Cited Article: Hummer, G. Water conduction through the hydrophobic channel of a carbon nanotube
Alert Expires: 09 NOV 2010
Number of Citing Articles: 6 new records this week (6 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Diameter Selectivity of Protein Encapsulation in Carbon Nanotubes
Authors:
Kang, Y; Wang, Q; Liu, YC; Shen, JW; Wu, T
Author Full Names:
Kang, Yu; Wang, Qi; Liu, Ying-Chun; Shen, Jia-Wei; Wu, Tao
Source:
JOURNAL OF PHYSICAL CHEMISTRY B 114 (8): 2869-2875 MAR 4 2010
Language:
English
Document Type:
Article
KeyWords Plus:
STEERED MOLECULAR-DYNAMICS; MEAN FORCE; TRANSPORTERS; SIMULATIONS; POTENTIALS; MECHANISM; AMYLOSE; CHANNEL; HELICES; CELLS
Abstract:
Biomolecular-carbon nanotube (CNT) complexes are of great importance in biological and biomedical devices, and recently spontaneous encapsulation of biomolecules into CNTs has attracted great interest. In this work, we explored the diameter selectivity of the protein encapsulation in CNTs via molecular dynamics simulations, and the free energy changes of the systems were calculated for mechanism exploration. It is proved that there is an optimal tube size which provides the most effective encapsulation for a given protein molecule, and the encapsulations in the overlarge and overcrowded tubes are hindered by different factors based on the analysis of system energy contribution. In addition, the significance of the solvents for the system is also of concern.
Reprint Address:
Wang, Q, Zhejiang Univ, Dept Chem, Hangzhou 310027, Peoples R China.
Research Institution addresses:
[Kang, Yu; Wang, Qi; Liu, Ying-Chun; Shen, Jia-Wei; Wu, Tao] Zhejiang Univ, Dept Chem, Hangzhou 310027, Peoples R China
E-mail Address:
qiwang@zju.edu.cn; liuyingch@zju.edu.cn
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Cited Reference Count:
36
Times Cited:
0
Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Subject Category:
Chemistry, Physical
ISSN:
1520-6106
DOI:
10.1021/jp905995s
IDS Number:
559QZ
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Title:
A water chain with trimeric/hexameric clusters trapped in a POM/Ln compound
Authors:
Pang, HJ; Zhang, CJ; Chen, YG; Shi, DM
Author Full Names:
Pang, Hai-Jun; Zhang, Chun-Jing; Chen, Ya-Guang; Shi, Dong-Mei
Source:
JOURNAL OF COORDINATION CHEMISTRY 63 (3): 418-425 2010
Language:
English
Document Type:
Article
Author Keywords:
Polyoxometalate; Water chain; Lanthanide; Luminescence properties
KeyWords Plus:
CRYSTAL-STRUCTURE; SOLID-STATE; 3-DIMENSIONAL FRAMEWORK; SUPRAMOLECULAR COMPLEX; METAL-COMPLEXES; PROTON-TRANSFER; RARE-EARTH; HYBRID; CHANNEL; CATIONS
Abstract:
A new 3-D supramolecular compound based on a Keggin polyoxometalate and lanthanide (Ln) coordination cations [Ce(H2O)3L3]2[HSiMo12O40]2[L] 7H2O (1) (L = isonicotinic acid) has been synthesized and characterized by routine methods. Compound 1 has a water chain with trimeric and hexameric water clusters trapped in the network. The isonicotinic acid plays a key role in forming the 1-D water chains. Compound 1 shows intense photoluminescence at room temperature.
Reprint Address:
Chen, YG, NE Normal Univ, Fac Chem, Key Lab Polyoxometalates Sci, Minist Educ, Changchun 130024, Peoples R China.
Research Institution addresses:
[Pang, Hai-Jun; Zhang, Chun-Jing; Chen, Ya-Guang; Shi, Dong-Mei] NE Normal Univ, Fac Chem, Key Lab Polyoxometalates Sci, Minist Educ, Changchun 130024, Peoples R China
E-mail Address:
chenyg146@nenu.edu.cn
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Cited Reference Count:
56
Times Cited:
0
Publisher:
TAYLOR & FRANCIS LTD; 4 PARK SQUARE, MILTON PARK, ABINGDON OX14 4RN, OXON, ENGLAND
Subject Category:
Chemistry, Inorganic & Nuclear
ISSN:
0095-8972
DOI:
10.1080/00958970903474225
IDS Number:
562DI
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Title:
Structural Water Drives Self-assembly of Organic Rosette Nanotubes and Holds Host Atoms in the Channel
Authors:
Yamazaki, T; Fenniri, H; Kovalenko, A
Author Full Names:
Yamazaki, Takeshi; Fenniri, Hicham; Kovalenko, Andriy
Source:
CHEMPHYSCHEM 11 (2): 361-367 FEB 1 2010
Language:
English
Document Type:
Article
Author Keywords:
molecular theory of solvation; rosette nanotube; self-assembly; solvent effects; water channel
KeyWords Plus:
CARBON NANOTUBES; FUNCTIONALIZED XENON; BIOLOGICAL WATER; MOLECULAR-BASIS; PROTEIN; TRANSPORT; CONDUCTION; SOLVATION; BIOSENSOR; MEMBRANES
Abstract:
We reveal how water solvent determines the self-assembly pathway and stability of organic rosette nanotubes (RNTs) and show their possible functions, using three-dimensional molecular theory of solvation (a.k.a. 3D-RISM). Structural water molecules penetrate the pockets on the RNT outer surface, form a wetting monolayer in the RNT channel and bridge RNT rosettes. We predict that the inner water shell might stabilizer rare gas atoms inside the RNT channel, and envision molecular devices with RNT channels transporting water or holding guest molecules for targeted delivery.
Reprint Address:
Fenniri, H, Univ Alberta, Dept Chem, 11421 Saskatchewan Dr, Edmonton, AB T6G 2M9, Canada.
Research Institution addresses:
[Fenniri, Hicham] Univ Alberta, Dept Chem, Edmonton, AB T6G 2M9, Canada; [Yamazaki, Takeshi; Fenniri, Hicham; Kovalenko, Andriy] Natl Inst Nanotechnol, Edmonton, AB T6G 2M9, Canada; [Kovalenko, Andriy] Univ Alberta, Dept Mech Engn, Edmonton, AB T6G 2M9, Canada
E-mail Address:
hicham.fenniri@ualberta.ca; andriy.kovalenko@nrc-cnrc.gc.ca
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34
Times Cited:
0
Publisher:
WILEY-V C H VERLAG GMBH; PO BOX 10 11 61, D-69451 WEINHEIM, GERMANY
Subject Category:
Chemistry, Physical; Physics, Atomic, Molecular & Chemical
ISSN:
1439-4235
DOI:
10.1002/cphc.200900324
IDS Number:
559RI
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Title:
Nanofluidics, from bulk to interfaces
Authors:
Bocquet, L; Charlaix, E
Author Full Names:
Bocquet, Lyderic; Charlaix, Elisabeth
Source:
CHEMICAL SOCIETY REVIEWS 39 (3): 1073-1095 2010
Language:
English
Document Type:
Review
KeyWords Plus:
SOLID-STATE NANOPORES; HYDRODYNAMIC BOUNDARY-CONDITIONS; THIN LIQUID-FILMS; CARBON NANOTUBES; HYDROPHOBIC SURFACES; SMOOTH SURFACES; TRANSPORT PHENOMENA; ENERGY-CONVERSION; WATER TRANSPORT; FLOW
Abstract:
Nanofluidics has emerged recently in the footsteps of microfluidics, following the quest for scale reduction inherent to nanotechnologies. By definition, nanofluidics explores transport phenomena of fluids at nanometer scales. Why is the nanometer scale specific? What fluid properties are probed at nanometric scales? In other words, why does 'nanofluidics' deserve its own brand name? In this critical review, we will explore the vast manifold of length scales emerging for fluid behavior at the nanoscale, as well as the associated mechanisms and corresponding applications. We will in particular explore the interplay between bulk and interface phenomena. The limit of validity of the continuum approaches will be discussed, as well as the numerous surface induced effects occurring at these scales, from hydrodynamic slippage to the various electro-kinetic phenomena originating from the couplings between hydrodynamics and electrostatics. An enlightening analogy between ion transpor!
t in nanochannels and transport in doped semi-conductors will be discussed (156 references).
Reprint Address:
Bocquet, L, Univ Lyon 1, Lab Phys Matiere Condensee & Nanostruct, 43 Bvd 11 Nov 1918, F-69622 Villeurbanne, France.
Research Institution addresses:
[Bocquet, Lyderic] Univ Lyon 1, Lab Phys Matiere Condensee & Nanostruct, F-69622 Villeurbanne, France; CNRS, UMR 5586, F-69622 Villeurbanne, France
E-mail Address:
lyderic.bocquet@univ-lyon1.fr
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153
Times Cited:
1
Publisher:
ROYAL SOC CHEMISTRY; THOMAS GRAHAM HOUSE, SCIENCE PARK, MILTON RD, CAMBRIDGE CB4 0WF, CAMBS, ENGLAND
Subject Category:
Chemistry, Multidisciplinary
ISSN:
0306-0012
DOI:
10.1039/b909366b
IDS Number:
560RR
========================================================================
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Title:
Cellular behavior of human mesenchymal stem cells cultured on single-walled carbon nanotube film
Authors:
Tay, CY; Gu, HG; Leong, WS; Yu, HY; Li, HQ; Heng, BC; Tantang, H; Loo, SCJ; Li, LJ; Tan, LP
Author Full Names:
Tay, Chor Yong; Gu, Haigang; Leong, Wen Shing; Yu, Haiyang; Li, Hua Qiong; Heng, Boon Chen; Tantang, Hosea; Loo, Say Chye Joachim; Li, Lain Jong; Tan, Lay Poh
Source:
CARBON 48 (4): 1095-1104 APR 2010
Language:
English
Document Type:
Article
KeyWords Plus:
IN-VITRO; NEURAL PROTEINS; DIFFERENTIATION; GROWTH; ADHESION; BIOCOMPATIBILITY; PROLIFERATION; KERATINOCYTES; CYTOTOXICITY; CROSSTALK
Abstract:
The influences of carboxylic functionalized single-walled carbon nanotubes (SWCNTs) on cell adhesion, spreading and cell lineage commitment of human mesenchymal stem cells (hMSCs) were evaluated. hMSCs were cultured on a thin mesh like layer of SWCNTs with a vertical height of less than 100 nm. The influence of the SWCNT film was significant on the cell spreading and focal adhesion distribution. Cells spread better on a SWCNT film as compared to cover slip (control), resulting in larger cell area and have higher occurrence of filopodia (microspikes) at the cell boundaries. Cytoskeleton arrangement was observed to be less orientated in the cells cultured on a SWCNT film as compared to control. Neurogenic markers such as nestin, glial fibrillary acidic protein and microtubule associated protein 2 genes were transiently upregulated (a process where cellular components, in this case RNA, is increased in response to external variable) over the first week while genes indicative of!
osteogenesis remained at its nominal level. These results suggest that nano roughness alone is sufficient to modulate cellular behavior and early stage of stem cell lineage commitment without the aid of an induction medium. (C) 2009 Elsevier Ltd. All rights reserved.
Reprint Address:
Tan, LP, Nanyang Technol Univ, Mat Technol Div, Sch Mat Sci & Engn, 50 Nanyang Ave, Singapore 639798, Singapore.
Research Institution addresses:
[Tay, Chor Yong; Gu, Haigang; Leong, Wen Shing; Yu, Haiyang; Li, Hua Qiong; Heng, Boon Chen; Tantang, Hosea; Loo, Say Chye Joachim; Li, Lain Jong; Tan, Lay Poh] Nanyang Technol Univ, Mat Technol Div, Sch Mat Sci & Engn, Singapore 639798, Singapore
E-mail Address:
lptan@ntu.edu.sg
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Cited Reference Count:
46
Times Cited:
0
Publisher:
PERGAMON-ELSEVIER SCIENCE LTD; THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
Subject Category:
Chemistry, Physical; Materials Science, Multidisciplinary
ISSN:
0008-6223
DOI:
10.1016/j.carbon.2009.11.031
IDS Number:
559MO
========================================================================
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Title:
Interaction energies, structure, and dynamics at functionalized graphitic structure-liquid phase interfaces in an aqueous calcium sulfate solution by molecular dynamics simulation
Authors:
Sanchez, F; Zhang, L
Author Full Names:
Sanchez, F.; Zhang, L.
Source:
CARBON 48 (4): 1210-1223 APR 2010
Language:
English
Document Type:
Article
KeyWords Plus:
CARBON NANOTUBES; WATER-ADSORPTION; COMPUTER-SIMULATION; SURFACES; COMPOSITES; DIFFUSION; MODEL; IONS; ENERGETICS; NANOPORES
Abstract:
Molecular dynamics simulations were performed to study the effect of surface functionalization of graphitic structures on the molecular-scale energetic, structure, and dynamics of water and ions at graphite surface-liquid phase interfaces. Three types of carbon surface structures were investigated: a pristine graphite plane and two graphite planes functionalized with hydroxyl (-OH) and carboxylate (-COO-, deprotonated carboxyl) groups. A divalent salt, calcium sulfate, was combined with water to simulate an electrolyte liquid phase. Results highlighted the ordering of H2O molecules that occurs near graphite surfaces and revealed a subtle effect on the position of the H2O layers associated with ions and functional group type. Surface functionalization of the graphitic structures affected the H-bond network and the orientation of near-surface H2O molecules, decreased the ion hydration, and significantly restrained the mobility of near-surface H2O molecules and bulk Ca2+ and SO!
42- ions. (C) 2009 Elsevier Ltd. All rights reserved.
Reprint Address:
Sanchez, F, Vanderbilt Univ, Dept Civil & Environm Engn, VU B35 1831, Nashville, TN 37235 USA.
Research Institution addresses:
[Sanchez, F.; Zhang, L.] Vanderbilt Univ, Dept Civil & Environm Engn, Nashville, TN 37235 USA
E-mail Address:
florence.sanchez@vanderbilt.edu
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Times Cited:
0
Publisher:
PERGAMON-ELSEVIER SCIENCE LTD; THE BOULEVARD, LANGFORD LANE, KIDLINGTON, OXFORD OX5 1GB, ENGLAND
Subject Category:
Chemistry, Physical; Materials Science, Multidisciplinary
ISSN:
0008-6223
DOI:
10.1016/j.carbon.2009.11.044
IDS Number:
559MO
========================================================================
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