Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
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Title:
Removal of disinfection byproducts from water by carbonized electrospun nanofibrous membranes
Authors:
Gurdev, S; Rana, D; Matsuura, T; Ramakrishna, S; Narbaitz, RM; Tabe, S
Author Full Names:
Singh, Gurdev; Rana, Dipak; Matsuura, Takeshi; Ramakrishna, Seeram; Narbaitz, Roberto M.; Tabe, Shahram
Source:
SEPARATION AND PURIFICATION TECHNOLOGY 74 (2): 202-212 AUG 17 2010
Language:
English
Document Type:
Article
Author Keywords:
Disinfection byproducts; Electrospun membrane; Carbonized nanofibrous membrane; Multiwalled carbon nanotubes; Membrane adsorption
KeyWords Plus:
ENVIRONMENTAL APPLICATIONS; NANOTUBE MEMBRANES; MASS-TRANSPORT; ADSORPTION; PURIFICATION; SURFACE; TRIHALOMETHANES; FILTERS; MEDIA; LAYER
Abstract:
Disinfection byproducts (DBPs), trihalomethanes and haloacetic acids present in water are well known carcinogens and their removal is an important priority. Highly porous nanofibrous membrane filters produced by electro-spinning were carbonized and used for the removal of DBPs from water. In the present investigation, chloroform and monochloroacetic acid (MCAA) was used as model DBPs compounds. The DBPs concentration in the range of 1-100 mg/L was used in well controlled adsorption experiments using the prepared membranes. For chloroform an adsorption capacity of 554 mg/g of carbonized nanofibrous membranes (CNMs) was determined based on the filtration of feed solution (100 mg/L). The adsorption capacity of MCAA was between 287 and 504 mg/g for a feed concentration of 4-18 mg/L based on the static adsorption study. The used membranes were regenerated by chemical/physical treatment and removal efficiencies of the regenerated membranes were determined. The DBPs removal from wat
er was also investigated using multiwalled carbon nanotubes (MWCNTs) incorporated in the CNMs and results were compared. Although the initial removal of MCAA was increased with increasing concentration of the MWCNTs, afterwards, the subsequent removals showed no effect of addition of MWCNTs. The possible mechanism was also discussed to better understand the adsorption phenomenon. These results suggest that the CNMs could be used as DBPs removal filter for drinking water purpose. (C) 2010 Elsevier B.V. All rights reserved.
Reprint Address:
Rana, D, Univ Ottawa, Ind Membrane Res Inst, Dept Chem & Biol Engn, 161 Louis Pasteur St, Ottawa, ON K1N 6N5, Canada.
Research Institution addresses:
[Singh, Gurdev; Rana, Dipak; Matsuura, Takeshi] Univ Ottawa, Ind Membrane Res Inst, Dept Chem & Biol Engn, Ottawa, ON K1N 6N5, Canada; [Singh, Gurdev; Ramakrishna, Seeram] Natl Univ Singapore, Fac Engn, Nanosci & Nanotechnol Initiat, Blk Nanobioengn Lab E3 05 12, Singapore 117576, Singapore; [Narbaitz, Roberto M.] Univ Ottawa, Dept Civil Engn, Ottawa, ON K1N 6N5, Canada; [Tabe, Shahram] Ontario Minist Environm, Stand Dev Branch, Water Stand Sect, Toronto, ON M4V 1M2, Canada
E-mail Address:
rana@eng.uottawa.ca; matsuura@eng.uottawa.ca
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Cited Reference Count:
77
Times Cited:
0
Publisher:
ELSEVIER SCIENCE BV; PO BOX 211, 1000 AE AMSTERDAM, NETHERLANDS
Subject Category:
Engineering, Chemical
ISSN:
1383-5866
DOI:
10.1016/j.seppur.2010.06.006
IDS Number:
647NF
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Title:
How Can Hydrophobic Association Be Enthalpy Driven?
Authors:
Setny, P; Baron, R; McCammon, JA
Author Full Names:
Setny, Piotr; Baron, Riccardo; McCammon, J. Andrew
Source:
JOURNAL OF CHEMICAL THEORY AND COMPUTATION 6 (9): 2866-2871 SEP 2010
Language:
English
Document Type:
Article
KeyWords Plus:
MAJOR URINARY PROTEIN; TEMPERATURE-DEPENDENCE; DEWETTING TRANSITION; FREE-ENERGY; COMPUTER-SIMULATION; POTENTIAL FUNCTIONS; MOLECULAR-DYNAMICS; NONPOLAR CAVITIES; LIGAND-BINDING; WATER CLUSTERS
Abstract:
Hydrophobic association is often recognized as being driven by favorable entropic contributions. Here, using explicit solvent molecular dynamics simulations we investigate binding in a model hydrophobic receptor ligand system which appears, instead, to be driven by enthalpy and opposed by entropy. We use the temperature dependence of the potential of mean force to analyze the thermodynamic contributions along the association coordinate. Relating such contributions to the ongoing changes in system hydration allows us to demonstrate that the overall binding thermodynamics is determined by the expulsion of disorganized water from the receptor cavity. Our model study sheds light on the solvent-induced driving forces for receptor ligand association of general, transferable relevance for biological systems with poorly hydrated binding sites.
Reprint Address:
Setny, P, Univ Calif San Diego, Dept Chem & Biochem, Ctr Theoret Biol Phys, Howard Hughes Med Inst,Dept Pharmacol, San Diego, CA 92103 USA.
Research Institution addresses:
[Setny, Piotr; Baron, Riccardo; McCammon, J. Andrew] Univ Calif San Diego, Dept Chem & Biochem, Ctr Theoret Biol Phys, Howard Hughes Med Inst,Dept Pharmacol, San Diego, CA 92103 USA; [Setny, Piotr] Tech Univ Munich, Dept Phys, D-85748 Garching, Germany
E-mail Address:
piotr.setny@tum.de; rbaron@mecammon.ucsd.edu
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Times Cited:
0
Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Subject Category:
Chemistry, Physical; Physics, Atomic, Molecular & Chemical
ISSN:
1549-9618
DOI:
10.1021/ct1003077
IDS Number:
648KQ
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Title:
Ion Interactions with the Carbon Nanotube Surface in Aqueous Solutions: Understanding the Molecular Mechanisms
Authors:
Frolov, AI; Rozhin, AG; Fedorov, MV
Author Full Names:
Frolov, Andrey I.; Rozhin, Alex G.; Fedorov, Maxim V.
Source:
CHEMPHYSCHEM 11 (12): 2612-2616 AUG 23 2010
Language:
English
Document Type:
Article
Author Keywords:
molecular simulations; nanotube modeling; nanotubes; photoluminescence; specific salt effects
KeyWords Plus:
DYNAMICS SIMULATIONS; BIOMOLECULAR SIMULATIONS; BIOMEDICAL APPLICATIONS; HYDROPHOBIC SURFACE; WATER-STRUCTURE; SALT-SOLUTIONS; METAL-IONS; HYDRATION; SOLVENT; THERMODYNAMICS
Abstract:
We study the molecular mechanisms of alkali halide ion interactions with the single-wall carbon nanotube surface in water by means of fully atomistic molecular dynamics simulations. We focus on the basic physical-chemical principles of ion-nanotube interactions in aqueous solutions and discuss them in light of recent experimental findings on selective ion effects on carbon nanotubes.
Reprint Address:
Fedorov, MV, Max Planck Inst Math Sci, D-04103 Leipzig, Germany.
Research Institution addresses:
[Frolov, Andrey I.; Fedorov, Maxim V.] Max Planck Inst Math Sci, D-04103 Leipzig, Germany; [Rozhin, Alex G.] Aston Univ, Sch Engn & Appl Sci, Birmingham B4 7ET, W Midlands, England
E-mail Address:
fedorov@mis.mpg.de
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Cited Reference Count:
66
Times Cited:
0
Publisher:
WILEY-V C H VERLAG GMBH; PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
Subject Category:
Chemistry, Physical; Physics, Atomic, Molecular & Chemical
ISSN:
1439-4235
DOI:
10.1002/cphc.201000231
IDS Number:
648JZ
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