Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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Number of Citing Articles: 2 new records this week (2 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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AU Qiao, Y
Liu, L
Chen, X
AF Qiao, Yu
Liu, Ling
Chen, Xi
TI Pressurized Liquid in Nanopores: A Modified Laplace-Young Equation
SO NANO LETTERS
LA English
DT Article
ID CARBON NANOTUBES; WATER; TRANSPORT; INFILTRATION; BEHAVIORS; FIELD; FLOW
AB In the current study, we analyze the motion of pressurized water
molecules in nanopores of a well-crystallized, hydrophobic zeolite
using both experiment and molecular dynamics simulation. It is
discovered that, contradictory to the prediction of the classic
Laplace-Young equation, the required infiltration pressure is highly
dependent on the infiltration volume. A modified Laplace-Young equation
is developed to take into consideration the effective solid-liquid
interfacial tension, the thermal energy exchange, as well as the
variation in configuration of confined liquid molecules. The last two
factors are significant only when the nanopore diameter is comparable
with the liquid molecule size. It is also remarkable that the
infiltrated liquid molecules, when confined in the nanoenvironment,
could transform from a single-chain conformation to a double-helical
structure as the pressure increases, accompanied by an abrupt system
free energy change that leads to different pressure-induced transport
behaviors.
C1 [Liu, Ling; Chen, Xi] Columbia Univ, Dept Civil Engn & Engn Mech, New York, NY 10027 USA.
[Qiao, Yu] Univ Calif San Diego, Dept Struct Engn, La Jolla, CA 92093 USA.
RP Chen, X, Columbia Univ, Dept Civil Engn & Engn Mech, New York, NY 10027
USA.
EM xichen@civil.columbia.edu
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NR 34
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
DI 10.1021/nl8030136
PD MAR
VL 9
IS 3
BP 984
EP 988
SC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary
GA 418IO
UT ISI:000264142100013
ER
PT J
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AU Shao, Q
Zhou, J
Lu, LH
Lu, XH
Zhu, YD
Jiang, SY
AF Shao, Qing
Zhou, Jian
Lu, Linghong
Lu, Xiaohua
Zhu, Yudan
Jiang, Shaoyi
TI Anomalous Hydration Shell Order of Na+ and K+ inside Carbon Nanotubes
SO NANO LETTERS
LA English
DT Article
ID MOLECULAR-DYNAMICS SIMULATIONS; SELECTIVE ION CONDUCTION; POTASSIUM
CHANNELS; MASS-TRANSPORT; GAS-TRANSPORT; ATOMIC BASIS; WATER;
MEMBRANES; TEMPERATURE; NANOPORES
AB We performed molecular dynamics simulations of the hydration of Na+ and
K+ in infinitely long single-walled armchair carbon nanotubes (CNTs) at
298 K. Simulation results Indicate that the preferential orientation of
water molecules in coordination shells of these two cations presents an
anomalous change In the CNTs and causes a diameter-dependent variation
for the interaction energy between the cation and water molecules In
Its coordination shell. In the five CNTs of this work, it is
energetically favorable for confining a hydrated K+ inside the two
narrow CNTs with diameters of 0.60 and 0.73 nm, whereas the situation
is reverse inside the wide CNTs with diameters of 0.87, 1.0, and 1.28
nm. This finding is Important for CNT applications in ionic systems
that control the selectivity and the Ionic flow.
C1 [Shao, Qing; Lu, Linghong; Lu, Xiaohua; Zhu, Yudan] Nanjing Univ Technol, State Key Lab Mat Oriented Chem Engn, Nanjing 210009, Peoples R China.
[Zhou, Jian] S China Univ Technol, Sch Chem & Chem Engn, Ghangzhou 510640, Peoples R China.
[Jiang, Shaoyi] Univ Washington, Dept Chem Engn, Seattle, WA 98195 USA.
RP Lu, XH, Nanjing Univ Technol, State Key Lab Mat Oriented Chem Engn,
Nanjing 210009, Peoples R China.
EM xhlu@njut.edu.cn
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NR 41
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
DI 10.1021/nl803044k
PD MAR
VL 9
IS 3
BP 989
EP 994
SC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary
GA 418IO
UT ISI:000264142100014
ER
EF
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