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Title: Spatial Dependence of Viscosity and Thermal Conductivity through a Planar Interface |
Authors: |
Author Full Names: Petravic, Janka; Harrowell, Peter |
Source: JOURNAL OF PHYSICAL CHEMISTRY B 113 (7): 2059-2065 FEB 19 2009 |
Language: English |
Document Type: Article |
KeyWords Plus: LIQUID-SOLID INTERFACE; MOLECULAR-DYNAMICS; RESISTANCE; SURFACES; FLOW |
Abstract: We present a general algorithm for calculating the spatial variation of the shear viscosity and thermal conductivity through an equilibrium solid-liquid interface using the zero-flux version of the boundary fluctuation theory. In the case of an equilibrium interface between a high melting point Lennard-Jones solid and a low melting point Lennard-Jones liquid, we find that the transport coefficients deviate from the bulk values only in a narrow layer close to the interface. We observe a sliding friction of the liquid against the surface of the solid that increases with increased wetting of the solid by the liquid. The thermal conductivity, in contrast, is suppressed in the interfacial region, irrespective of how the liquid wets the solid. |
Reprint Address: Petravic, J, Univ Sydney, Sch Chem, Sydney, NSW 2006, Australia. |
Research Institution addresses: [Petravic, Janka; Harrowell, Peter] Univ Sydney, Sch Chem, Sydney, NSW 2006, Australia |
Cited References: ALLEN MP, 1987, COMPUTER SIMULATION. BARRAT JL, 1994, PHYS REV E, V49, P3079. BARRAT JL, 2003, MOL PHYS, V101, P1605, DOI 10.1080/0026897031000068578. BOCQUET L, 1997, J STAT PHYS, V89, P321. COTTINBIZONNE C, 2005, PHYS REV LETT, V94, P6102. EVANS DJ, 1993, PHYS REV E, V48, P65. GE ZB, 2006, PHYS REV LETT, V96, ARTN 186101. GUO HX, 2002, PHYS REV E 1, V66, ARTN 061503. HELFAND E, 1960, PHYS REV, V119, P1. MCQUARRIE DA, 2000, STAT MECH. PETRAVIC J, 2005, PHYS REV E 1, V71, ARTN 061201. PETRAVIC J, 2006, J CHEM PHYS, V124, ARTN 014103. PETRAVIC J, 2006, J CHEM PHYS, V124, ARTN 044512. PETRAVIC J, 2008, J CHEM PHYS, V128, ARTN 194710. SIMON JM, 2004, J PHYS CHEM B, V108, P7186, DOI 10.1021/jp0375719. THOMPSON PA, 1990, PHYS REV A, V41, P6830. THOMPSON PA, 1997, NATURE, V389, P360. VINOGRADOVA OI, 1995, LANGMUIR, V11, P2213. XUE L, 2003, J CHEM PHYS, V118, P337, DOI 10.1063/1.1525806. |
Cited Reference Count: 19 |
Times Cited: 0 |
Publisher: AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA |
Subject Category: Chemistry, Physical |
ISSN: 1520-6106 |
DOI: 10.1021/jp807254b |
IDS Number: 406MK |
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Title: A continuum model for the flow of thin liquid films over intermittently chemically patterned surfaces |
Authors: |
Author Full Names: Sprittles, J. E.; Shikhmurzaev, Y. D. |
Source: EUROPEAN PHYSICAL JOURNAL-SPECIAL TOPICS 166: 159-163 JAN 2009 |
Language: English |
Document Type: Proceedings Paper |
Abstract: It is known from both experiments and molecular dynamics simulations that chemically patterning a solid surface has an effect on the flow of an adjacent liquid. This fact is in stark contrast with predictions of classical fluid mechanics where the no-slip boundary condition is insensitive to the chemistry of the solid substrate. It has been shown that the influence on the flow caused by a steep change in the wettability of the solid substrate can be described in the framework of continuum mechanics using the interface formation theory. The present work extends this study to the case of intermittent patterning. Results show that variations in wettability of the substrate can significantly affect the flow, especially of thin films, which may have applications to the design of microfluidic devices. |
Reprint Address: Sprittles, JE, Univ Birmingham, Sch Math, Birmingham B15 2TT, W Midlands, England. |
Research Institution addresses: [Sprittles, J. E.; Shikhmurzaev, Y. D.] Univ Birmingham, Sch Math, Birmingham B15 2TT, W Midlands, England |
E-mail Address: sprittlj@maths.bham.ac.uk; yulii@for.mat.bham.ac.uk |
Cited References: BLAKE TD, 2002, J COLLOID INTERF SCI, V253, P196, DOI 10.1006/jcis.2002.8513. COTTINBIZONNE C, 2005, PHYS REV LETT, V94, P6102. LAUGA E, 2003, J FLUID MECH, V489, P55, DOI 10.1017/S0022112003004695. LAUGA E, 2005, HDB EXPT FLUID DYNAM. NAVIER CLM, 1823, MEMOIRES ACAD ROYALE, V6, P389. PRIEZJEV NV, 2005, PHYS REV E 1, V71, P1608. SHIKHMURZAEV YD, 2005, IMA J APPL MATH, V70, P880, DOI 10.1093/imamat/hxh075. SHIKHMURZAEV YD, 2006, PHYSICA D, V217, P121, DOI 10.1016/j.physd.2006.03.003. SHIKHMURZAEV YD, 2007, CAPILLARY FLOWS FORM. SOKHAN VP, 2001, J CHEM PHYS, V115, P3878. SPRITTLES JE, 2007, PHYS REV E 1, V76, P1602. TABELING P, 2006, INTRO MICROFLUIDICS. THOMPSON PA, 1997, NATURE, V389, P360. |
Cited Reference Count: 13 |
Times Cited: 0 |
Publisher: EDP SCIENCES S A; 17, AVE DU HOGGAR, PA COURTABOEUF, BP 112, F-91944 LES ULIS CEDEX A, FRANCE |
Subject Category: Physics, Multidisciplinary |
ISSN: 1951-6355 |
DOI: 10.1140/epjst/e2009-00899-5 |
IDS Number: 404VO |
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