Cited Article: Holt JK. Fast mass transport through sub-2-nanometer carbon nanotubes
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Number of Citing Articles: 4 new records this week (4 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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AU Gruener, S
Hofmann, T
Wallacher, D
Kityk, AV
Huber, P
AF Gruener, Simon
Hofmann, Tommy
Wallacher, Dirk
Kityk, Andriy V.
Huber, Patrick
TI Capillary rise of water in hydrophilic nanopores
SO PHYSICAL REVIEW E
LA English
DT Article
DE boundary layers; capillarity; capillary waves; flow through porous
media; hydrophilicity; nanofluidics; nanoporous materials; silicon
compounds; sorption; water
ID VYCOR GLASS; NEGATIVE PRESSURES; CARBON NANOTUBES; POROUS VYCOR;
DYNAMICS; FLOW; NANOSCALE; LIQUIDS; NANOFLUIDICS; ADSORPTION
AB We report on the capillary rise of water in three-dimensional networks
of hydrophilic silica pores with 3.5 nm and 5 nm mean radii,
respectively (porous Vycor monoliths). We find classical square root of
time Lucas-Washburn laws for the imbibition dynamics over the entire
capillary rise times of up to 16 h investigated. Provided we assume two
preadsorbed strongly bound layers of water molecules resting at the
silica walls, which corresponds to a negative velocity slip length of
-0.5 nm for water flow in silica nanopores, we can describe the filling
process by a retained fluidity and capillarity of water in the pore
center. This anticipated partitioning in two dynamic components
reflects the structural-thermodynamic partitioning in strongly silica
bound water layers and capillary condensed water in the pore center
which is documented by sorption isotherm measurements.
C1 [Gruener, Simon; Hofmann, Tommy; Huber, Patrick] Univ Saarland, Fac Phys & Mechatron Engn, D-66041 Saarbrucken, Germany.
[Wallacher, Dirk] Helmholtz Ctr Mat & Energy, D-14109 Berlin, Germany.
[Kityk, Andriy V.] Czestochowa Univ Technol, Inst Comp Sci, PL-42220 Czestochowa, Poland.
RP Gruener, S, Univ Saarland, Fac Phys & Mechatron Engn, D-66041
Saarbrucken, Germany.
EM s.gruener@mx.uni-saarland.de
p.huber@physik.uni-saarland.de
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NR 58
TC 0
PU AMER PHYSICAL SOC; ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
SN 1539-3755
DI 10.1103/PhysRevE.79.067301
PD JUN
VL 79
IS 6
PN Part 2
AR 067301
SC Physics, Fluids & Plasmas; Physics, Mathematical
GA 466XP
UT ISI:000267698900086
ER
PT J
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AU Okazaki, M
Seelan, S
Toriyama, K
AF Okazaki, M.
Seelan, S.
Toriyama, K.
TI Condensation process of alcohol molecules on mesoporous silica MCM-41
and SBA-15 and fumed silica: a spin-probe ESR study
SO APPLIED MAGNETIC RESONANCE
LA English
DT Proceedings Paper
ID LIQUID-PHASE PHOTOREACTION; CARBON NANOTUBES; DIFFUSION; FLOW;
NANOCHANNEL; MECHANISM; DYNAMICS; NMR
AB A few alcoholic solutions of di-tert-butyl nitroxide (DTBN), a spin
probe, at a high concentration were condensed on several silica
materials, such as MCM-41, two types of SBA-15, and fumed silica, at
various amounts in vacuum. At a very low solution dose the electron
spin resonance (ESR) spectrum is that of an immobilized nitroxide
radical. With increasing solution dose, the spectrum is gradually
sharpened and a well-separated three-line spectrum is observed at the
dose that is estimated to fill the surface with a monomolecular layer.
Thus, the DTBN molecule can make rapid tumbling motion on this solvent
layer. With a further increase in the solution dose the ESR spectrum is
modified in different ways from system to system: the line width
increases approximately linearly with respect to the solution dose for
the SBA-15 and fumed silica systems, but it remains almost constant for
the MCM-41 system until the solution dose exceeds the total volume of a
nanochannel. The line width increase with respect to the solution dose
is small for the SBA-15 system but large for the fumed silica system.
These results have been interpreted geometrically with the structures
of these silica materials and a condensation model for the alcohols on
these surfaces. In relation to the present results, a model of the
collective molecular flow of the alcohol solutions through the
nanochannel of MCM-41 is given.
C1 [Okazaki, M.] Natl Inst Adv Ind Sci & Technol, Res Inst Instrumentat Frontier, Moriyama Ku, Nagoya, Aichi 4638560, Japan.
RP Okazaki, M, Natl Inst Adv Ind Sci & Technol, Res Inst Instrumentat
Frontier, Moriyama Ku, 2266-98 Shimoshidami, Nagoya, Aichi 4638560,
Japan.
EM masa-okazaki@aist.go.jp
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10.1016/j.micromeso.2005.07.036
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NR 26
TC 0
PU SPRINGER WIEN; SACHSENPLATZ 4-6, PO BOX 89, A-1201 WIEN, AUSTRIA
SN 0937-9347
DI 10.1007/s00723-009-0168-2
PD APR
VL 35
IS 3
BP 363
EP 378
SC Physics, Atomic, Molecular & Chemical; Spectroscopy
GA 466NM
UT ISI:000267668900002
ER
PT J
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AU Zang, J
Konduri, S
Nair, S
Sholl, DS
AF Zang, Ji
Konduri, Suchitra
Nair, Sankar
Sholl, David S.
TI Self-Diffusion of Water and Simple Alcohols in Single-Walled
Aluminosilicate Nanotubes
SO ACS NANO
LA English
DT Article
DE inorganic nanotubes; aluminosilicate; self-diffusion; water; methanol;
ethanol
ID MIXED-OXIDE NANOTUBES; FAST MASS-TRANSPORT; CARBON NANOTUBE; IMOGOLITE
NANOTUBES; CORRELATED FLIGHTS; MEMBRANES; MODELS; NANOPARTICLES;
RESISTANCES; DIMENSIONS
AB Understanding transport phenomena of fluids through nanotubes (NTs) is
of great interest in order to enable potential application of NTs as
separation devices, encapsulation media for molecule storage and
delivery, and sensors. Single-walled metal oxide NTs are interesting
materials because they present a well-defined solid-state structure,
precisely tunable diameter and length, as well as a hydrophilic and
functionalizable interior for tuning transport and adsorption
selectivity. Here, we study the transport properties of
hydrogen-bonding liquids (water, methanol, and ethanol) through a
single-walled aluminosilicate NT to investigate the influence of
liquid-surface and liquid-liquid interactions and the effects of
competitive transport of different chemical species using molecular
dynamics (MD) simulations. The self-diffusivities (D-s) for all the
three species decrease with increasing loading and are comparable to
bulk liquid diffusivities at low molecular loadings. We show that the
hydrogen-bond network associated with water makes its diffusion
behavior different from methanol and ethanol. Mixtures of water and
methanol show segregation in the NT, with water located closer to the
tube wall and the alcohol molecules localized near the center of the
NT. D, values of water in an analogous aluminogermanate NT are larger
than those in the aluminosilicate NT due to a larger pore diameter.
C1 [Zang, Ji; Konduri, Suchitra; Nair, Sankar; Sholl, David S.] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA.
RP Sholl, DS, Georgia Inst Technol, Sch Chem & Biomol Engn, 311 Ferst Dr
NW, Atlanta, GA 30332 USA.
EM david.sholl@chbe.gatech.edu
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NR 37
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1936-0851
DI 10.1021/nn9001837
PD JUN
VL 3
IS 6
BP 1548
EP 1556
SC Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials
Science, Multidisciplinary
GA 464UP
UT ISI:000267533600032
ER
PT J
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AU Nuxoll, EE
Hillmyer, MA
Wang, RF
Leighton, C
Siegel, RA
AF Nuxoll, Eric E.
Hillmyer, Marc A.
Wang, Ruifang
Leighton, C.
Siegel, Ronald A.
TI Composite Block Polymer-Microfabricated Silicon Nanoporous Membrane
SO ACS APPLIED MATERIALS & INTERFACES
LA English
DT Article
DE microelectromechanical system; nanoporous; membrane; block polymer;
size selectivity
ID POLYLACTIDE DIBLOCK COPOLYMERS; THIN-FILMS; FILTRATION MEMBRANES;
TRIBLOCK COPOLYMERS; TRANSPORT; POLYSTYRENE; ARRAYS
AB Block polymers offer an attractive route to densely packed,
monodisperse nanoscale pores. However, their fragility as thin films
complicates their use as membranes. By integrating a block polymer film
with a thin (100 mu m) silicon substrate, we have developed a composite
membrane providing both nanoscale size exclusion and fast transport of
small molecules. Here we describe the fabrication of this membrane,
evaluate its mechanical integrity, and demonstrate its transport
properties for model solutes of large and small molecular weight. The
ability to block large molecules without hindering smaller ones,
coupled with the potential for surface modification of the polymer and
the microelectromechanical system style of support, makes this
composite membrane an attractive candidate for interfacing implantable
sensing and drug-delivery devices with biological hosts.
C1 [Nuxoll, Eric E.; Siegel, Ronald A.] Univ Minnesota, Dept Pharmaceut, Minneapolis, MN 55455 USA.
[Hillmyer, Marc A.] Univ Minnesota, Dept Chem, Minneapolis, MN 55455 USA.
[Wang, Ruifang; Leighton, C.] Univ Minnesota, Dept Chem Engn & Mat Sci, Minneapolis, MN 55455 USA.
[Siegel, Ronald A.] Univ Minnesota, Dept Biomed Engn, Minneapolis, MN 55455 USA.
RP Siegel, RA, Univ Minnesota, Dept Pharmaceut, 9-177 Weaver Densford
Hall,308 Harvard St SE, Minneapolis, MN 55455 USA.
EM siege017@umn.edu
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NR 38
TC 0
PU AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
SN 1944-8244
DI 10.1021/am900013v
PD APR
VL 1
IS 4
BP 888
EP 893
GA 464VM
UT ISI:000267536100021
ER
EF
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