

ISSN:
0957-4484

DOI:
10.1088/0957-4484/20/27/275706

IDS Number:
459GN

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Title:
Open-Cage Fullerene-like Graphitic Carbons as Catalysts for Oxidative Dehydrogenation of Isobutane

Authors:
Liang, CD; Xie, H; Schwartz, V; Howe, J; Dai, S; Overbury, SH

Author Full Names:
Liang, Chengdu; Xie, Hong; Schwartz, Viviane; Howe, Jane; Dai, Sheng; Overbury, Steven H.

Source:
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY 131 (22): 7735-7741 JUN 10 2009

Language:
English

Document Type:
Article

KeyWords Plus:
ORDERED MESOPOROUS POLYMERS; BLOCK-COPOLYMERS; NANOTUBES; ETHYLBENZENE; TRANSFORMATION; FRAMEWORKS

Abstract:
We report herein a facile synthesis of fullerene-like cages, which can be opened and closed through simple thermal treatments. A glassy carbon with enclosed fullerene-like cages of 2-3 nm was synthesized through a soft-template approach that created open mesopores of 7 nm. The open mesopores provided access to the fullerene-like cages, which were opened and closed through heat treatments in air and inert gas at various temperatures. Catalytic measurements showed that the open cages displayed strikingly higher activity for the oxidative dehydrogenation of isobutane in comparison to the closed ones. We anticipate that this synthesis approach could unravel an avenue for pursuing fundamental understanding of the unique catalytic properties of graphitic carbon nanostructures.

Reprint Address:
Liang, CD, Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA.

Research Institution addresses:
[Liang, Chengdu; Xie, Hong; Schwartz, Viviane; Dai, Sheng; Overbury, Steven H.] Oak Ridge Natl Lab, Ctr Nanophase Mat Sci, Oak Ridge, TN 37831 USA; [Howe, Jane] Oak Ridge Natl Lab, Div Mat Sci & Technol, Oak Ridge, TN 37831 USA; [Dai, Sheng; Overbury, Steven H.] Oak Ridge Natl Lab, Div Chem Sci, Oak Ridge, TN 37831 USA

E-mail Address:
liangcn@ornl.gov; schwartzv@ornl.gov

Cited References:
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Cited Reference Count:
30

Times Cited:
0

Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA

Subject Category:
Chemistry, Multidisciplinary

ISSN:
0002-7863

DOI:
10.1021/ja900888p

IDS Number:
460HD

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ISI Web of Knowledge Alert - Ghosh, S

ISI Web of Knowledge Citation Alert

Cited Article: Ghosh, S. Carbon nanotube flow sensors
Alert Expires: 22 OCT 2009
Number of Citing Articles: 1 new records this week (1 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Interaction kinetics of atoms and molecules on carbon nanotube surfaces

Authors:
Ulbricht, H

Author Full Names:
Ulbricht, Hendrik

Source:
SURFACE SCIENCE 603 (10-12): 1853-1862 Sp. Iss. SI JUN 1 2009

Language:
English

Document Type:
Article

Author Keywords:
Thermal desorption spectroscopy; Electrical transport measurements; Laser induced thermal desorption (LITD); Adsorption kinetics; Surface diffusion; Ammonia; Xenon; Carbon nanotubes

KeyWords Plus:
PHYSICAL ADSORPTION; THERMOELECTRIC-POWER; THERMAL-DESORPTION; GRAPHITE; BUNDLES; GASES; XE; SENSITIVITY; HYDROGEN; SENSORS

Abstract:
We review recent experimental investigations of the interaction of gases with the surface of single-wall carbon nanotube bundles. We discuss thermal desorption spectra of both non-polar and polar adsorbates for low and high coverage. We show experimental results for diffusion processes of Xe along and within carbon nanotube bucky paper material, which is consistent with a recently proposed coupled desorption diffusion (CDD) model. We further discuss details of the interaction of ammonia with carbon nanotube surfaces, including the experimental investigation of the influence of adsorbed ammonia on the electrical transport properties of carbon nanotubes under ultra-high vacuum conditions. (C) 2009 Elsevier B.V. All rights reserved.

Reprint Address:
Ulbricht, H, Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England.

Research Institution addresses:
Univ Southampton, Sch Phys & Astron, Southampton SO17 1BJ, Hants, England

E-mail Address:
h.ulbricht@soton.ac.uk

Cited References:
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Cited Reference Count:
48

Times Cited:
0

Publisher:
ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS

Subject Category:
Chemistry, Physical; Physics, Condensed Matter

ISSN:
0039-6028

DOI:
10.1016/j.susc.2008.09.062

IDS Number:
455ST

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