Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
Alert Expires: 09 NOV 2010
Number of Citing Articles: 4 new records this week (4 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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AU Yang, LJ
Gao, YQ
AF Yang, Lijiang
Gao, Yi Qin
TI Effects of Cosolvents on the Hydration of Carbon Nanotubes
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID AQUEOUS UREA SOLUTIONS; MOLECULAR-DYNAMICS; HYDROPHOBIC INTERACTIONS;
WATER; PROTEINS; DENATURATION; TRANSPORT; STABILITY; MECHANISM; SYSTEMS
AB Molecular dynamics simulations of a nonpolar single-walled carbon
nanotube (SWNT) solvated in aqueous solutions of urea, methanol, and
trimethylamine N-oxide (TMAO) show clearly the effects of cosolvents on
the hydration of the interior of the SWNT. The size of the SWNT was
chosen to be small enough that water but not the cosolvent molecules
can penetrate into its interior. Urea as a protein denaturant improves
hydration of the interior of the SWNT, while the protein protectant
TMAO dehydrates the SWNT. The interior of the SWNT is also dehydrated
when methanol is added to the solution. The analysis of interaction
energies of the water confined inside the SWNT pore shows that the
stability of the confined water in the methanol and TMAO solutions
mainly depends on electrostatic interactions. In contrast, both van der
Waals and electrostatic interactions were shown to be important in
stabilizing the confined water when the SWNT is immersed in the urea
solution.
C1 [Yang, Lijiang; Gao, Yi Qin] Texas A&M Univ, Dept Chem, College Stn, TX 77842 USA.
RP Gao, YQ, Texas A&M Univ, Dept Chem, POB 30012, College Stn, TX 77842
USA.
EM yiqin@mail.chem.tamu.edu
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NR 30
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
DI 10.1021/ja9091825
PD JAN 20
VL 132
IS 2
BP 842
EP 848
SC Chemistry, Multidisciplinary
GA 562VY
UT ISI:000275084600065
ER
PT J
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AU Gong, XJ
Li, JC
Xu, K
Wang, JF
Yang, H
AF Gong, Xiaojing
Li, Jichen
Xu, Ke
Wang, Jianfeng
Yang, Hui
TI A Controllable Molecular Sieve for Na+ and K+ Ions
SO JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
LA English
DT Article
ID CARBON NANOTUBE MEMBRANES; POTASSIUM CHANNELS; MASS-TRANSPORT; WATER
CHANNEL; SELECTIVITY; CONDUCTION; FLOW; NANOPORES
AB The selective rate of specific ion transport across nanoporous material
is critical to biological and nanofluidic systems Molecular sieves for
ions can be achieved by steric and electrical effects However, the
radii of Na+ and K+ are quite similar, they both carry a positive
charge, making them difficult to separate Biological ionic channels
contain precisely arranged arrays of amino acids that can efficiently
recognize and guide the passage of K+ or Na+ across the cell membrane
However, the design of inorganic channels with novel recognition
mechanisms that control the ionic selectivity remains a challenge. We
present here a design for a controllable ion-selective nanopore
(molecular sieve) based on a single-walled carbon nanotube with
specially arranged carbonyl oxygen atoms modified inside the nanopore,
which was inspired by the structure of potassium channels in membrane
spanning proteins (e g, KcsA) Our molecular dynamics simulations show
that the remarkable selectivity is attributed to the hydration
structure of Na+ or K+ confined in the nanochannels, which can be
precisely tuned by different patterns of the carbonyl oxygen atoms The
results also suggest that a confined environment plays a dominant role
in the selectivity process. These studies provide a better
understanding of the mechanism of ionic selectivity in the KcsA channel
and possible technical applications in nanotechnology and
biotechnology, including serving as a laboratory-in-nanotube for
special chemical interactions and as a high-efficiency nanodevice for
purification or desalination of sea and brackish water
C1 [Gong, Xiaojing; Xu, Ke; Wang, Jianfeng; Yang, Hui] Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion, Suzhou 215125, Peoples R China.
[Yang, Hui] Univ Sci & Technol China, Dept Phys, Hefei 230026, Peoples R China.
[Li, Jichen] Univ Manchester, Dept Phys & Astron, Manchester M13 9PL, Lancs, England.
RP Gong, XJ, Chinese Acad Sci, Suzhou Inst Nanotech & Nanobion, Suzhou
215125, Peoples R China.
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NR 38
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 0002-7863
DI 10.1021/ja905753p
PD FEB 17
VL 132
IS 6
BP 1873
EP 1877
SC Chemistry, Multidisciplinary
GA 562WC
UT ISI:000275085000049
ER
PT J
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AU Rivera, JL
Starr, FW
AF Rivera, Jose L.
Starr, Francis W.
TI Rapid Transport of Water via a Carbon Nanotube Syringe
SO JOURNAL OF PHYSICAL CHEMISTRY C
LA English
DT Article
ID MOLECULAR-DYNAMICS; FLOW; CONDUCTION; MEMBRANES; CHANNEL; FILMS
AB The controlled flow of water molecules at the nanoscale is an initial
step to many fluidic processes ill nanotechnology. Here we show how
thin films of water call be drawn through a nanosyringe built from a
carbon nanotube membrane and a "plunger". By increasing the speed of
withdrawal of the plunger, we call obtain Molecular transport through
the membrane at flux rates exceeding 1()25 molecules cm(-2) s(-1).
Above I threshold speed around 0.25 nm/ns (25 cm/s), molecules cannot
fill the chamber created by the plunger motion as fast as the chamber
expands, and the resulting flux rate drops. By considering hydrophobic
or hydrophilic Plungers, we unexpectedly find that the nature of the
water-plunger interactions does not affect the flux rate or the
threshold plunger speed. While the water structure near the plunger
Surface differs significantly For different plunger interactions, the
failure of the film away From the plunger surface is responsible for
loss of transport. As I result, the surface interactions play a limited
role in controlling the flux.
C1 [Rivera, Jose L.; Starr, Francis W.] Wesleyan Univ, Dept Phys, Middletown, CT 06457 USA.
[Rivera, Jose L.] Univ Nacl Autonoma Mexico, Inst Invest Mat, Mexico City 04510, DF, Mexico.
RP Starr, FW, Wesleyan Univ, Dept Phys, Middletown, CT 06457 USA.
EM joserivera@iim.unam.mx
fstarr@wesleyan.edu
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NR 33
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1932-7447
DI 10.1021/jp906527c
PD MAR 11
VL 114
IS 9
BP 3737
EP 3742
SC Chemistry, Physical; Nanoscience & Nanotechnology; Materials Science,
Multidisciplinary
GA 562JG
UT ISI:000275045600003
ER
PT J
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AU Kocherginsky, N
AF Kocherginsky, N.
TI Mass transport and membrane separations: Universal description in terms
of physicochemical potential and Einstein's mobility
SO CHEMICAL ENGINEERING SCIENCE
LA English
DT Article
DE Membranes; Energy; Entropy; Separations; Transport processes; Linear
thermodynamics; Reverse osmosis; Barodiffusion; Solution-diffusion model
ID SOLUTION-DIFFUSION MODEL; PERMEABILITY; VOLUME; WATER
AB General yet simple description of chemical transport processes in
non-isolated system is suggested. It is based on extended Teorell
equation and just two fundamental parameters: physicochemical potential
and Einstein's mobility. Using mobility it is possible to compare the
rates of all major linear transport phenomena, including
pressure-driven migration and also nonideal and multicomponent
diffusion. Relationship with the Stefan-Maxwell approach and Onsager's
linear thermodynamics is demonstrated and physical interpretation of
both diagonal and off-diagonal phenomenological coefficients is
suggested. Imposing boundary conditions for transport equations allows
description of transport in homogeneous membranes caused by several
concurrent driving factors, such as concentration, pressure, and
voltage. Differences of barodiffusion, membrane filtration, and reverse
osmosis are considered. For a porous membrane an expression for the
pressure-driven volumetric flux through the pores as a function of
mobility and pore size is derived. It is explained why hydraulic flow
prevails in submicron pores and why diffusion is the dominant mechanism
in reverse osmosis if the pressure difference is not too high. The
theory naturally leads to the solution-diffusion model equations but
does not need usual assumptions of constant pressure across the
membrane and the pressure jump only at one surface. Internal pressure
and mechanical stress gradients within a membrane exist and can be
useful in a description of rheology of aging polymer membranes. A new
equation for concurrent diffusion and hydraulic transport is derived
and two possible molecular mechanisms leading to the Kedem-Katchalsky
equations for reverse osmosis membranes are suggested. Finally,
electrokinetic processes are described and their similarity to
concentration- and pressure-driven transport is discussed. (C) 2009
Elsevier Ltd. All rights reserved.
C1 Biomime, Urbana, IL 61801 USA.
RP Kocherginsky, N, Biomime, 909 E Sunnycrest Dr, Urbana, IL 61801 USA.
EM biomime@gmail.com
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NR 55
TC 0
PU PERGAMON-ELSEVIER SCIENCE LTD; THE BOULEVARD, LANGFORD LANE,
KIDLINGTON, OXFORD OX5 1GB, ENGLAND
SN 0009-2509
DI 10.1016/j.ces.2009.10.024
PD FEB 15
VL 65
IS 4
BP 1474
EP 1489
SC Engineering, Chemical
GA 564MA
UT ISI:000275217500017
ER
EF
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