Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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AU Rossi, MP
Gogotsi, Y
Kornev, KG
AF Rossi, Maria Pia
Gogotsi, Yury
Kornev, Konstantin G.
TI Deformation of Carbon Nanotubes by Exposure to Water Vapor
SO LANGMUIR
LA English
DT Article
ID SCANNING-ELECTRON-MICROSCOPY; DER-WAALS FORCES; CAPILLARY CONDENSATION;
KELVIN EQUATION; YOUNGS MODULUS; NANOPIPES; RINGS; FILMS; TRANSPORT;
SORBENTS
AB The condensation of water inside multiwalled carbon nanotubes has been
monitored and controlled using environmental scanning electron
microscopy. Undersaturated vapor condenses inside nanotubes and forms
nanometer-thick water films. Simultaneously, nanotubes deform and
decrease their apparent diameter. When the vapor pressure in the
chamber approaches the saturation pressure, we observe the formation of
menisci and spontaneous buckling of the nanotubes. We derive a
criterion of the buckling instability caused by capillary condensation.
Remarkably, the buckling criterion appears to be independent of the
meniscus shape. Using our experiments and models, we estimated the
circumferential Young's modulus of large-diameter carbon nanotubes with
disordered wall structure produced by the chemical vapor deposition
method (CVD) to be E-theta theta approximate to 13-18 MPa. It appears
to be at least 2 orders of magnitude lower than the longitudinal
modulus of nanotubes produced by arc discharge or catalytic CVD
methods. The reported experiments and proposed theory suggest possible
applications of "soft" nanotubes as sensors to probe minute
concentrations of absorbable gases and vapors.
C1 [Kornev, Konstantin G.] Clemson Univ, Sch Mat Sci & Engn, Clemson, SC 29634 USA.
[Rossi, Maria Pia; Gogotsi, Yury] Drexel Univ, Dept Mat Sci & Engn, Philadelphia, PA 19104 USA.
[Rossi, Maria Pia; Gogotsi, Yury] Drexel Univ, AJ Drexel Nanotechnol Inst, Philadelphia, PA 19104 USA.
RP Kornev, KG, Clemson Univ, Sch Mat Sci & Engn, 161 Sirrine Hall,
Clemson, SC 29634 USA.
EM kkornev@clemson.edu
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NR 60
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0743-7463
DI 10.1021/la802684q
PD MAR 3
VL 25
IS 5
BP 2804
EP 2810
SC Chemistry, Physical
GA 413CP
UT ISI:000263770800041
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PT J
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AU Zeng, L
Guo, HK
Zuo, GH
Wan, RZ
Fang, HP
AF Zeng Li
Guo Hong-Kai
Zuo Guang-Hong
Wan Rong-Zheng
Fang Hai-Ping
TI Water Transport through Multinanopores Membranes
SO CHINESE PHYSICS LETTERS
LA English
DT Article
ID WALLED CARBON NANOTUBES; MASS-TRANSPORT; LIQUID WATER; CHANNEL;
PERMEATION; MICROFLUIDICS; DIFFUSION; MODEL; FLOW
AB We investigate the influence of correlation between water molecules
transport through the neighbouring nanopores, whose centres are at a
distance of only 6.2 angstrom, using the molecular dynamics
simulations. Water molecule distribution in nanopore and average water
flow are obtained. It is found that the average water molecule number
and water flow are slightly different between a system made of the
neighbouring nanopores and a system of a single pore. This indicates
that transport of water chains in neighbouring pores do no show
significant influence each other. These findings should be helpful in
designing efficient artificial membrane made of nanopores and providing
an insight into effects of the biological channel structure on the
water permeation.
C1 [Zeng Li; Wan Rong-Zheng; Fang Hai-Ping] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China.
[Zeng Li] Chinese Acad Sci, Grad Sch, Beijing 100049, Peoples R China.
[Guo Hong-Kai] Shijiazhuang Railway Inst, Shijiazhuang 050043, Peoples R China.
[Zuo Guang-Hong] Fudan Univ, Dept Phys, T Life Res Ctr, Shanghai 200433, Peoples R China.
[Fang Hai-Ping] Chinese Acad Sci, TPCSF, Beijing 100049, Peoples R China.
RP Wan, RZ, Chinese Acad Sci, Shanghai Inst Appl Phys, POB 800-204,
Shanghai 201800, Peoples R China.
EM wanrongzheng@sinap.ac.cn
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PU IOP PUBLISHING LTD; DIRAC HOUSE, TEMPLE BACK, BRISTOL BS1 6BE, ENGLAND
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AR 038701
SC Physics, Multidisciplinary
GA 410TN
UT ISI:000263601300083
ER
PT J
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AU Worsley, MA
Kucheyev, SO
Satcher, JH
Hamza, AV
Baumann, TF
AF Worsley, Marcus A.
Kucheyev, Sergei O.
Satcher, Joe H., Jr.
Hamza, Alex V.
Baumann, Theodore F.
TI Mechanically robust and electrically conductive carbon nanotube foams
SO APPLIED PHYSICS LETTERS
LA English
DT Article
DE carbon nanotubes; elasticity; electrical conductivity; foams;
nanofabrication; nanoparticles; nanoporous materials
ID ORGANIC AEROGELS; FILMS; TRANSPARENT
AB We describe the fabrication of ultralow-density carbon nanotube (CNT)
foams that simultaneously exhibit high electrical conductivities and
robust mechanical properties. Our approach utilizes carbon
nanoparticles as a binder to crosslink randomly oriented bundles of
single-walled CNTs. The resulting CNT foams are the stiffest
low-density nanoporous solids reported and exhibit elastic behavior up
to strains as large as similar to 80%. The use of the carbon binder
also allows bulk electrical conductivity to be maintained at low
densities.
C1 [Worsley, Marcus A.; Kucheyev, Sergei O.; Satcher, Joe H., Jr.; Hamza, Alex V.; Baumann, Theodore F.] Lawrence Livermore Natl Lab, Phys & Life Sci Directorate, Livermore, CA 94550 USA.
RP Worsley, MA, Lawrence Livermore Natl Lab, Phys & Life Sci Directorate,
Livermore, CA 94550 USA.
EM baumann2@llnl.gov
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NR 26
TC 0
PU AMER INST PHYSICS; CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON
QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0003-6951
DI 10.1063/1.3086293
PD FEB 16
VL 94
IS 7
AR 073115
SC Physics, Applied
GA 410SS
UT ISI:000263599200071
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