Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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AU Gong, XJ
Li, JY
Zhang, H
Wan, RZ
Lu, HJ
Wang, S
Fang, HP
AF Gong, Xiaojing
Li, Jingyuan
Zhang, He
Wan, Rongzheng
Lu, Hangjun
Wang, Shen
Fang, Haiping
TI Enhancement of Water Permeation across a Nanochannel by the Structure
outside the Channel
SO PHYSICAL REVIEW LETTERS
LA English
DT Article
ID CARBON NANOTUBES; MASS-TRANSPORT; AQUAPORIN-1; CONDUCTION; MEMBRANES;
MOLECULES; MECHANISM; DYNAMICS; FUTURE
AB We used molecular dynamics simulation to study the effect of the
external structure on water permeation across a single-walled
nanochannel. In contrast with the macroscopic scenario, the outside
structure greatly affects the water transport across the nanochannel.
Remarkably, the ratio of maximal to minimal flux reached a value of
about two for different outside structures. These findings are expected
to be helpful in design of high-flux nanochannels and provide an
insight into the contribution of the lipid membrane to water permeation
across biological water channels.
C1 [Gong, Xiaojing; Li, Jingyuan; Wan, Rongzheng; Wang, Shen; Fang, Haiping] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China.
[Gong, Xiaojing] Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion, Suzhou 215125, Peoples R China.
[Gong, Xiaojing; Wang, Shen] Chinese Acad Sci, Grad Sch, Beijing 100080, Peoples R China.
[Zhang, He] Shanghai Jiao Tong Univ, Dept Biol, Shanghai 200240, Peoples R China.
[Lu, Hangjun] Zhejiang Normal Univ, Dept Phys, Jinhua 321004, Peoples R China.
RP Gong, XJ, Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800,
Peoples R China.
EM fanghaiping@sinap.ac.cn
CR *EPAPS, EPRLTAO101079850 EPA
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NR 34
TC 0
PU AMER PHYSICAL SOC; ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0031-9007
DI 10.1103/PhysRevLett.101.257801
PD DEC 19
PY 2008
VL 101
IS 25
AR 257801
SC Physics, Multidisciplinary
GA 386NZ
UT ISI:000261891200072
ER
PT J
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AU Goldsmith, J
Martens, CC
AF Goldsmith, Jacob
Martens, Craig C.
TI Pressure-induced water flow through model nanopores
SO PHYSICAL CHEMISTRY CHEMICAL PHYSICS
LA English
DT Article
ID MOLECULAR-DYNAMICS; CARBON NANOTUBES; TRANSPORT; DIFFUSION; SURFACES
AB This paper describes nonequilibrium molecular dynamics simulations of
pressure induced transport of liquid water through model nanopores. We
consider a simple model for a porous membrane consisting of a slab of
water molecules held in a rigid ice structure and penetrated by a pore
of nanometer scale dimensions. Both hydrophilic membranes composed of
conventional TIP3P water and hydrophobic membranes consisting of
modified water with the model partial charges set to zero are treated.
Molecular dynamics simulation is employed to investigate the rate of
water flow through the pore induced by a pressure difference across the
membrane. The results are compared with the predictions of continuum
hydrodynamics. We find that the flow rate of water through hydrophilic
pores is much less than the continuum predictions, while the flux
through hydrophobic pores can significantly exceed the continuum
theory. Finally, we show asymmetric behavior in the flux vs. pressure
difference for a conical nanopore, which thus acts as a Brownian
ratchet.
C1 [Goldsmith, Jacob; Martens, Craig C.] Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.
RP Martens, CC, Univ Calif Irvine, Dept Chem, Irvine, CA 92697 USA.
EM cmartens@uci.edu
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NR 31
TC 0
PU ROYAL SOC CHEMISTRY; THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD,
CAMBRIDGE CB4 0WF, CAMBS,
ENGLAND
SN 1463-9076
DI 10.1039/b807823h
PY 2009
VL 11
IS 3
BP 528
EP 533
SC Chemistry, Physical; Physics, Atomic, Molecular & Chemical
GA 388FZ
UT ISI:000262007000010
ER
PT S
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AU Alexeeva, OK
Chelyak, MM
Kotenko, AA
Shapir, BL
Nechaev, YS
AF Alexeeva, O. K.
Chelyak, M. M.
Kotenko, A. A.
Shapir, B. L.
Nechaev, Yu. S.
TI CREATION OF NEW COMPOSITE MATERIALS FOR HYDROGEN ENERGY PURPOSES. I.
NEW LINES OF MEMBRANE PRODUCTION TECHNOLOGY
SO CARBON NANOMATERIALS IN CLEAN ENERGY HYDROGEN SYSTEMS
LA English
DT Proceedings Paper
DE hydrogen energy; carbon; nanostructures; membranes; composite materials
ID NANOPOROUS CARBON MEMBRANES; MOLECULAR-SIEVE MEMBRANES; TRANSPORT;
NANOTUBES; SEPARATION; NANOSTRUCTURES
AB One of the main problems of hydrogen energy is separation and
purification of hydrogen produced by various conversion methods from
raw hydrocarbons. Carbon membranes can become real alternative both to
inorganic and polymeric ones and enlarge possibilities of membrane
methods of gas separation. Investigations aimed at the creation of
composite carbon membranes suitable for operation at high temperatures
in the presence of organic vapors, in acid or alkaline (non-oxidizing)
medium are presented. Our approach is based on the carbonization of
polymeric layers on the porous inorganic high temperature supports with
definite structure which opens up new possibilities for carbon
nanostructure production. Main trends of future developments of
composite carbon gas separation and filtration membranes are also
discussed.
C1 [Alexeeva, O. K.; Chelyak, M. M.; Kotenko, A. A.; Shapir, B. L.] Russian Res Ctr, Kurchatov Inst, Hydrogen Energy & Plasma Technol Inst, Moscow 123182, Russia.
RP Alexeeva, OK, Russian Res Ctr, Kurchatov Inst, Hydrogen Energy & Plasma
Technol Inst, Kurchatov Sq 1, Moscow 123182, Russia.
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NR 27
TC 0
PU SPRINGER; PO BOX 17, 3300 AA DORDRECHT, NETHERLANDS
SN 1871-4668
PY 2008
BP 255
EP 262
GA BIQ05
UT ISI:000261798800026
ER
EF
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