Cited Article: Majumder M. Nanoscale hydrodynamics - Enhanced flow in carbon nanotubes
Alert Expires: 18 OCT 2009
Number of Citing Articles: 4 new records this week (4 in this e-mail)
Organization ID: 3b97d1bbc1878baed0ab183d8b03130b
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Title:
Capillary rise of water in hydrophilic nanopores
Authors:
Gruener, S; Hofmann, T; Wallacher, D; Kityk, AV; Huber, P
Author Full Names:
Gruener, Simon; Hofmann, Tommy; Wallacher, Dirk; Kityk, Andriy V.; Huber, Patrick
Source:
PHYSICAL REVIEW E 79 (6): Art. No. 067301 Part 2 JUN 2009
Language:
English
Document Type:
Article
Author Keywords:
boundary layers; capillarity; capillary waves; flow through porous media; hydrophilicity; nanofluidics; nanoporous materials; silicon compounds; sorption; water
KeyWords Plus:
VYCOR GLASS; NEGATIVE PRESSURES; CARBON NANOTUBES; POROUS VYCOR; DYNAMICS; FLOW; NANOSCALE; LIQUIDS; NANOFLUIDICS; ADSORPTION
Abstract:
We report on the capillary rise of water in three-dimensional networks of hydrophilic silica pores with 3.5 nm and 5 nm mean radii, respectively (porous Vycor monoliths). We find classical square root of time Lucas-Washburn laws for the imbibition dynamics over the entire capillary rise times of up to 16 h investigated. Provided we assume two preadsorbed strongly bound layers of water molecules resting at the silica walls, which corresponds to a negative velocity slip length of -0.5 nm for water flow in silica nanopores, we can describe the filling process by a retained fluidity and capillarity of water in the pore center. This anticipated partitioning in two dynamic components reflects the structural-thermodynamic partitioning in strongly silica bound water layers and capillary condensed water in the pore center which is documented by sorption isotherm measurements.
Reprint Address:
Gruener, S, Univ Saarland, Fac Phys & Mechatron Engn, D-66041 Saarbrucken, Germany.
Research Institution addresses:
[Gruener, Simon; Hofmann, Tommy; Huber, Patrick] Univ Saarland, Fac Phys & Mechatron Engn, D-66041 Saarbrucken, Germany; [Wallacher, Dirk] Helmholtz Ctr Mat & Energy, D-14109 Berlin, Germany; [Kityk, Andriy V.] Czestochowa Univ Technol, Inst Comp Sci, PL-42220 Czestochowa, Poland
E-mail Address:
s.gruener@mx.uni-saarland.de; p.huber@physik.uni-saarland.de
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Cited Reference Count:
58
Times Cited:
0
Publisher:
AMER PHYSICAL SOC; ONE PHYSICS ELLIPSE, COLLEGE PK, MD 20740-3844 USA
Subject Category:
Physics, Fluids & Plasmas; Physics, Mathematical
ISSN:
1539-3755
DOI:
10.1103/PhysRevE.79.067301
IDS Number:
466XP
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Title:
Transport properties and induced voltage in the structure of water-filled single-walled boron-nitrogen nanotubes
Authors:
Yuan, QZ; Zhao, YP
Author Full Names:
Yuan, Quanzi; Zhao, Ya-Pu
Source:
BIOMICROFLUIDICS 3 (2): Art. No. 022411 APR-JUN 2009
Language:
English
Document Type:
Proceedings Paper
Author Keywords:
boron compounds; density functional theory; diffusion; III-V semiconductors; molecular dynamics method; nanofluidics; pipe flow; semiconductor nanotubes; wide band gap semiconductors
KeyWords Plus:
CARBON NANOTUBES; MOLECULAR-DYNAMICS; NITRIDE NANOTUBES; CHANNEL; FLOW; LIQUIDS
Abstract:
Density functional theory/molecular dynamics simulations were employed to give insights into the mechanism of voltage generation based on a water-filled single-walled boron-nitrogen nanotube (SWBNNT). Our calculations showed that (1) the transport properties of confined water in a SWBNNT are different from those of bulk water in view of configuration, the diffusion coefficient, the dipole orientation, and the density distribution, and (2) a voltage difference of several millivolts would generate between the two ends of a SWBNNT due to interactions between the water dipole chains and charge carriers in the tube. Therefore, this structure of a water-filled SWBNNT can be a promising candidate for a synthetic nanoscale power cell as well as a practical nanopower harvesting device.
Reprint Address:
Zhao, YP, Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech LNM, Beijing 100190, Peoples R China.
Research Institution addresses:
[Yuan, Quanzi; Zhao, Ya-Pu] Chinese Acad Sci, Inst Mech, State Key Lab Nonlinear Mech LNM, Beijing 100190, Peoples R China
E-mail Address:
yzhao@imech.ac.cn
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28
Times Cited:
1
Publisher:
AMER INST PHYSICS; CIRCULATION & FULFILLMENT DIV, 2 HUNTINGTON QUADRANGLE, STE 1 N O 1, MELVILLE, NY 11747-4501 USA
Subject Category:
Biophysics; Nanoscience & Nanotechnology; Physics, Fluids & Plasmas
ISSN:
1932-1058
DOI:
10.1063/1.3158618
IDS Number:
465PW
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Title:
Condensation process of alcohol molecules on mesoporous silica MCM-41 and SBA-15 and fumed silica: a spin-probe ESR study
Authors:
Okazaki, M; Seelan, S; Toriyama, K
Author Full Names:
Okazaki, M.; Seelan, S.; Toriyama, K.
Source:
APPLIED MAGNETIC RESONANCE 35 (3): 363-378 APR 2009
Language:
English
Document Type:
Proceedings Paper
KeyWords Plus:
LIQUID-PHASE PHOTOREACTION; CARBON NANOTUBES; DIFFUSION; FLOW; NANOCHANNEL; MECHANISM; DYNAMICS; NMR
Abstract:
A few alcoholic solutions of di-tert-butyl nitroxide (DTBN), a spin probe, at a high concentration were condensed on several silica materials, such as MCM-41, two types of SBA-15, and fumed silica, at various amounts in vacuum. At a very low solution dose the electron spin resonance (ESR) spectrum is that of an immobilized nitroxide radical. With increasing solution dose, the spectrum is gradually sharpened and a well-separated three-line spectrum is observed at the dose that is estimated to fill the surface with a monomolecular layer. Thus, the DTBN molecule can make rapid tumbling motion on this solvent layer. With a further increase in the solution dose the ESR spectrum is modified in different ways from system to system: the line width increases approximately linearly with respect to the solution dose for the SBA-15 and fumed silica systems, but it remains almost constant for the MCM-41 system until the solution dose exceeds the total volume of a nanochannel. The line wi!
dth increase with respect to the solution dose is small for the SBA-15 system but large for the fumed silica system. These results have been interpreted geometrically with the structures of these silica materials and a condensation model for the alcohols on these surfaces. In relation to the present results, a model of the collective molecular flow of the alcohol solutions through the nanochannel of MCM-41 is given.
Reprint Address:
Okazaki, M, Natl Inst Adv Ind Sci & Technol, Res Inst Instrumentat Frontier, Moriyama Ku, 2266-98 Shimoshidami, Nagoya, Aichi 4638560, Japan.
Research Institution addresses:
[Okazaki, M.] Natl Inst Adv Ind Sci & Technol, Res Inst Instrumentat Frontier, Moriyama Ku, Nagoya, Aichi 4638560, Japan
E-mail Address:
masa-okazaki@aist.go.jp
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Cited Reference Count:
26
Times Cited:
0
Publisher:
SPRINGER WIEN; SACHSENPLATZ 4-6, PO BOX 89, A-1201 WIEN, AUSTRIA
Subject Category:
Physics, Atomic, Molecular & Chemical; Spectroscopy
ISSN:
0937-9347
DOI:
10.1007/s00723-009-0168-2
IDS Number:
466NM
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Title:
Self-Diffusion of Water and Simple Alcohols in Single-Walled Aluminosilicate Nanotubes
Authors:
Zang, J; Konduri, S; Nair, S; Sholl, DS
Author Full Names:
Zang, Ji; Konduri, Suchitra; Nair, Sankar; Sholl, David S.
Source:
ACS NANO 3 (6): 1548-1556 JUN 2009
Language:
English
Document Type:
Article
Author Keywords:
inorganic nanotubes; aluminosilicate; self-diffusion; water; methanol; ethanol
KeyWords Plus:
MIXED-OXIDE NANOTUBES; FAST MASS-TRANSPORT; CARBON NANOTUBE; IMOGOLITE NANOTUBES; CORRELATED FLIGHTS; MEMBRANES; MODELS; NANOPARTICLES; RESISTANCES; DIMENSIONS
Abstract:
Understanding transport phenomena of fluids through nanotubes (NTs) is of great interest in order to enable potential application of NTs as separation devices, encapsulation media for molecule storage and delivery, and sensors. Single-walled metal oxide NTs are interesting materials because they present a well-defined solid-state structure, precisely tunable diameter and length, as well as a hydrophilic and functionalizable interior for tuning transport and adsorption selectivity. Here, we study the transport properties of hydrogen-bonding liquids (water, methanol, and ethanol) through a single-walled aluminosilicate NT to investigate the influence of liquid-surface and liquid-liquid interactions and the effects of competitive transport of different chemical species using molecular dynamics (MD) simulations. The self-diffusivities (D-s) for all the three species decrease with increasing loading and are comparable to bulk liquid diffusivities at low molecular loadings. We sho!
w that the hydrogen-bond network associated with water makes its diffusion behavior different from methanol and ethanol. Mixtures of water and methanol show segregation in the NT, with water located closer to the tube wall and the alcohol molecules localized near the center of the NT. D, values of water in an analogous aluminogermanate NT are larger than those in the aluminosilicate NT due to a larger pore diameter.
Reprint Address:
Sholl, DS, Georgia Inst Technol, Sch Chem & Biomol Engn, 311 Ferst Dr NW, Atlanta, GA 30332 USA.
Research Institution addresses:
[Zang, Ji; Konduri, Suchitra; Nair, Sankar; Sholl, David S.] Georgia Inst Technol, Sch Chem & Biomol Engn, Atlanta, GA 30332 USA
E-mail Address:
david.sholl@chbe.gatech.edu
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Cited Reference Count:
37
Times Cited:
0
Publisher:
AMER CHEMICAL SOC; 1155 16TH ST, NW, WASHINGTON, DC 20036 USA
Subject Category:
Chemistry, Multidisciplinary; Nanoscience & Nanotechnology; Materials Science, Multidisciplinary
ISSN:
1936-0851
DOI:
10.1021/nn9001837
IDS Number:
464UP
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