Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
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Title:
Thermodynamic Analysis for Synthesis of Advanced Materials
Authors:
Liu, C; Ji, Y; Shao, Q; Feng, X; Lu, X
Author Full Names:
Liu, C.; Ji, Y.; Shao, Q.; Feng, X.; Lu, X.
Source:
MOLECULAR THERODYNAMICS OF COMPLEX SYSTEMS 131: 193-270 2009
Language:
English
Document Type:
Review
Author Keywords:
Advanced materials; Electrolyte; Interface; Molecular simulation; Thermodynamics
Keywords Plus:
WALLED CARBON NANOTUBES; POTASSIUM-SULFATE CRYSTALS; ACTIVITY-COEFFICIENTS; DISSOLUTION KINETICS; SUPERCRITICAL WATER; AQUEOUS-SOLUTIONS; LOW-TEMPERATURE; ION-EXCHANGE; LIQUID WATER; STRUCTURAL-CHARACTERIZATION
Abstract:
In this paper, thermodynamic modeling for materials-oriented chemical engineering systems were investigated in order to solve critical scientific problems, such as the material structure, chemical properties, thermodynamic properties, and transfer behaviors on the interfaces or under confined circumstances. On the basis of the theory and approaches of chemical engineering, and the principles of chemical engineering thermodynamics and transfer processes, molecular simulations were combined with modern physical characterization methods to study thermodynamic modeling in materials-oriented chemical engineering processes.
Reprint Address:
Lu, X, Nanjing Univ Technol, Coll Chem & Chem Engn, State Key Lab Mat Oriented Chem Engn, Nanjing 210009, Peoples R China.
Research Institution addresses:
[Liu, C.; Ji, Y.; Shao, Q.; Feng, X.; Lu, X.] Nanjing Univ Technol, Coll Chem & Chem Engn, State Key Lab Mat Oriented Chem Engn, Nanjing 210009, Peoples R China
E-mail Address:
xhlu@njut.edu.cn
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Times Cited:
0
Publisher:
SPRINGER-VERLAG BERLIN; HEIDELBERGER PLATZ 3, D-14197 BERLIN, GERMANY
ISSN:
0081-5993
DOI:
10.1007/430_2008_4
IDS Number:
BIR94
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Title:
THz Investigations of Condensed Phase Blomolecular Systems
Authors:
Zhang, HL; Siegrist, K; Douglas, KO; Gregurick, SK; Plusquellic, DF
Author Full Names:
Zhang, Hailiang; Siegrist, Karen; Douglas, Kevin O.; Gregurick, Susan K.; Plusquellic, David F.
Source:
METHODS IN NANO CELL BIOLOGY 90: 417-+ 2008
Language:
English
Document Type:
Review
Keywords Plus:
TERAHERTZ SPECTROSCOPY; VIBRATIONAL-MODES; AB-INITIO; WATER; DYNAMICS; MOLECULES; PROTEIN; PORES; FIELD; IONS
Abstract:
Terahertz (THz) spectroscopic investigations of crystalline dipeptide nanotubes are discussed in the frequency region from 0.6 (2 cm(-1)) to 3 THz (100 cm(-1)). The THz region provides access to collective modes of biomolecular systems and is therefore sensitive to the large scale motions important for understanding the impact of environmental stimuli in biomolecular systems. The focus of this chapter is on THz spectral changes observed in this region when crystals of alanyl isoleucine (AI) and isoleucyl alanine (IA) nanotubes are exposed to water. Of biological significance is the water permeability through hydrophobic pore regions as exemplified in the disparate behavior of these two dipeptide nanotubes. AI is known from X-ray studies and confirmed here to act reversibly to the exchange of water while IA does not accept water into its pore region. Both quantum chemical and classical calculations are performed to better understand the subtle balance that determines guest mo!
lecule absorption and conduction through these hydrophobic channels. Examination of the vibrational character of the THz modes with and without water suggests water mode coupling/decoupling with collective modes of the nanotube may play an important role in the permeability dynamics.
Reprint Address:
Zhang, HL, Univ Maryland Baltimore Cty, Dept Chem & Biochem, Baltimore, MD 21250 USA.
Research Institution addresses:
[Zhang, Hailiang; Douglas, Kevin O.] Univ Maryland Baltimore Cty, Dept Chem & Biochem, Baltimore, MD 21250 USA; [Siegrist, Karen] Johns Hopkins Appl Phys Lab, Electroopt & Infrared Syst & Technol Grp, Laurel, MD 20723 USA; [Douglas, Kevin O.; Plusquellic, David F.] NIST, Phys Lab, Biophys Grp, Gaithersburg, MD 20899 USA
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42
Times Cited:
0
Publisher:
ELSEVIER ACADEMIC PRESS INC; 525 B STREET, SUITE 1900, SAN DIEGO, CA 92101-4495 USA
ISSN:
0091-679X
DOI:
10.1016/S0091-679X(08)00818-2
IDS Number:
BIR53
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Title:
Effective viscosity of glycerin in a nanoporous silica gel
Authors:
Han, AJ; Lu, WY; Punyamurtula, VK; Chen, X; Surani, FB; Kim, T; Qiao, Y
Author Full Names:
Han, Aijie; Lu, Weiyi; Punyamurtula, Venkata K.; Chen, Xi; Surani, Falgun B.; Kim, Taewan; Qiao, Yu
Source:
JOURNAL OF APPLIED PHYSICS 104 (12): Art. No. 124908 DEC 15 2008
Language:
English
Document Type:
Article
Author Keywords:
gels; nanoporous materials; organic compounds; silicon compounds; surface tension; viscosity
Keywords Plus:
CARBON NANOTUBE; WATER; INFILTRATION; PRESSURE; CHANNEL
Abstract:
The infiltration of glycerin in a lyophobic nanoporous silica gel is investigated experimentally, and the effective interfacial tension and viscosity are discussed. While the simple superposition principle can be employed for the analysis of interfacial tension, in a nanopore the effective liquid viscosity is no longer a material constant. It is highly dependent on the pore size and the loading rate, much smaller than its bulk counterpart.
Reprint Address:
Han, AJ, Univ Calif San Diego, Dept Struct Engn, La Jolla, CA 92093 USA.
Research Institution addresses:
[Han, Aijie; Lu, Weiyi; Punyamurtula, Venkata K.; Qiao, Yu] Univ Calif San Diego, Dept Struct Engn, La Jolla, CA 92093 USA; [Kim, Taewan; Qiao, Yu] Univ Calif San Diego, Program Mat Sci & Engn, La Jolla, CA 92093 USA; [Surani, Falgun B.] Univ Akron, Dept Civil Engn, Akron, OH 44325 USA; [Chen, Xi] Columbia Univ, Dept Civil Engn & Engn Mech, New York, NY 10027 USA
E-mail Address:
yqiao@ucsd.edu
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22
Times Cited:
0
Publisher:
AMER INST PHYSICS; CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA
Subject Category:
Physics, Applied
ISSN:
0021-8979
DOI:
10.1063/1.3020535
IDS Number:
391HT
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Title:
Enhanced Polymer Melts Flow though Nanoscale Channels under Vibration
Authors:
Kong, J; Xu, Y; Yung, KL; Xie, YC; He, L
Author Full Names:
Kong, Jie; Xu, Yan; Yung, Kai-Leung; Xie, Yunchuan; He, Lan
Source:
JOURNAL OF PHYSICAL CHEMISTRY C 113 (2): 624-629 JAN 15 2009
Language:
English
Document Type:
Article
Keywords Plus:
MOLECULAR-DYNAMICS SIMULATION; WALLED CARBON NANOTUBES; WATER; NANOCHANNELS; BEHAVIOR; NANOCRYSTALS; CAPILLARIES; CONDUCTION; NANOFIBERS; INTERFACE
Abstract:
The enhanced poly(epsilon-caprolactone) melts flow behaviors though nanoscale channels under vibration were observed. The effect of vibration on the nanoflow is dependent on the vibration frequency of piezoelectric transducer that generates the vibration fields. The flow rate of poly(epsilon-caprolactone) melts in nanochannels increases with the increase of vibration frequency within the range from 2.0 to 14.0 kHz. The observed enhanced flow through nanochannels under vibration is a new nanoscale phenomenon, which is potential in vibration-assisted nanofluidic, nanoimprint lithography, and micro-/nanoinjection molding etc.
Reprint Address:
Kong, J, Hong Kong Polytech Univ, Dept Ind & Syst Engn, Kowloon, Hong Kong, Peoples R China.
Research Institution addresses:
[Kong, Jie; Xu, Yan; Yung, Kai-Leung; Xie, Yunchuan; He, Lan] Hong Kong Polytech Univ, Dept Ind & Syst Engn, Kowloon, Hong Kong, Peoples R China; [Kong, Jie] NW Polytech Univ, Sch Sci, Dept Appl Chem, Xian 710072, Peoples R China
E-mail Address:
mfkongjie@hotmail.com
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Cited Reference Count:
44
Times Cited:
0
Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Subject Category:
Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
ISSN:
1932-7447
DOI:
10.1021/jp809164k
IDS Number:
392TH
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Title:
Bidirectional Transport of Guest Molecules through the Nanoporous Tunnel Structure of a Solid Inclusion Compound
Authors:
Marti-Rujas, J; Desmedt, A; Harris, KDM; Guillaume, F
Author Full Names:
Marti-Rujas, Javier; Desmedt, Arnaud; Harris, Kenneth D. M.; Guillaume, Francois
Source:
JOURNAL OF PHYSICAL CHEMISTRY C 113 (2): 736-743 JAN 15 2009
Language:
English
Document Type:
Article
Keywords Plus:
CONFOCAL RAMAN MICROSPECTROMETRY; ELASTIC NEUTRON-SCATTERING; CARBON NANOTUBE MEMBRANES; AQUAPORIN WATER CHANNELS; SELECTIVE ION CONDUCTION; POTASSIUM CHANNELS; SELF-DIFFUSION; NOBEL LECTURE; ATOMIC BASIS; UREA
Abstract:
Confocal Raman microspectrometry is used to probe, for the first time, the transport of guest molecules along the one-dimensional tunnels in a crystalline urea inclusion compound under conditions of guest exchange in which new guest molecules are introduced simultaneously at both ends of the urea tunnel structure. We focus on the system comprising 1,8-dibromooctane as the original type of guest and pentadecane as the new type of guest, and results are presented for experiments in which the guest exchange process is probed both ex situ and in situ. The Raman data, recorded as a function of position along the tunnel direction and, in the case of the in situ experiments, as a function of time, demonstrate that pentadecane guest molecules enter the tunnels at both ends of the crystal and that transport of guest molecules occurs in both directions along the crystal. Mechanistic aspects of this bidirectional transport process are discussed, particularly in relation to the correspo!
nding process for unidirectional transport of guest molecules in urea inclusion compounds reported previously.
Reprint Address:
Harris, KDM, Cardiff Univ, Sch Chem, Pk Pl, Cardiff CF10 3AT, S Glam, Wales.
Research Institution addresses:
[Marti-Rujas, Javier; Harris, Kenneth D. M.] Cardiff Univ, Sch Chem, Cardiff CF10 3AT, S Glam, Wales; [Desmedt, Arnaud; Guillaume, Francois] Univ Bordeaux, UMR 5255, ISM, Grp Spect Mol, F-33405 Talence, France
E-mail Address:
harriskdm@cardiff.ac.uk; f.guillaume@ism.u-bordeauxl.fr
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53
Times Cited:
0
Publisher:
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Subject Category:
Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
ISSN:
1932-7447
DOI:
10.1021/jp806380p
IDS Number:
392TH
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