Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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AU Shiomi, J
Maruyama, S
AF Shiomi, J.
Maruyama, S.
TI Water transport inside a single-walled carbon nanotube driven by a
temperature gradient
SO NANOTECHNOLOGY
LA English
DT Article
ID MOLECULAR-DYNAMICS SIMULATION; HEAT-CONDUCTION; MASS-TRANSPORT;
ICE-NANOTUBES
AB In this work, by means of molecular dynamics simulations, we consider
the mass transport of a water cluster inside a single-walled carbon
nanotube (SWNT) with a diameter of about 1.4 nm. The influence of the
non-equilibrium thermal environment on the confined water cluster has
been investigated by imposing a longitudinal temperature gradient on
the SWNT. It is demonstrated that the water cluster is transported with
an average acceleration proportional to the temperature gradient.
Additional equilibrium simulations suggest that the temperature
dependence of the potential energy of the confined water is sufficient
to realize the transport. In particular, for a system with a
hydrophobic interface, the water-water intrinsic potential energy
appears to play a dominant role. The transport simulations were also
performed for a system with a junction between two different SWNTs. The
results suggest that an angstrom difference in diameter may result in a
large barrier for water being transported through a small diameter SWNT.
C1 [Shiomi, J.; Maruyama, S.] Univ Tokyo, Dept Mech Engn, Bunkyo Ku, Tokyo 1138656, Japan.
RP Shiomi, J, Univ Tokyo, Dept Mech Engn, Bunkyo Ku, 7-3-1 Hongo, Tokyo
1138656, Japan.
EM shiomi@photon.t.u-tokyo.ac.jp
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NR 22
TC 0
PU IOP PUBLISHING LTD; DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND
SN 0957-4484
DI 10.1088/0957-4484/20/5/055708
PD FEB 4
PY 2009
VL 20
IS 5
AR 055708
SC Engineering, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary; Physics, Applied
GA 393LV
UT ISI:000262375700036
ER
PT J
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AU Kong, J
Xu, Y
Yung, KL
Xie, YC
He, L
AF Kong, Jie
Xu, Yan
Yung, Kai-Leung
Xie, Yunchuan
He, Lan
TI Enhanced Polymer Melts Flow though Nanoscale Channels under Vibration
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID MOLECULAR-DYNAMICS SIMULATION; WALLED CARBON NANOTUBES; WATER;
NANOCHANNELS; BEHAVIOR; NANOCRYSTALS; CAPILLARIES; CONDUCTION;
NANOFIBERS; INTERFACE
AB The enhanced poly(epsilon-caprolactone) melts flow behaviors though
nanoscale channels under vibration were observed. The effect of
vibration on the nanoflow is dependent on the vibration frequency of
piezoelectric transducer that generates the vibration fields. The flow
rate of poly(epsilon-caprolactone) melts in nanochannels increases with
the increase of vibration frequency within the range from 2.0 to 14.0
kHz. The observed enhanced flow through nanochannels under vibration is
a new nanoscale phenomenon, which is potential in vibration-assisted
nanofluidic, nanoimprint lithography, and micro-/nanoinjection molding
etc.
C1 [Kong, Jie; Xu, Yan; Yung, Kai-Leung; Xie, Yunchuan; He, Lan] Hong Kong Polytech Univ, Dept Ind & Syst Engn, Kowloon, Hong Kong, Peoples R China.
[Kong, Jie] NW Polytech Univ, Sch Sci, Dept Appl Chem, Xian 710072, Peoples R China.
RP Kong, J, Hong Kong Polytech Univ, Dept Ind & Syst Engn, Kowloon, Hong
Kong, Peoples R China.
EM mfkongjie@hotmail.com
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NR 44
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
DI 10.1021/jp809164k
PD JAN 15
PY 2009
VL 113
IS 2
BP 624
EP 629
SC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
GA 392TH
UT ISI:000262324600022
ER
PT J
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AU Li, YX
Ito, T
AF Li, Yongxin
Ito, Takashi
TI Size-Exclusion Properties of Nanoporous Films Derived from
Polystyrene-Poly(methylmethacrylate) Diblock Copolymers Assessed Using
Direct Electrochemistry of Ferritin
SO ANALYTICAL CHEMISTRY
LA English
DT Article
ID SELF-ASSEMBLED MONOLAYERS; DIRECT ELECTRON-TRANSFER; INDIUM OXIDE
ELECTRODES; BLOCK-COPOLYMERS; NANOTUBE MEMBRANES; PROTEIN-TRANSPORT;
GOLD ELECTRODES; TEMPLATES; SURFACE; POLYSTYRENE
AB This paper reports the size-exclusion properties of nanoporous films
derived from polystyrene-poly(methylmethacrylate) diblock copolymers
(PS-b-PMMA) for biomacro-molecules. These properties were assessed by
measuring cyclic voltammetry of ferritin (12 nm in diameter) adsorbed
onto recessed nanodisk-array gold electrodes (RNEs) fabricated from the
nanoporous films having different effective pore diameters and surface
functionalities. RNEs having 20-nm-diameter nanopores modified with a
poly(ethylene glycol) (PEG) layer showed the redox currents of ferritin
after their immersion in a ferritin solution (5 mg/mL) for longer than
2 h. The currents originated from the direct electron transfer reaction
of ferritin molecules immobilized on the underlying gold surface as a
result of their penetration through the 20-nm-diameter nanopores. The
PEG modification of the nanopore surface was required for the
penetration of ferritin, probably because it reduced the nonspecific
adsorption of ferritin to the nanopore surface. In contrast, no redox
current of ferritin was observed for RNEs having PEG-modified
15-nm-diameter nanopores after their immersion in the ferritin solution
for 12 h, indicating the size-exclusion of ferritin from the 15-nm
nanopores. The distinct size-exclusion properties of the
PS-b-PMMA-derived nanoporous films reflect their uniform diameters and
shapes and will provide a means for fabricating separation membranes
for biomolecules with high size-based selectivity.
C1 [Li, Yongxin; Ito, Takashi] Kansas State Univ, Dept Chem, Manhattan, KS 66506 USA.
RP Ito, T, Kansas State Univ, Dept Chem, 111 Willard Hall, Manhattan, KS
66506 USA.
EM ito@ksu.edu
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NR 37
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0003-2700
DI 10.1021/ac802201w
PD JAN 15
PY 2009
VL 81
IS 2
BP 851
EP 855
SC Chemistry, Analytical
GA 394WB
UT ISI:000262482700044
ER
EF
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