Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
Alert Expires: 22 OCT 2009
Number of Citing Articles: 4 new records this week (4 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Intrinsic Ion Selectivity of Narrow Hydrophobic Pores
Authors:
Song, C; Corry, B
Author Full Names:
Song, Chen; Corry, Ben
Source:
JOURNAL OF PHYSICAL CHEMISTRY B 113 (21): 7642-7649 MAY 28 2009
Language:
English
Document Type:
Article
KeyWords Plus:
CARBON NANOTUBE MEMBRANES; FREE-ENERGY CALCULATIONS; MOLECULAR-DYNAMICS; MEAN FORCE; ACETYLCHOLINE-RECEPTOR; POTASSIUM CHANNEL; PEPTIDE NANOTUBE; WATER TRANSPORT; MASS-TRANSPORT; K+ ION
Abstract:
We show that narrow hydrophobic pores have an intrinsic ion selectivity by using single-walled carbon nanotube membranes as a model. We examined pores of radius 3.4-6.1 angstrom, and conducted molecular dynamics simulations to show that Na+, K+, and Cl- face different free energy barriers when entering hydrophobic pores. Most of the differences result from the different dehydration energies of the ions; however, changes in the solvation shell structure in the confined nanotube interior and van der Waals interactions in the small tubes can both play a role. Molecular dynamics simulations conducted under hydrostatic pressure show that carbon nanotube membranes can act as ion sieves, with the pore radius and pressure determining which ions will permeate through the membrane. This work suggests that the intrinsic ion selectivity of biological pores of differing radii might also play a role in determining their selectivity, in addition to the more common explanations based on ele!
ctrostatic effects. In addition, "hydrophobic gating" can arise in continuous water-filled pores.
Reprint Address:
Corry, B, Univ Western Australia, Sch Biomed Biomol & Chem Sci, Crawley, WA 6009, Australia.
Research Institution addresses:
[Song, Chen; Corry, Ben] Univ Western Australia, Sch Biomed Biomol & Chem Sci, Crawley, WA 6009, Australia
E-mail Address:
ben.corry@uwa.edu.au
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Cited Reference Count:
52
Times Cited:
0
Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Subject Category:
Chemistry, Physical
ISSN:
1520-6106
DOI:
10.1021/jp810102u
IDS Number:
448YA
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Title:
Fabrication and characterization of carbon nanotubes immobilized in porous polymeric membranes
Authors:
Sae-Khow, O; Mitra, S
Author Full Names:
Sae-Khow, Ornthida; Mitra, Somenath
Source:
JOURNAL OF MATERIALS CHEMISTRY 19 (22): 3713-3718 2009
Language:
English
Document Type:
Article
KeyWords Plus:
MIXED MATRIX MEMBRANES; HOLLOW-FIBER MEMBRANES; GAS SEPARATION; BENZENE/CYCLOHEXANE MIXTURES; PERVAPORATION SEPARATION; POLY(VINYL ALCOHOL); HYBRID MEMBRANES; BARRIER FILM; EXTRACTION; CHROMATOGRAPHY
Abstract:
We demonstrate that the incorporation of carbon nanotubes (CNTs) in the pores of a membrane can offer several advantages. A dispersion of CNTs in polyvinylidene fluoride was injected through a porous membrane, which immobilized the nanotubes in the pore structure. The CNTs served as a sorbent facilitating solute exchange between the two phases leading to enhancement of the enrichment factor by as much as 93%. The presence of CNTs also developed a diffusion barrier by sorbing solvent on its surface, which led to higher retention of the extractant within the membrane.
Reprint Address:
Mitra, S, New Jersey Inst Technol, Dept Chem & Environm Sci, Newark, NJ 07102 USA.
Research Institution addresses:
[Sae-Khow, Ornthida; Mitra, Somenath] New Jersey Inst Technol, Dept Chem & Environm Sci, Newark, NJ 07102 USA
E-mail Address:
Mitra@njit.edu
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Cited Reference Count:
30
Times Cited:
0
Publisher:
ROYAL SOC CHEMISTRY; THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND
Subject Category:
Chemistry, Physical; Materials Science, Multidisciplinary
ISSN:
0959-9428
DOI:
10.1039/b822879e
IDS Number:
450OO
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Title:
Determinants of Water Permeability through Nanoscopic Hydrophilic Channels
Authors:
Portella, G; de Groot, BL
Author Full Names:
Portella, Guillem; de Groot, Bert L.
Source:
BIOPHYSICAL JOURNAL 96 (3): 925-938 FEB 4 2009
Language:
English
Document Type:
Article
KeyWords Plus:
PARTICLE MESH EWALD; SINGLE-FILE PORE; MOLECULAR-DYNAMICS; GRAMICIDIN CHANNEL; PEPTIDE NANOTUBES; PROTON EXCLUSION; CARBON NANOTUBE; CELL-MEMBRANE; ION CHANNELS; FORCE-FIELD
Abstract:
Naturally occurring pores show a variety of polarities and sizes that are presumably directly linked to their biological function. Many biological channels are selective toward permeants similar or smaller in size than water molecules, and therefore their pores operate in the regime of single-file water pores. Intrinsic factors affecting water permeability through such pores include the channel-membrane match, the structural stability of the channel, the channel geometry and channel-water affinity. We present an extensive molecular dynamics study on the role of the channel geometry and polarity on the water osmotic and diffusive permeability coefficients. We show that the polarity of the naturally occurring peptidic channels is close to optimal for water permeation, and that the water mobility for a wide range of channel polarities is essentially length independent. By systematically varying the geometry and polarity of model hydrophilic pores, based on the fold of gramicidi!
n A, the water density, occupancy, and permeability are studied. Our focus is on the characterization of the transition between different permeation regimes in terms of the structure of water in the pores, the average pore occupancy and the dynamics of the permeating water molecules. We show that a general relationship between osmotic and diffusive water permeability coefficients in the single-file regime accounts for the time averaged pore occupancy, and that the dynamics of the permeating water molecules through narrow non single file channels effectively behaves like independent single-file columns.
Reprint Address:
de Groot, BL, Max Planck Inst Biophys Chem, Computat Biomol Dynam Grp, D-37077 Gottingen, Germany.
Research Institution addresses:
[Portella, Guillem; de Groot, Bert L.] Max Planck Inst Biophys Chem, Computat Biomol Dynam Grp, D-37077 Gottingen, Germany
E-mail Address:
bgroot@gwdg.de
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65
Times Cited:
0
Publisher:
ELSEVIER SCI LTD; THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, OXON, ENGLAND
Subject Category:
Biophysics
ISSN:
0006-3495
DOI:
10.1016/j.bpj.2008.09.059
IDS Number:
450CB
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Title:
Dielectric Properties of Water inside Single-Walled Carbon Nanotubes
Authors:
Mikami, F; Matsuda, K; Kataura, H; Maniwa, Y
Author Full Names:
Mikami, Fuminori; Matsuda, Kazuyuki; Kataura, Hiromichi; Maniwa, Yutaka
Source:
ACS NANO 3 (5): 1279-1287 MAY 2009
Language:
English
Document Type:
Article
Author Keywords:
carbon nanotubes; ferroelectric; water; ice nanotubes; dielectric property
KeyWords Plus:
X-RAY-DIFFRACTION; ICE-NANOTUBES; LIQUID WATER; TRANSITION; DYNAMICS
Abstract:
In this paper, we report novel ferroelectric properties of a new form of ice inside single-walled carbon nanotubes (SWCNTs). These are called "ice nanotubes" (ice NTs) and they consist of polygonal water rings stacked one-dimensionally along the SWCNT axis. We performed molecular dynamics (MD) calculations for the ice NTs under an external electric field and in a temperature range between 100 and 350 K. It is revealed that ice NTs show stepwise polarization with a significant hysteresis loop as a function of the external field strength. In particular, pentagonal and heptagonal ice NTs are found to be the world's smallest ferroelectrics with spontaneous polarization of around 1 mu C/cm(2). The n-gonal ice NT, where n = 5, 6, or 7, has (n + 1)-polarized structures with different polarizations. These findings suggest potential applications of SWCNTs encapsulating dielectric materials for the fabrication of the smallest ferroelectric devices. Experimental evidence for the presen!
ce of ice NTs inside SWCNTs is also discussed in great detail.
Reprint Address:
Maniwa, Y, Tokyo Metropolitan Univ, Fac Sci, Dept Phys, 1-1 Minami Osawa, Tokyo 1920397, Japan.
Research Institution addresses:
[Mikami, Fuminori; Matsuda, Kazuyuki; Maniwa, Yutaka] Tokyo Metropolitan Univ, Fac Sci, Dept Phys, Tokyo 1920397, Japan; [Kataura, Hiromichi] Natl Inst Adv Ind Sci & Technol, Nanotechnol Inst, Tsukuba, Ibaraki 3058562, Japan; [Kataura, Hiromichi; Maniwa, Yutaka] JST, CREST, Kawaguchi, Saitama 3320012, Japan
E-mail Address:
maniwa@phys.metro-u.ac.jp
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Cited Reference Count:
32
Times Cited:
0
Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Subject Category:
Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
ISSN:
1936-0851
DOI:
10.1021/nn900221t
IDS Number:
449IH
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If you have any questions, please visit the Thomson Scientific Technical Support Contact Information Web page:
http://www.thomsonscientific.com/support/techsupport
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