Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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AU Gurdev, S
Rana, D
Matsuura, T
Ramakrishna, S
Narbaitz, RM
Tabe, S
AF Singh, Gurdev
Rana, Dipak
Matsuura, Takeshi
Ramakrishna, Seeram
Narbaitz, Roberto M.
Tabe, Shahram
TI Removal of disinfection byproducts from water by carbonized electrospun
nanofibrous membranes
SO SEPARATION AND PURIFICATION TECHNOLOGY
LA English
DT Article
DE Disinfection byproducts; Electrospun membrane; Carbonized nanofibrous
membrane; Multiwalled carbon nanotubes; Membrane adsorption
ID ENVIRONMENTAL APPLICATIONS; NANOTUBE MEMBRANES; MASS-TRANSPORT;
ADSORPTION; PURIFICATION; SURFACE; TRIHALOMETHANES; FILTERS; MEDIA;
LAYER
AB Disinfection byproducts (DBPs), trihalomethanes and haloacetic acids
present in water are well known carcinogens and their removal is an
important priority. Highly porous nanofibrous membrane filters produced
by electro-spinning were carbonized and used for the removal of DBPs
from water. In the present investigation, chloroform and
monochloroacetic acid (MCAA) was used as model DBPs compounds. The DBPs
concentration in the range of 1-100 mg/L was used in well controlled
adsorption experiments using the prepared membranes. For chloroform an
adsorption capacity of 554 mg/g of carbonized nanofibrous membranes
(CNMs) was determined based on the filtration of feed solution (100
mg/L). The adsorption capacity of MCAA was between 287 and 504 mg/g for
a feed concentration of 4-18 mg/L based on the static adsorption study.
The used membranes were regenerated by chemical/physical treatment and
removal efficiencies of the regenerated membranes were determined. The
DBPs removal from water was also investigated using multiwalled carbon
nanotubes (MWCNTs) incorporated in the CNMs and results were compared.
Although the initial removal of MCAA was increased with increasing
concentration of the MWCNTs, afterwards, the subsequent removals showed
no effect of addition of MWCNTs. The possible mechanism was also
discussed to better understand the adsorption phenomenon. These results
suggest that the CNMs could be used as DBPs removal filter for drinking
water purpose. (C) 2010 Elsevier B.V. All rights reserved.
C1 [Singh, Gurdev; Rana, Dipak; Matsuura, Takeshi] Univ Ottawa, Ind Membrane Res Inst, Dept Chem & Biol Engn, Ottawa, ON K1N 6N5, Canada.
[Singh, Gurdev; Ramakrishna, Seeram] Natl Univ Singapore, Fac Engn, Nanosci & Nanotechnol Initiat, Blk Nanobioengn Lab E3 05 12, Singapore 117576, Singapore.
[Narbaitz, Roberto M.] Univ Ottawa, Dept Civil Engn, Ottawa, ON K1N 6N5, Canada.
[Tabe, Shahram] Ontario Minist Environm, Stand Dev Branch, Water Stand Sect, Toronto, ON M4V 1M2, Canada.
RP Rana, D, Univ Ottawa, Ind Membrane Res Inst, Dept Chem & Biol Engn, 161
Louis Pasteur St, Ottawa, ON K1N 6N5, Canada.
EM rana@eng.uottawa.ca
matsuura@eng.uottawa.ca
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NR 77
TC 0
PU ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 1383-5866
DI 10.1016/j.seppur.2010.06.006
PD AUG 17
VL 74
IS 2
BP 202
EP 212
SC Engineering, Chemical
GA 647NF
UT ISI:000281624500007
ER
PT J
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AU Lee, CY
Choi, W
Han, JH
Strano, MS
AF Lee, Chang Young
Choi, Wonjoon
Han, Jae-Hee
Strano, Michael S.
TI Coherence Resonance in a Single-Walled Carbon Nanotube Ion Channel
SO SCIENCE
LA English
DT Article
ID STOCHASTIC RESONANCE; MEMBRANE PATCHES; SURFACE-CHARGE; K+ CHANNEL;
NOISE; TRANSPORT; WATER; TRANSLOCATION; COORDINATION; ENHANCEMENT
AB Biological ion channels are able to generate coherent and oscillatory
signals from intrinsically noisy and stochastic components for
ultrasensitive discrimination with the use of stochastic resonance, a
concept not yet demonstrated in human-made analogs. We show that a
single-walled carbon nanotube demonstrates oscillations in
electroosmotic current through its interior at specific ranges of
electric field that are the signatures of coherence resonance.
Stochastic pore blocking is observed when individual cations partition
into the nanotube obstructing an otherwise stable proton current. The
observed oscillations occur because of coupling between pore blocking
and a proton-diffusion limitation at the pore mouth. The result
illustrates how simple ionic transport can generate coherent waveforms
within an inherently noisy environment and points to new types of
nanoreactors, sensors, and nanofluidic channels based on this platform.
C1 [Lee, Chang Young; Choi, Wonjoon; Han, Jae-Hee; Strano, Michael S.] MIT, Dept Chem Engn, Cambridge, MA 02139 USA.
[Choi, Wonjoon] MIT, Dept Mech Engn, Cambridge, MA 02139 USA.
RP Strano, MS, MIT, Dept Chem Engn, Cambridge, MA 02139 USA.
EM strano@mit.edu
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NR 39
TC 0
PU AMER ASSOC ADVANCEMENT SCIENCE; 1200 NEW YORK AVE, NW, WASHINGTON, DC
20005 USA
SN 0036-8075
DI 10.1126/science.1193383
PD SEP 10
VL 329
IS 5997
BP 1320
EP 1324
SC Multidisciplinary Sciences
GA 647YR
UT ISI:000281657300032
ER
PT J
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AU Kong, CL
Kanezashi, M
Yamomoto, T
Shintani, T
Tsuru, T
AF Kong, Chunlong
Kanezashi, Masakoto
Yamomoto, Tetsuya
Shintani, Takuji
Tsuru, Toshinori
TI Controlled synthesis of high performance polyamide membrane with thin
dense layer for water desalination
SO JOURNAL OF MEMBRANE SCIENCE
LA English
DT Article
DE Polyamide; Co-solvent; Interfacial polymerization; Nanofiltration;
Desalination
ID REVERSE-OSMOSIS MEMBRANES; NANOFILTRATION MEMBRANES; INTERFACIAL
POLYMERIZATION; RO MEMBRANES; SEPARATION; ELECTROLYTES; TRANSPORT
AB A new concept for the synthesis of thin polyamide nanofiltration
membranes on ultrafiltration polysulfone supports is reported.
Polyamide membranes with controllable thin dense layer and effective
"nanopores" were fabricated by adding co-solvent (acetone) to nonpolar
organic phase (hexane), referred to as co-solvent assisted interfacial
polymerization (CAIP), which exhibited a high water flux with no
considerable salt rejection loss Higher co-solvent addition into the
hexane solution resulted in relatively larger pore sizes as well as
higher water fluxes, which were determined by the analysis of membrane
permeation data using aqueous solutions of sodium chloride. The best
nanocomposite membrane that was prepared with 2 wt% of acetone showed
approximate 4 times higher water flux with no considerable rejection
loss than polyamide membranes fabricated with no acetone co-solvent The
CAIP method will offer new degrees of freedom in modifying polymer
membrane with high separation performance (C) 2010 Elsevier B V All
rights reserved
C1 [Kong, Chunlong; Kanezashi, Masakoto; Yamomoto, Tetsuya; Tsuru, Toshinori] Hiroshima Univ, Dept Chem Engn, Higashihiroshima 7398527, Japan.
[Shintani, Takuji] Nitto Denko Corp, Osaka 5678860, Japan.
RP Tsuru, T, Hiroshima Univ, Dept Chem Engn, Higashihiroshima 7398527,
Japan.
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NR 24
TC 0
PU ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0376-7388
DI 10.1016/j.memsci.2010.06.022
PD OCT 15
VL 362
IS 1-2
BP 76
EP 80
SC Engineering, Chemical; Polymer Science
GA 646VK
UT ISI:000281571100008
ER
PT J
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AU Wu, HQ
Tang, BB
Wu, PY
AF Wu, Huiqing
Tang, Beibei
Wu, Peiyi
TI Novel ultrafiltration membranes prepared from a multi-walled carbon
nanotubes/polymer composite
SO JOURNAL OF MEMBRANE SCIENCE
LA English
DT Article
DE Multi-walled carbon nanotubes (MWNTs); Brominated polyphenylene oxide
(BPPO); Dry-wet phase inversion; Hydrophilicity
ID GAS SEPARATION; INTERFACIAL POLYMERIZATION; NANOTUBE MEMBRANES; PHASE
INVERSION; MASS-TRANSPORT; POLYSULFONE; FABRICATION; PERMEATION;
MIXTURES; TRADEOFF
AB Novel ultrafiltration membranes were prepared by incorporating
multi-walled carbon nanotubes (MWNTs) Into a matrix of brominated
polyphenylene oxide (BPPO) and using triethanolamine (TEOA) as the
crosslinking agent The membranes exhibited not only high permeability
and hydrophilicity but also excellent separation performance and
chemical stability Furthermore, the water permeability increased as the
weight fraction of MWNTs Increased, reaching a maximum of 487 L/m(2) h
at 5 wt% of MWNTs, while maintaining a 94% membrane rejection rate to
egg albumin The addition of TEOA into the BPPO/MWNTs casting solution
might result in an increase in water permeation rate of membrane if the
amount of TEOA exceeded a threshold value, however, the membrane
rejection rate was essentially constant despite increasing the molar
fraction of TEOA in the casting solution. Using an adequate amount of
MWNTs and a proper TEOA/BPPO ratio, it is feasible to make
MWNTs/polymer ultrafiltration membranes with both high permeation flux
and excellent selectivity (C) 2010 Elsevier B.V. All rights reserved.
C1 [Tang, Beibei] Fudan Univ, Dept Macromol Sci, Key Lab Mol Engn Polymers, Minist Educ, Shanghai 200433, Peoples R China.
Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China.
RP Tang, BB, Fudan Univ, Dept Macromol Sci, Key Lab Mol Engn Polymers,
Minist Educ, Shanghai 200433, Peoples R China.
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NR 26
TC 0
PU ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
SN 0376-7388
DI 10.1016/j.memsci.2010.06.064
PD OCT 15
VL 362
IS 1-2
BP 374
EP 383
SC Engineering, Chemical; Polymer Science
GA 646VK
UT ISI:000281571100042
ER
EF
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or 734-459-8565.
IDS Customers
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IDS customers can purchase the full text of an article (having page number,
volume, and issue information) by returning this ENTIRE message as a Reply
to Sender or Forward to orders@isidoc.com. Mark your choices with an X in
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Please enter your account number here:
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*Import Records into an ISI ResearchSoft product*
1) Save the email as a text file. If your e-mail software removed extra line breaks, restore them before saving.
2) From within an ISI ResearchSoft product, import the text file using the ISI-CE filter.
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*Help Desk Contact Information*
If you have any questions, please visit the Thomson Scientific Technical Support Contact Information Web page:
http://www.thomsonscientific.com/support/techsupport
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