Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
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Title:
Noble metal nanoparticles for water purification: A critical review
Authors:
Pradeep, T; Anshup
Author Full Names:
Pradeep, T.; Anshup
Source:
THIN SOLID FILMS 517 (24): 6441-6478 OCT 30 2009
Language:
English
Document Type:
Review
Author Keywords:
Water purification; Nanotechnology; Noble metals; Nanoparticles; Pesticides; Heavy metal ions; Micro-organisms; Drinking water
KeyWords Plus:
SURFACE-ENHANCED RAMAN; FUNCTIONALIZED GOLD NANOPARTICLES; COLLOIDAL SILVER NANOPARTICLES; FUNDAMENTAL-STUDIES RANKING; SELF-ASSEMBLED MONOLAYERS; CORE-SHELL NANOPARTICLES; OPTICAL-PROPERTIES; COLORIMETRIC DETECTION; NANOCLUSTER FORMATION; ESCHERICHIA-COLI
Abstract:
Water is one of the essential enablers of life on earth. Beginning with the origin of the earliest form of life in seawater, it has been central to the evolution of human civilizations. Noble metals have been similarly associated with the prosperity of human civilizations through their prominent use in jewellery and medical applications. The most important reason for the use of noble metals is the minimal reactivity at the bulk scale, which can be explained by a number of concepts such as electrochemical potential, relativisitic contraction, molecular orbital theory, etc. Recently, water quality has been associated with the development index of society. A number of chemical and biological contaminants have endangered the quality of drinking water. An overview of important events during last 200 years in the area of drinking water purification is presented. Realizing the molecular nature of contamination in drinking water, significant progress has been made to utilize the che!
mistry of nanomaterials for water purification. This article summarizes recent efforts in the area of noble metal nanoparticle synthesis and the origin of their reactivity at the nanoscale. The application of noble metal nanoparticle based chemistry for drinking water purification is summarized for three major types of contaminants: halogenated organics including pesticides, heavy metals and microorganisms. Recent efforts for the removal, as well as ultralow concentration detection of such species, using noble metal nanoparticles are summarized. important challenges during the commercialization of nano-based products are highlighted through a case study of pesticide removal using noble metal nanoparticles. Recent efforts in drinking water purification using other forms of nanomaterials are also summarized. The article concludes with recent investigations on the issue of nanotoxicity and its implications for the future. (C) 2009 Elsevier B.V. All rights reserved.
Reprint Address:
Pradeep, T, Indian Inst Technol, Dept Chem, Madras 600036, Tamil Nadu, India.
Research Institution addresses:
[Pradeep, T.] Indian Inst Technol, Dept Chem, Madras 600036, Tamil Nadu, India; Indian Inst Technol, Sophisticated Analyt Instrument Facil, Madras 600036, Tamil Nadu, India
E-mail Address:
pradeep@iitm.ac.in
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Cited Reference Count:
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Times Cited:
0
Publisher:
ELSEVIER SCIENCE SA; PO BOX 564, 1001 LAUSANNE, SWITZERLAND
Subject Category:
Materials Science, Multidisciplinary; Materials Science, Coatings & Films; Physics, Applied; Physics, Condensed Matter
ISSN:
0040-6090
DOI:
10.1016/j.tsf.2009.03.195
IDS Number:
501VI
========================================================================
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Title:
Theory of single-file multiparticle diffusion in narrow pores
Authors:
Kharkyanen, VN; Yesylevskyy, SO
Author Full Names:
Kharkyanen, Valery N.; Yesylevskyy, Semen O.
Source:
PHYSICAL REVIEW E 80 (3): Art. No. 031118 Part 1 SEP 2009
Language:
English
Document Type:
Article
KeyWords Plus:
ION CHANNELS; BROWNIAN DYNAMICS; MOLECULAR-DYNAMICS; POTASSIUM CHANNEL; BIOLOGICAL-MEMBRANES; SELECTIVITY FILTER; CONTINUUM-THEORIES; K+ CHANNEL; CONDUCTION; PERMEATION
Abstract:
Single-file diffusion of multiple strongly interacting particles in a one-dimensional pore is described within a general analytical framework. The theory accounts for nonequilibrium conditions, explicit particle-particle interactions, external potential acting on the particles and the fluctuations of the number of particles due to their exchange with external equilibrium reservoirs. It is shown that the problem can be reduced to a closed hierarchical set of partial differential equations of increasing dimensionality, which can be solved numerically. Our framework allows computing any macroscopic characteristic of multiparticle diffusion in the pore. It is shown that the pore occupancy probabilities and the current are rational functions of external concentrations in the steady state. The theory is tested on a simplified model of the narrow rigid pore inspired by the selectivity filter of biological ion channel. Perspectives and limitations of the theory are discussed.
Reprint Address:
Kharkyanen, VN, Natl Acad Sci Ukraine, Inst Phys, Dept Phys Biol Syst, Prospect Nauki 46, UA-03039 Kiev, Ukraine.
Research Institution addresses:
[Kharkyanen, Valery N.; Yesylevskyy, Semen O.] Natl Acad Sci Ukraine, Inst Phys, Dept Phys Biol Syst, UA-03039 Kiev, Ukraine
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Times Cited:
0
Publisher:
AMER PHYSICAL SOC; ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
Subject Category:
Physics, Fluids & Plasmas; Physics, Mathematical
ISSN:
1539-3755
DOI:
10.1103/PhysRevE.80.031118
IDS Number:
501LM
========================================================================
*Record 3 of 6.
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Title:
Induced beta-Barrel Formation of the Alzheimer's A beta 25-35 Oligomers on Carbon Nanotube Surfaces: Implication for Amyloid Fibril Inhibition
Authors:
Fu, ZM; Luo, Y; Derreumaux, P; Wei, GH
Author Full Names:
Fu, Zhaoming; Luo, Yin; Derreumaux, Philippe; Wei, Guanghong
Source:
BIOPHYSICAL JOURNAL 97 (6): 1795-1803 SEP 16 2009
Language:
English
Document Type:
Article
KeyWords Plus:
ATOMIC-FORCE MICROSCOPY; MOLECULAR-DYNAMICS; PROTEIN FIBRILLATION; PEPTIDE AGGREGATION; SIMULATIONS; MECHANISM; WATER; NANOPARTICLES; CHAPERONES; FULLERENE
Abstract:
Recent experimental studies show that carbon nanotubes; impact the aggregation process of proteins associated with neurodegenerative diseases. However, the details of molecular interactions between proteins and carbon nanotubes are still not well understood. In this study, we investigate the initial adsorption features and dynamics of the Alzheimer's amyloid-beta peptide spanning residues 25-35 (A beta 25-35) on a single-walled carbon nanotube (SWNT) surface using fully atomic molecular dynamics simulations (MD) in explicit solvent. The initial configurations of the A beta 25-35 peptides consist of two preformed bilayer beta-sheets, each with four or five beta-strands in parallel or mixed antiparallel-parallel orientations. Our simulations show, for what we believe is the first time, that two disjointed A beta 25-35 beta-sheets with mixed antiparallel-parallel strands can assemble into beta-barrels wrapping the SWNT. In contrast, both simulations of A beta 25-35 without SWNT!
, and simulations of SWNT-A beta 25-35 with purely parallel beta-strands, lead to disordered aggregates. We find that A beta 25-35 beta-barrel formation involves at least two steps: i), curving of the A beta 25-35 beta-sheets as a result of strong hydrophobic interactions with carbon nanotube concomitantly with dehydration of the SWNT-peptide interface; and ii), intersheet backbone hydrogen bond formation with fluctuating intrasheet hydrogen bonds, Detailed analysis of the conversion shows that beta-barrel formation on SWNT surface results from the interplay of dehydration and peptide-SWNT/peptide-peptide interactions. Implications of our results on amyloid fibril inhibition are discussed.
Reprint Address:
Wei, GH, Fudan Univ, Surface Phys Lab, Natl Key Lab, Shanghai 200433, Peoples R China.
Research Institution addresses:
[Fu, Zhaoming; Luo, Yin; Wei, Guanghong] Fudan Univ, Surface Phys Lab, Natl Key Lab, Shanghai 200433, Peoples R China; [Fu, Zhaoming; Luo, Yin; Wei, Guanghong] Fudan Univ, Dept Phys, Shanghai 200433, Peoples R China; [Derreumaux, Philippe] Inst Biol Physicochim, CNRS, UPR 9080, Lab Biochim Theor, F-75005 Paris, France; [Derreumaux, Philippe] Univ Paris 07, Paris, France
E-mail Address:
ghwei@fudan.edu.cn
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49
Times Cited:
0
Publisher:
CELL PRESS; 600 TECHNOLOGY SQUARE, 5TH FLOOR, CAMBRIDGE, MA 02139 USA
Subject Category:
Biophysics
ISSN:
0006-3495
DOI:
10.1016/j.bpj.2009.07.014
IDS Number:
501KO
========================================================================
*Record 4 of 6.
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Title:
Noncoaxial vibration of fluid-filled multi-walled carbon nanotubes
Authors:
Yan, Y; Wang, WQ; Zhang, L
Author Full Names:
Yan, Y.; Wang, W. Q.; Zhang, Lx
Source:
APPLIED MATHEMATICAL MODELLING 34 (1): 122-128 JAN 2010
Language:
English
Document Type:
Article
Author Keywords:
Fluid-filled multi-walled carbon nanotubes; Natural resonant frequency; Intertube resonant frequency; Amplitude ratio; Noncoaxial vibration
KeyWords Plus:
CONVEYING FLUID; CYLINDRICAL-SHELLS; INSTABILITY; FLOW
Abstract:
This paper is concerned with the free vibration of the fluid-filled multi-walled carbon nanotubes (MWCNTs) with simply supported ends. Based on simplified Donnell's cylindrical shell model and potential flow theory, the effect of internal fluid on the coupling vibration of the MWCNTs-fluid system is discussed in detail. The results show that the resonant frequencies are decreased due to the effect of the fluid, and the fluid has only a little influence on the associated amplitude ratio in MWCNTs corresponding to the natural resonant frequency (frequency of the innermost tube), while plays a significant role in the associated amplitude ratios corresponding to the intertube resonant frequency. For the natural resonant frequency, the vibration mode is coaxial. However, for the intertube resonant frequency, the system shows complex noncoaxial vibration, which plays a critical role in electronic and transport properties of carbon nanotubes (CNTs). (C) 2009 Elsevier Inc. All right!
s reserved.
Reprint Address:
Wang, WQ, Kunming Univ Sci & Technol, Dept Engn Mech, 50 E Ring Rd, Kunming 650051, Peoples R China.
Research Institution addresses:
[Yan, Y.; Wang, W. Q.; Zhang, Lx] Kunming Univ Sci & Technol, Dept Engn Mech, Kunming 650051, Peoples R China
E-mail Address:
yanyankm@126.com; wwqquan@126.com; zlxzcc@126.com
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29
Times Cited:
0
Publisher:
ELSEVIER SCIENCE INC; 360 PARK AVE SOUTH, NEW YORK, NY 10010-1710 USA
Subject Category:
Engineering, Multidisciplinary; Mathematics, Interdisciplinary Applications; Mechanics
ISSN:
0307-904X
DOI:
10.1016/j.apm.2009.03.031
IDS Number:
500QL
========================================================================
*Record 5 of 6.
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Title:
Carbon Nanotubes and Nanofluidic Transport
Authors:
Holt, JK
Author Full Names:
Holt, Jason Knowles
Source:
ADVANCED MATERIALS 21 (35): 3542-3550 SEP 18 2009
Language:
English
Document Type:
Article
KeyWords Plus:
WATER TRANSPORT; GAS-TRANSPORT; LIQUID SLIP; MEMBRANES; FLOW; MOLECULES; CHANNEL; IONS
Abstract:
Recent strides have been made in both the modeling and measurement of fluid flow on the nanoscale. Carbon nanotubes, with their atomic dimensions and atomic smoothness, are ideal materials for studying such flow. This Progress Report describes recent modeling and experimental advances concerning fluid transport in carbon nanotubes. The varied flow characteristics predicted by molecular dynamics are described, as are the roles of defects and chirality on transport. Analytical models are increasingly being used to describe nanofluidic transport by relaxing many of the assumptions commonly used to describe bulk water. Recent experimental studies examine the size dependence of flow enhancements through carbon nanotubes and use varied spectroscopies to probe water structure and dynamics in these systems. Carbon nanotubes are finding increasing applications in biology, from protein filters to platforms for cell interrogation.
Reprint Address:
Holt, JK, NanOasis Technol, 4677 Meade St,Suite 210, Richmond, CA 94804 USA.
Research Institution addresses:
NanOasis Technol, Richmond, CA 94804 USA
E-mail Address:
jason.holt@nanoasisinc.com
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55
Times Cited:
0
Publisher:
WILEY-V C H VERLAG GMBH; PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
Subject Category:
Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter
ISSN:
0935-9648
DOI:
10.1002/adma.200900867
IDS Number:
502FH
========================================================================
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Title:
Proton Transport from Dendritic Helical-Pore-Incorporated Polymersomes
Authors:
Kim, AJ; Kaucher, MS; Davis, KP; Peterca, M; Imam, MR; Christian, NA; Levine, DH; Bates, FS; Percec, V; Hammer, DA
Author Full Names:
Kim, Anthony J.; Kaucher, Mark S.; Davis, Kevin P.; Peterca, Mihai; Imam, Mohammad R.; Christian, Natalie A.; Levine, Dalia H.; Bates, Frank S.; Percec, Virgil; Hammer, Daniel A.
Source:
ADVANCED FUNCTIONAL MATERIALS 19 (18): 2930-2936 SEP 23 2009
Language:
English
Document Type:
Article
KeyWords Plus:
VESICLES; COPOLYMERS; DIPEPTIDES; MEMBRANE; SOLUBILITY; LIPOSOMES; DYNAMICS; DIBLOCK; CHANNEL
Abstract:
The ability to add synthetic channels to polymersome (polymer vesicle) membranes could lead to novel membrane composites with unique selectivity and permeability. Proton transport through two different synthetic pores, self-assembled from either a dendritic dipeptide, (6Nf-3,4-3,5)12G2-CH2-Boc-L-Tyr-L-Ala-OMe, or a dendritic ester, (R)-4Bp-3,4-dm8G1-COOMe, incorporated into polymersome membranes are studied. Polymersomes; provide an excellent platform for studying such transport processes due to their robustness and mechanical and chemical stability compared to liposomes. It is found that the incorporated dendritic dipeptide and dendritic ester assemble into stable helical pores in the poly(ethylene oxide)-polybutadiene (PEO-PBD) polymersomes but not in the poly(2-methyloxazoline)-poly(dimethylsiloxane)-poly(2-methyl oxazoline) (PMOX-PDMS-PMOX) polymersomes. The incorporation is confirmed by circular dichroism (CD), changes in purely synthetic mechanical strength (e.g., area!
l expansion modulus) as assessed by micropipette aspiration, and cryo-TEM. In addition to the structural analyses, a transport measurement shows the incorporated dendritic helical pores allow facile transport of protons across the polymersome membranes after up to one month of storage. This integration of synthetic porous channels with polymersome substrates could provide a valuable tool for studying active transport processes in a composite membrane. These composites will ultimately expand the family of biologically inspired porous-membrane mimics.
Reprint Address:
Kim, AJ, Univ Penn, Dept Chem & Biomol Engn, Philadelphia, PA 19104 USA.
Research Institution addresses:
[Kim, Anthony J.; Levine, Dalia H.; Hammer, Daniel A.] Univ Penn, Dept Chem & Biomol Engn, Philadelphia, PA 19104 USA; [Christian, Natalie A.; Hammer, Daniel A.] Univ Penn, Dept Bioengn, Philadelphia, PA 19104 USA; [Kaucher, Mark S.; Peterca, Mihai; Imam, Mohammad R.; Percec, Virgil] Univ Penn, Dept Chem, Philadelphia, PA 19104 USA; [Davis, Kevin P.; Bates, Frank S.] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA
E-mail Address:
hammer@seas.upenn.edu
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Cited Reference Count:
22
Times Cited:
0
Publisher:
WILEY-V C H VERLAG GMBH; PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
Subject Category:
Chemistry, Multidisciplinary; Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary; Physics, Applied; Physics, Condensed Matter
ISSN:
1616-301X
DOI:
10.1002/adfm.200900076
IDS Number:
502EN
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