Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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AU Rawat, DS
Krungleviciute, V
Heroux, L
Bulut, A
Calbi, AA
Migone, AD
AF Rawat, D. S.
Krungleviciute, V.
Heroux, L.
Bulut, A.
Calbi, A. A.
Migone, A. D.
TI Dependence of Single-Walled Carbon Nanotube Adsorption Kinetics on
Temperature and Binding Energy
SO LANGMUIR
LA English
DT Article
ID GAS-ADSORPTION; DESORPTION-KINETICS; EXTERNAL SURFACES; SELF-DIFFUSION;
MASS-TRANSPORT; BUNDLES; MEMBRANES; CF4; PHYSISORPTION; SIMULATIONS
AB We present results for the isothermal adsorption kinetics of methane,
hydrogen, and tetrafluoromethane on closed-ended single-walled carbon
nanotubes. In these experiments, we monitor the pressure decrease as a
function of time as equilibrium is approached, after a dose of gas is
added to the cell containing the nanotubes. The measurements were
performed at different fractional coverages limited to the first layer.
The results indicate that, for a given coverage and temperature, the
equilibration time is an increasing function of E/(k(B)T), where E is
the binding energy of the adsorbate and k(B)T is the thermal energy.
These findings are consistent with recent theoretical predictions and
Computer simulations results that we use to interpret the experimental
measurements.
C1 [Rawat, D. S.; Krungleviciute, V.; Heroux, L.; Bulut, A.; Calbi, A. A.; Migone, A. D.] So Illinois Univ, Dept Phys, Carbondale, IL 62901 USA.
RP Migone, AD, So Illinois Univ, Dept Phys, Carbondale, IL 62901 USA.
EM aldo@physics.siu.edu
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NR 72
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0743-7463
DI 10.1021/la8022002
PD DEC 2
PY 2008
VL 24
IS 23
BP 13465
EP 13469
SC Chemistry, Physical
GA 376XO
UT ISI:000261216500036
ER
PT J
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AU Hylton, K
Chen, YH
Mitra, S
AF Hylton, Kamilah
Chen, Yuhong
Mitra, Somenath
TI Carbon nanotube mediated microscale membrane extraction
SO JOURNAL OF CHROMATOGRAPHY A
LA English
DT Article
DE Carbon nanotube; Membrane; Membrane extraction
ID MIXED MATRIX MEMBRANES; LIQUID-PHASE MICROEXTRACTION; HOLLOW-FIBER
MEMBRANES; GAS SEPARATION; SAMPLE PREPARATION; WATER; CHROMATOGRAPHY;
TRANSPORT; FUNCTIONALIZATION; PESTICIDES
AB We demonstrate that functionalized carbon nanotubes can be readily
immobilized into the pore structure of a polymeric membrane, which can
dramatically improve its performance in analytical scale membrane
extraction. This was accomplished by injecting an aqueous dispersion of
the nanotubes through a Polypropylene hollow fiber under pressure. The
nanotubes were trapped and held within the pores and served as sorbents
facilitating solute exchange from the donor to the acceptor phase. The
effectiveness of this carbon nanotube mediated process was studied by
direct solvent enrichment of nonpolar organics, and also by selective
extraction of organic acids via a supported liquid membrane. In both
cases, the enrichment factor measured as the ratio of concentrations in
the acceptor to the donor-phases could be increased by more than 200%.
(C) 2008 Elsevier B.V. All rights reserved.
C1 [Chen, Yuhong; Mitra, Somenath] Univ Heights, New Jersey Inst Technol, Dept Chem & Environm Sci, Newark, NJ 07104 USA.
[Hylton, Kamilah] Univ Technol, Jamaica, WI USA.
RP Mitra, S, Univ Heights, New Jersey Inst Technol, Dept Chem & Environm
Sci, Newark, NJ 07104 USA.
EM Mitra@njit.edu
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NR 47
TC 0
PU ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0021-9673
DI 10.1016/j.chroma.2008.09.092
PD NOV 21
PY 2008
VL 1211
IS 1-2
BP 43
EP 48
SC Biochemical Research Methods; Chemistry, Analytical
GA 377RM
UT ISI:000261268300006
ER
EF
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