Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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AU Hanggi, P
Marchesoni, F
AF Haenggi, Peter
Marchesoni, Fabio
TI Artificial Brownian motors: Controlling transport on the nanoscale
SO REVIEWS OF MODERN PHYSICS
LA English
DT Review
DE Brownian motion; fluctuations; microfluidics; quantum theory;
superconducting devices; transport processes
ID MAGNETIC-FLUX QUANTA; ABSOLUTE NEGATIVE CONDUCTANCE;
FLUCTUATION-INDUCED TRANSPORT; MOLECULAR TRAFFIC CONTROL; SINGLE
KINESIN MOLECULES; NOISE-INDUCED TRANSPORT; FREE-ENERGY DIFFERENCES;
LONG DNA-MOLECULES; CARBON NANOTUBES; THERMAL RATCHETS
AB In systems possessing spatial or dynamical symmetry breaking, Brownian
motion combined with unbiased external input signals, deterministic and
random alike, can assist directed motion of particles at submicron
scales. In such cases, one speaks of "Brownian motors." In this review
the constructive role of Brownian motion is exemplified for various
physical and technological setups, which are inspired by the cellular
molecular machinery: the working principles and characteristics of
stylized devices are discussed to show how fluctuations, either thermal
or extrinsic, can be used to control diffusive particle transport.
Recent experimental demonstrations of this concept are surveyed with
particular attention to transport in artificial, i.e., nonbiological,
nanopores, lithographic tracks, and optical traps, where
single-particle currents were first measured. Much emphasis is given to
two- and three-dimensional devices containing many interacting
particles of one or more species; for this class of artificial motors,
noise rectification results also from the interplay of particle
Brownian motion and geometric constraints. Recently, selective control
and optimization of the transport of interacting colloidal particles
and magnetic vortices have been successfully achieved, thus leading to
the new generation of microfluidic and superconducting devices
presented here. The field has recently been enriched with impressive
experimental achievements in building artificial Brownian motor devices
that even operate within the quantum domain by harvesting quantum
Brownian motion. Sundry akin topics include activities aimed at
noise-assisted shuttling other degrees of freedom such as charge, spin,
or even heat and the assembly of chemical synthetic molecular motors.
This review ends with a perspective for future pathways and potential
new applications.
C1 [Haenggi, Peter] Univ Augsburg, Inst Phys, D-86135 Augsburg, Germany.
[Haenggi, Peter] Natl Univ Singapore, Dept Phys, Singapore 117542, Singapore.
[Haenggi, Peter] Natl Univ Singapore, Ctr Computat Sci & Engn, Singapore 117542, Singapore.
[Marchesoni, Fabio] Univ Camerino, Dipartimento Fis, I-62032 Camerino, Italy.
[Marchesoni, Fabio] Korea Inst Adv Study, Sch Phys, Seoul 130722, South Korea.
RP Hanggi, P, Univ Augsburg, Inst Phys, Univ Str 1, D-86135 Augsburg,
Germany.
EM peter.hanggi@physik.uni-augsburg.de
fabio.marchesoni@pg.infn.it
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NR 398
TC 0
PU AMER PHYSICAL SOC; ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 0034-6861
DI 10.1103/RevModPhys.81.387
PD JAN-MAR
VL 81
IS 1
BP 387
EP 442
SC Physics, Multidisciplinary
GA 427FG
UT ISI:000264764600009
ER
PT J
*Record 2 of 4.
L5 <http://gateway.isiknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcAuth=Alerting&SrcApp=Alerting&DestApp=WOS&DestLinkType=FullRecord;UT=000265030000006>
*Order Full Text [ ]
AU Vermesh, U
Choi, JW
Vermesh, O
Fan, R
Nagarah, J
Heath, JR
AF Vermesh, Udi
Choi, Jang Wook
Vermesh, Ophir
Fan, Rong
Nagarah, John
Heath, James R.
TI Fast Nonlinear Ion Transport via Field-induced Hydrodynamic Slip in
Sub-20-nm Hydrophilic Nanofluidic Transistors
SO NANO LETTERS
LA English
DT Article
ID CARBON NANOTUBES; ENERGY-CONVERSION; CHANNELS; FLOW; FABRICATION
AB Electrolyte transport through an array of 20 nm wide, 20 mu m long SiO2
nanofluldic transistors is described. At sufficiently low ionic
strength, the Debye screening length exceeds the channel width, and ion
transport is limited by the negatively charged channel surfaces. At
source-drain biases >5 V, the current exhibits a sharp, nonlinear
increase, with a 20-50-fold conductance enhancement. This behavior is
attributed to a breakdown of the zero-slip condition. Implications for
energy conversion devices are discussed.
C1 [Choi, Jang Wook; Vermesh, Ophir; Fan, Rong; Nagarah, John; Heath, James R.] CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA.
CALTECH, Kavli Nanosci Inst, Pasadena, CA 91125 USA.
[Vermesh, Udi] CALTECH, Div Engn & Appl Sci, Pasadena, CA 91125 USA.
RP Heath, JR, CALTECH, Div Chem & Chem Engn, Pasadena, CA 91125 USA.
EM heath@caltech.edu
CR BOCQUET L, 2007, SOFT MATTER, V3, P685, DOI 10.1039/b616490k
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10.1016/j.memsci.2004.07.009
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10.1016/j.jcis.2007.07.027
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VLASSIOUK I, 2007, NANO LETT, V7, P552, DOI 10.1021/nl062924b
NR 25
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1530-6984
DI 10.1021/nl802931r
PD APR
VL 9
IS 4
BP 1315
EP 1319
SC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary
GA 430ZB
UT ISI:000265030000006
ER
PT J
*Record 3 of 4.
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*Order Full Text [ ]
AU Xiu, P
Zhou, B
Qi, WP
Lu, HJ
Tu, YS
Fang, HP
AF Xiu, Peng
Zhou, Bo
Qi, Wenpeng
Lu, Hangjun
Tu, Yusong
Fang, Haiping
TI Manipulating Biomolecules with Aqueous Liquids Confined within
Single-Walled Nanotubes
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID DIP-PEN NANOLITHOGRAPHY; CARBON NANOTUBES; WATER CHANNEL;
MASS-TRANSPORT; PROTEIN; MEMBRANES; PEPTIDE; ICE; SIMULATIONS; SOLVATION
AB Confinement of molecules inside nanoscale pores has become an important
method for exploiting new dynamics not happening in bulk systems and
for fabricating novel structures. Molecules that are encapsulated in
nanopores are difficult to control with respect to their position and
activity. On the basis of molecular dynamics simulations, we have
achieved controllable manipulation, both in space and time, of
biomolecules with aqueous liquids inside a single-walled nanotube by
using an external charge or a group of external charges. The remarkable
manipulation abilities are attributed to the single-walled structure of
the nanotube that the electrostatic interactions of charges inside and
outside the single-walled nanotube are strong enough, and the
charge-induced dipole-orientation ordering of water confined in the
nanochannel so that water has a strong interaction with the external
charge. These designs are expected to serve as lab-in-nanotube for the
interactions and chemical reactions of molecules especially
biomolecules, and have wide applications in nanotechnology and
biotechnology.
C1 [Xiu, Peng; Zhou, Bo; Qi, Wenpeng; Lu, Hangjun; Tu, Yusong; Fang, Haiping] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China.
[Xiu, Peng; Qi, Wenpeng] Shandong Univ, Sch Phys, Jinan 250100, Peoples R China.
[Zhou, Bo; Tu, Yusong] Chinese Acad Sci, Grad Sch, Beijing 100080, Peoples R China.
[Lu, Hangjun] Zhejiang Normal Univ, Dept Phys, Jinhua 321004, Peoples R China.
[Fang, Haiping] CAS, Theoret Phys Ctr Sci Facil, Beijing 100049, Peoples R China.
RP Fang, HP, Chinese Acad Sci, Shanghai Inst Appl Phys, POB 800-204,
Shanghai 201800, Peoples R China.
EM fanghaiping@sinap.ac.cn
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10.1073/pnas.0402699101
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ZHOU RH, 2004, SCIENCE, V305, P1605
ZIMMERLI U, 2008, BIOPHYS J, V94, P2546, DOI 10.1529/biophysj.106.102467
NR 62
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
DI 10.1021/ja804586w
PD MAR 4
VL 131
IS 8
BP 2840
EP 2845
SC Chemistry, Multidisciplinary
GA 427PX
UT ISI:000264792300036
ER
PT J
*Record 4 of 4.
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*Order Full Text [ ]
AU Wang, L
Zhao, JJ
Li, FY
Fang, HP
Lu, JP
AF Wang, Lu
Zhao, Jijun
Li, Fengyu
Fang, Haiping
Lu, Jian Ping
TI First-Principles Study of Water Chains Encapsulated in Single-Walled
Carbon Nanotube
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID DENSITY-FUNCTIONAL THEORY; INFRARED PREDISSOCIATION SPECTRA;
SIZE-SELECTED WATER; LIQUID WATER; AB-INITIO; SUPERCRITICAL WATER;
MOLECULAR-BEAM; VIBRATIONAL-SPECTRA; INTERACTION ENERGY; CLUSTERS
(H2O)(N)
AB Water molecules confined inside a single-walled (6, 6) carbon nanotube
were investigated using density functional theory. In this narrow-sized
carbon nanotube (of about 0.8 nm in diameter), the encapsulated water
molecules form chain-like configurations via hydrogen bonding. As
compared to the water chains in vacuum, the intramolecular charge
transfer in the encapsulated water chain is enhanced and the dipole
moment is reduced due to the screening effect of the carbon nanotube.
The tube-molecule interaction characterized by the coupling energy is
about 0.28 eV per water molecule by local density approximation and 0.1
eV by general gradient approximation; the latter one is close to the
results by empirical potentials. Weak coupling between the molecular
orbitals of the encapsulated water molecules and the delocalized pi
electrons from the carbon nanotube was observed, implying that the
tube-water interaction is not a simple effect of geometry confinement.
Vibrational analysis revealed some unique hydrogen-bond modes for the
water chains as well as red shift of the O-H stretching modes for the
encapsulated water molecules with regard to the vacuum frequencies due
to the tube-water interaction.
C1 [Wang, Lu; Zhao, Jijun; Li, Fengyu] Dalian Univ Technol, Sch Phys & Optoelect Technol, Dalian 116024, Peoples R China.
[Wang, Lu; Zhao, Jijun; Li, Fengyu] Dalian Univ Technol, Coll Adv Sci & Technol, Dalian 116024, Peoples R China.
[Fang, Haiping] Chinese Acad Sci, Shanghai Inst Appl Phys, Shanghai 201800, Peoples R China.
[Lu, Jian Ping] Univ N Carolina, Dept Phys & Astron, Chapel Hill, NC 27599 USA.
RP Zhao, JJ, Dalian Univ Technol, Sch Phys & Optoelect Technol, Dalian
116024, Peoples R China.
EM zhaojj@dlut.edu.cn
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NR 90
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
DI 10.1021/jp808873r
PD APR 9
VL 113
IS 14
BP 5368
EP 5375
SC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
GA 427UX
UT ISI:000264805700006
ER
EF
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