Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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AU Sparreboom, W
van den Berg, A
Eijkel, JCT
AF Sparreboom, W.
van den Berg, A.
Eijkel, J. C. T.
TI Principles and applications of nanofluidic transport
SO NATURE NANOTECHNOLOGY
LA English
DT Review
ID ELECTROKINETIC ENERGY-CONVERSION; PRESSURE-DRIVEN TRANSPORT;
HYDRODYNAMIC CHROMATOGRAPHY; CONCENTRATION POLARIZATION; HYDROPHOBIC
SURFACES; SILICA-NANOCHANNELS; CARBON NANOTUBES; POWER-GENERATION;
DNA-MOLECULES; ION-TRANSPORT
AB The evolution from microfluidic to nanofluidic systems has been
accompanied by the emergence of new fluid phenomena and the potential
for new nanofluidic devices. This review provides an introduction to
the theory of nanofluidic transport, focusing on the various forces
that influence the movement of both solvents and solutes through
nanochannels,and reviews the applications of nanofluidic devices in
separation science and energy conversion.
C1 [Sparreboom, W.; van den Berg, A.; Eijkel, J. C. T.] Univ Twente, MESA Inst Nanotechnol, BIOS Lab Chip Grp, NL-7500 AE Enschede, Netherlands.
RP Sparreboom, W, Univ Twente, MESA Inst Nanotechnol, BIOS Lab Chip Grp,
POB 217, NL-7500 AE Enschede, Netherlands.
EM w.sparreboom@utwente.nl
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NR 103
TC 0
PU NATURE PUBLISHING GROUP; MACMILLAN BUILDING, 4 CRINAN ST, LONDON N1
9XW, ENGLAND
SN 1748-3387
DI 10.1038/NNANO.2009.332
PD NOV
VL 4
IS 11
BP 713
EP 720
SC Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
GA 528AW
UT ISI:000272413500011
ER
PT J
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AU Ahadian, S
Mizuseki, H
Kawazoe, Y
AF Ahadian, Samad
Mizuseki, Hiroshi
Kawazoe, Yoshiyuki
TI An efficient tool for modeling and predicting fluid flow in nanochannels
SO JOURNAL OF CHEMICAL PHYSICS
LA English
DT Article
ID ARTIFICIAL NEURAL-NETWORKS; CARBON NANOTUBES; MOLECULAR-DYNAMICS;
CAPILLARY RISE; TRANSPORT; LIQUIDS; SURFACE; NANOFLUIDICS; IMBIBITION;
NANOPORES
AB Molecular dynamics simulations were performed to evaluate the
penetration of two different fluids (i.e., a Lennard-Jones fluid and a
polymer) through a designed nanochannel. For both fluids, the length of
permeation as a function of time was recorded for various wall-fluid
interactions. A novel methodology, namely, the artificial neural
network (ANN) approach was then employed for modeling and prediction of
the length of imbibition as a function of influencing parameters (i.e.,
time, the surface tension and the viscosity of fluids, and the
wall-fluid interaction). It was demonstrated that the designed ANN is
capable of modeling and predicting the length of penetration with
superior accuracy. Moreover, the importance of variables in the
designed ANN, i.e., time, the surface tension and the viscosity of
fluids, and the wall-fluid interaction, was demonstrated with the aid
of the so-called connection weight approach, by which all parameters
are simultaneously considered. It was revealed that the wall-fluid
interaction plays a significant role in such transport phenomena,
namely, fluid flow in nanochannels. (C) 2009 American Institute of
Physics. [doi: 10.1063/1.3253701]
C1 [Ahadian, Samad; Mizuseki, Hiroshi; Kawazoe, Yoshiyuki] Tohoku Univ, IMR, Sendai, Miyagi 9808577, Japan.
RP Ahadian, S, Tohoku Univ, IMR, Sendai, Miyagi 9808577, Japan.
EM ahadian@imr.edu
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NR 51
TC 0
PU AMER INST PHYSICS; CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON
QUADRANGLE, STE 1 N O 1,
MELVILLE, NY 11747-4501 USA
SN 0021-9606
DI 10.1063/1.3253701
PD NOV 14
VL 131
IS 18
AR 184506
SC Physics, Atomic, Molecular & Chemical
GA 528NY
UT ISI:000272454500026
ER
PT B
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AU Whitby, M
Thanou, M
Quirke, N
AF Whitby, M.
Thanou, M.
Quirke, N.
TI Enhanced Fluid Transport Through Carbon Nanopipes
SO NSTI NANOTECH 2008, VOL 3, TECHNICAL PROCEEDINGS
LA English
DT Proceedings Paper
DE nanopipes; nanotubes; carbon; nanofluidics; flow; plasma
ID NANOTUBES; ALUMINA; FLOW
AB Experimental measurement of fluid flow and diffusion through nanoscale
channels is important both for determining how classical theories of
fluid dynamics apply at very small length scales and with a view to
constructing practical nanofluidic devices. In this study, we observe
water flow enhancement of more than 250% in relatively large 271 +/- 31
nm diameter carbon nanopipes with plasma induced surface modification
of the carbon walls. Our findings have application in the development
of biomedical devices both for sensing and for delivery of therapeutic
drugs.
C1 [Whitby, M.; Thanou, M.; Quirke, N.] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England.
RP Whitby, M, Univ London Imperial Coll Sci Technol & Med, Dept Chem,
London SW7 2AZ, England.
CR CHE G, 1998, CHEM MATER, V10, P260
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JOSEPH S, 2008, NANOLETT
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WHITBY M, UNPUB
WHITBY M, 2007, NAT NANOTECHNOL, V2, P87, DOI 10.1038/nnano.2006.175
NR 9
TC 0
PU CRC PRESS-TAYLOR & FRANCIS GROUP; 6000 BROKEN SOUND PARKWAY NW, STE
300, BOCA RATON, FL 33487-2742 USA
BP 367
EP 369
GA BMF51
UT ISI:000272170200096
ER
PT B
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AU Fornasiero, F
Park, HG
Holt, JK
Stadermann, M
Kim, S
In, JB
Grigoropoulos, CP
Noy, A
Bakajin, O
AF Fornasiero, Francesco
Park, Hyung Gyu
Holt, Jason K.
Stadermann, Michael
Kim, Sangil
In, Jung Bin
Grigoropoulos, Costas P.
Noy, Aleksandr
Bakajin, Olgica
TI Nanofiltration of Electrolyte Solutions by Sub-2nm Carbon Nanotube
Membranes
SO NSTI NANOTECH 2008, VOL 2, TECHNICAL PROCEEDINGS
LA English
DT Proceedings Paper
DE carbon nanotube; membrane; ion exclusion; fast flow
ID WATER; TRANSPORT; GROWTH
AB Both MD simulations and experimental studies have shown that liquid and
gas flow through carbon nanotubes with nanometer size diameter is
exceptionally fast. For applications in separation technology,
selectivity is required together with fast flow. In this work, we use
pressure-driven filtration experiments to study ion exclusion in
silicon nitride/sub-2-nm CNT composite membranes as a function of
solution ionic strength, pH, and ion valence. We show that carbon
nanotube membranes exhibit significant ion exclusion at low salt
concentration. Our results support a rejection mechanism dominated by
electrostatic interactions between fixed membrane charges and mobile
ions, while steric and hydrodynamic effects appear to be less
important. Comparison with commercial nanofiltration membranes for
water softening reveals that our carbon nanotube membranes provides far
superior water fluxes for similar ion rejection capabilities.
C1 [Fornasiero, Francesco; Park, Hyung Gyu; Holt, Jason K.; Stadermann, Michael; Noy, Aleksandr; Bakajin, Olgica] Lawrence Livermore Natl Lab, CMELS, Biosci & Biotechnol Div, Livermore, CA 94550 USA.
RP Fornasiero, F, Lawrence Livermore Natl Lab, CMELS, Biosci & Biotechnol
Div, Livermore, CA 94550 USA.
CR CHEUNG CL, 2002, J PHYS CHEM B, V106, P2429
FORNASIERO F, 2008, PNAS IN PRESS
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10.1007/s00339-005-3256-7
YAMADA T, 2006, NAT NANOTECHNOL, V1, P131, DOI 10.1038/nnano.2006.95
NR 17
TC 0
PU CRC PRESS-TAYLOR & FRANCIS GROUP; 6000 BROKEN SOUND PARKWAY NW, STE
300, BOCA RATON, FL 33487-2742 USA
BP 106
EP 109
GA BMF49
UT ISI:000272169900030
ER
PT B
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*Order Full Text [ ]
AU Park, HG
In, J
Kim, S
Fornasiero, F
Holt, JK
Grigoropoulos, CP
Noy, A
Bakajin, O
AF Park, H. G.
In, J.
Kim, S.
Fornasiero, F.
Holt, J. K.
Grigoropoulos, C. P.
Noy, A.
Bakajin, O.
TI A High-Flux, Flexible Membrane with Parylene-encapsulated Carbon
Nanotubes
SO NSTI NANOTECH 2008, VOL 1, TECHNICAL PROCEEDINGS
LA English
DT Proceedings Paper
DE membrane; carbon nanotube; parylene; high-flux
ID BOUNDARY-CONDITIONS; MASS-TRANSPORT; WATER; NANOPORES; FABRICATION;
FLOW; ARRAYS
AB We present fabrication and characterization of a membrane based on
carbon nanotubes (CNTs) and parylene. Carbon nanotubes have shown
orders of magnitude enhancement in gas and water permeability compared
to estimates generated by conventional theories [1, 2]. Large area
membranes that exhibit flux enhancement characteristics of carbon
nanotubes may provide an economical solution to a variety of
technologies including water desalination [3] and gas sequestration
[4]. We report a novel method of making carbon nanotube-based, robust
membranes with large areas. A vertically aligned dense carbon nanotube
array is infiltrated with parylene. Parylene polymer creates a pinhole
free transparent film by exhibiting high surface conformity and
excellent crevice penetration. Using this moisture-, chemical- and
solvent-resistant polymer creates carbon nanotube membranes that
promise to exhibit high stability and biocompatibility. CNT membranes
are formed by releasing a free-standing film that consists of
parylene-infiltrated CNTs, followed by CNT uncapping on both sides of
the composite material. Thus fabricated membranes show flexibility and
ductility due to the parylene matrix material. These membranes have a
potential for applications that may require high flux, flexibility and
durability.
C1 [Park, H. G.; Fornasiero, F.; Holt, J. K.; Noy, A.; Bakajin, O.] LLNS LLC, Livermore, CA USA.
RP Park, HG, LLNS LLC, Livermore, CA USA.
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